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Triphenylene adsorption on Cu(111) and relevant graphene self-assembly |
| Qiao-Yue Chen(陈乔悦)1, Jun-Jie Song(宋俊杰)3, Liwei Jing(井立威)1, Kaikai Huang(黄凯凯)1, Pimo He(何丕模)1,2, Hanjie Zhang(张寒洁)1 |
1 Zhejiang Province Key Laboratory of Quantum Technology and Device, Department of Physics, Zhejiang University, Hangzhou 310027, China;
2 Collaborative Innovation Center of Advanced Microstructure, Nanjing University, Nanjing 210093, China;
3 Department of Fundamental and Social Science, Zhejiang University of Water Resources and Electric Power, Hangzhou 310018, China |
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Abstract Investigations on adsorption behavior of triphenylene (TP) and subsequent graphene self-assembly on Cu(111) were carried out mainly by using scanning tunneling microscopy (STM). At monolayer coverage, TP molecules formed a long-range ordered adsorption structure on Cu(111) with an uniform orientation. Graphene self-assembly on the Cu(111) substrate with TP molecules as precursor was achieved by annealing the sample, and a large-scale graphene overlayer was successfully captured after the sample annealing up to 1000 K. Three different Moiré patterns generated from relative rotational disorders between the graphene overlayer and the Cu(111) substrate were observed, one with 4° rotation between the graphene overlayer and the Cu(111) substrate with a periodicity of 2.93 nm, another with 7° rotation and 2.15 nm of the size of the Moiré supercell, and the third with 10° rotation with a periodicity of 1.35 nm.
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Received: 04 November 2019
Revised: 16 December 2019
Accepted manuscript online:
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PACS:
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68.43.Fg
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(Adsorbate structure (binding sites, geometry))
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68.37.Ef
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(Scanning tunneling microscopy (including chemistry induced with STM))
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68.43.-h
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(Chemisorption/physisorption: adsorbates on surfaces)
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| Fund: Project supported by the National Key Research and Development Program of China (Grant No. 2017YFB0503100) and the National Natural Science Foundation of China (Grant No. 11790313). |
Corresponding Authors:
Pimo He, Hanjie Zhang
E-mail: zhj_fox@zju.edu.cn;phypmhe@zju.edu.cn
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Cite this article:
Qiao-Yue Chen(陈乔悦), Jun-Jie Song(宋俊杰), Liwei Jing(井立威), Kaikai Huang(黄凯凯), Pimo He(何丕模), Hanjie Zhang(张寒洁) Triphenylene adsorption on Cu(111) and relevant graphene self-assembly 2020 Chin. Phys. B 29 026801
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