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Chin. Phys. B, 2018, Vol. 27(8): 086804    DOI: 10.1088/1674-1056/27/8/086804
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High quality PdTe2 thin films grown by molecular beam epitaxy

En Li(李恩)1, Rui-Zi Zhang(张瑞梓)1, Hang Li(李航)1, Chen Liu(刘晨)2, Geng Li(李更)1, Jia-Ou Wang(王嘉鸥)2, Tian Qian(钱天)1, Hong Ding(丁洪)1, Yu-Yang Zhang(张余洋)1, Shi-Xuan Du(杜世萱)1, Xiao Lin(林晓)1, Hong-Jun Gao(高鸿钧)1
1 Institute of Physics & University of Chinese Academy of Sciences, Chinese Academy of Sciences, Beijing 100190, China;
2 Institute of High Energy Physics, Chinese Academy of Sciences, Beijing 100049, China
Abstract  

PdTe2, a member of layered transition metal dichalcogenides (TMDs), has aroused significant research interest due to the coexistence of superconductivity and type-Ⅱ Dirac fermions. It provides a promising platform to explore the interplay between superconducting quasiparticles and Dirac fermions. Moreover, PdTe2 has also been used as a substrate for monolayer antimonene growth. Here in this paper, we report the epitaxial growth of high quality PdTe2 films on bilayer graphene/SiC(0001) by molecular beam epitaxy (MBE). Atomically thin films are characterized by scanning tunneling microscopy (STM), X-ray photoemission spectroscopy (XPS), low-energy electron diffraction (LEED), and Raman spectroscopy. The band structure of 6-layer PdTe2 film is measured by angle-resolved photoemission spectroscopy (ARPES). Moreover, our air exposure experiments show excellent chemical stability of epitaxial PdTe2 film. High-quality PdTe2 films provide opportunities to build antimonene/PdTe2 heterostructure in ultrahigh vacuum for future applications in electronic and optoelectronic nanodevices.

Keywords:  two-dimensional materials      transition-metal dichalcogenides      PdTe2      molecular beam epitaxy  
Received:  28 April 2018      Revised:  04 May 2018      Accepted manuscript online: 
PACS:  68.37.Ef (Scanning tunneling microscopy (including chemistry induced with STM))  
  68.55.-a (Thin film structure and morphology)  
  81.15.Hi (Molecular, atomic, ion, and chemical beam epitaxy)  
  61.05.jh (Low-energy electron diffraction (LEED) and reflection high-energy electron diffraction (RHEED))  
Corresponding Authors:  Xiao Lin, Hong-Jun Gao     E-mail:  xlin@ucas.ac.cn;hjgao@iphy.ac.cn

Cite this article: 

En Li(李恩), Rui-Zi Zhang(张瑞梓), Hang Li(李航), Chen Liu(刘晨), Geng Li(李更), Jia-Ou Wang(王嘉鸥), Tian Qian(钱天), Hong Ding(丁洪), Yu-Yang Zhang(张余洋), Shi-Xuan Du(杜世萱), Xiao Lin(林晓), Hong-Jun Gao(高鸿钧) High quality PdTe2 thin films grown by molecular beam epitaxy 2018 Chin. Phys. B 27 086804

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