Scaling behavior of thermal conductivity in single-crystalline α-Fe2O3 nanowires

doi:10.1088/1674-1056/ab90f0

Abstract Unveiling the thermal transport properties of various one-dimensional (1D) or quasi-1D materials like nanowires, nanotubes, and nanorods is of great importance both theoretically and experimentally. The dimension or size dependence of thermal conductivity is crucial in understanding the phonon-phonon interaction in the low-dimensional systems. In this paper, we experimentally investigate the size-dependent thermal conductivity of individual single crystalline α-Fe₂O₃ nanowires collaborating the suspended thermal bridge method and the focused electron-beam self-heating technique, with the sample diameter (d) ranging from 180 nm to 661 nm and length (L) changing from 4.84 μm to 20.73 μm. An empirical relationship for diameter-/length-dependent thermal conductivity is obtained, which shows an approximately linear dependence on the aspect ratio (L/(1+Cd)) at T=300 K, where C is a fitting parameter. This is related to the boundary scattering and diameter effect of α-Fe₂O₃ nanowires although rigorous calculations are needed to confirm the result.

Keywords: thermal conductivity size-dependent boundary scattering nanowire

Received: 25 March 2020
Revised: 30 April 2020
Accepted manuscript online:

PACS:	44.10.+i	(Heat conduction)
	63.22.-m	(Phonons or vibrational states in low-dimensional structures and nanoscale materials)
	63.20.-e	(Phonons in crystal lattices)

Fund: Project supported by the Key-Area Research and Development Program of Guangdong Province, China (Grant No. 2020B010190004), the National Natural Science Foundation of China (Grant Nos. 11674245, 11775158, 11890703, and 11935010), and the Open Fund of Zhejiang Provincial Key Laboratory of Quantum Technology and Device, China (Grant No. 20190301), and the Shanghai Committee of Science and Technology in China (Grant Nos. 17142202100, 17ZR1447900, and 17ZR1432600).

Corresponding Authors: Nianbei Li, Nianbei Li
E-mail: nbli@hqu.edu.cn;xuxiangfan@tongji.edu.cn

Cite this article:

Qilang Wang(王啟浪), Yunyu Chen(陈允玉), Adili Aiyiti(阿地力·艾依提), Minrui Zheng(郑敏锐), Nianbei Li(李念北), Xiangfan Xu(徐象繁) Scaling behavior of thermal conductivity in single-crystalline α-Fe₂O₃ nanowires 2020 Chin. Phys. B 29 084402

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Scaling behavior of thermal conductivity in single-crystalline α-Fe2O3 nanowires

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Scaling behavior of thermal conductivity in single-crystalline α-Fe₂O₃ nanowires