Crystal growth and characterization of a hole-doped iron-based superconductor Ba(Fe0.875Ti0.125)2As2

doi:10.1088/1674-1056/ae0d5a

Abstract We report the crystal growth of a new hole-doped iron-based superconductor Ba(Fe$_{0.875}$Ti$_{0.125}$)$_2$As$_2$ by substituting Ti on the Fe site. The crystals are accidentally obtained in trying to grow Ni doped Ba$_2$Ti$_2$Fe$_2$As$_4$O. After annealing at 500~$^\circ$C in vacuum for one week, superconductivity is observed with zero resistance at $T_{\rm c0} \approx 17.5$ K, and about 20 % diamagnetic volume down to 2 K. While both the small anisotropy of superconductivity and the temperature dependence of normal state resistivity are akin to the electron doped 122-type compounds, the Hall coefficient is positive and similar to the case in hole-doped Ba$_{0.9}$K$_{0.1}$Fe$_2$As$_2$. The density functional theory calculations suggest dominated hole pockets contributed by Fe/Ti 3d orbitals. Therefore, the Ba(Fe$_{1-x}$Ti$_{x}$)$_2$As$_2$ system provides a new platform to study the superconductivity with hole doping on the Fe site of iron-based superconductors.

Keywords: iron-based superconductors crystal growth flux method hole-doped compounds

Received: 13 August 2025
Revised: 15 September 2025
Accepted manuscript online: 30 September 2025

PACS:	74.25.-q	(Properties of superconductors)
	74.25.Dw	(Superconductivity phase diagrams)
	74.70.-b	(Superconducting materials other than cuprates)
	74.25.Fy

Fund: This work is supported by the National Key R&D Program of China (Grant Nos. 2023YFA1406100, 2022YFA1403800, 2022YFA1403400, and 2021YFA1400400), the National Natural Science Foundation of China (Grant Nos. 12274444 and 12574165), the Chinese Academy of Sciences (Grant No. XDB25000000). DFT calculations are performed at the HPC facilities at RRCAT. AP acknowledges financial support from HBNI-RRCAT.

Corresponding Authors: Haranath Ghosh, Shi-Liang Li, Hui-Qian Luo
E-mail: hng@rrcat.gov.in;slli@iphy.ac.cn;hqluo@iphy.ac.cn

About author: 2025-127401-251405.pdf

Cite this article:

Yi-Li Sun(孙毅丽), Ze-Zhong Li(李泽众), Yang Li(李阳), Hong-Lin Zhou(周宏霖), Amit Pokhriyal, Haranath Ghosh, Shi-Liang Li(李世亮), and Hui-Qian Luo(罗会仟) Crystal growth and characterization of a hole-doped iron-based superconductor Ba(Fe_0.875Ti_0.125)₂As₂ 2025 Chin. Phys. B 34 127401

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Crystal growth and characterization of a hole-doped iron-based superconductor Ba(Fe0.875Ti0.125)2As2

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Crystal growth and characterization of a hole-doped iron-based superconductor Ba(Fe_0.875Ti_0.125)₂As₂