Please wait a minute...
Chin. Phys. B, 2023, Vol. 32(5): 057301    DOI: 10.1088/1674-1056/aca396
CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES Prev   Next  

Room temperature quantum anomalous Hall insulator in honeycomb lattice, RuCS3, with large magnetic anisotropy energy

Yong-Chun Zhao(赵永春)1, Ming-Xin Zhu(朱铭鑫)1, Sheng-Shi Li(李胜世)2, and Ping Li(李萍)1,†
1 School of Physics and Technology, University of Jinan, Jinan 250022, China;
2 Institute of Spintronics, University of Jinan, Jinan 250022, China
Abstract  The quantum anomalous Hall (QAH) effect has attracted enormous attention since it can induce topologically protected conducting edge states in an intrinsic insulating material. For practical quantum applications, the main obstacle is the non-existent room temperature QAH systems, especially with both large topological band gap and robust ferromagnetic order. Here, according to first-principles calculations, we predict the realization of the room temperature QAH effect in a two-dimensional (2D) honeycomb lattice, RuCS3 with a non-zero Chern number of C = 1. Especially, the nontrivial topology band gap reaches up to 336 meV for RuCS3. Moreover, we find that RuCS3 has a large magnetic anisotropy energy (2.065 meV) and high Curie temperature (696 K). We further find that the non-trivial topological properties are robust against the biaxial strain. The robust topological and magnetic properties make RuCS3 have great applications in room temperature spintronics and nanoelectronics.
Keywords:  quantum anomalous Hall (QAH) effect      room temperature      magnetic anisotropy energy      topological properties      first-principles calculations  
Received:  05 August 2022      Revised:  22 October 2022      Accepted manuscript online:  17 November 2022
PACS:  73.20.At (Surface states, band structure, electron density of states)  
  75.50.Gg (Ferrimagnetics)  
  75.70.Ak (Magnetic properties of monolayers and thin films)  
Fund: Project supported by the Natural Science Foundation of Shandong Province, China (Grant No. ZR2019MA041), the Taishan Scholar Project of Shandong Province, China (Grant No. ts20190939), the National Natural Science Foundation of China (Grant No. 62071200), and the Shandong Provincial Natural Science Foundation, China (Grant No. ZR2020QA052).
Corresponding Authors:  Ping Li     E-mail:  ss_lip@ujn.edu.cn

Cite this article: 

Yong-Chun Zhao(赵永春), Ming-Xin Zhu(朱铭鑫), Sheng-Shi Li(李胜世), and Ping Li(李萍) Room temperature quantum anomalous Hall insulator in honeycomb lattice, RuCS3, with large magnetic anisotropy energy 2023 Chin. Phys. B 32 057301

[1] Müchler L, Yan B, Casper F, Chadov S and Felser C 2013 Springer Ser. Mater. Sci. 182 123
[2] Nagaosa N, Sinova J, Onoda S, MacDonald A H and Ong N P 2010 Rev. Mod. Phys. 82 1539
[3] Qi X L and Zhang S C 2011 Rev. Mod. Phys. 83 1
[4] Weng H, Yu R, Hu X, Dai X and Fang Z 2015 Adv. Phys. 64 227
[5] Zhang S, Genov D A, Wang Y, Liu M and Zhang X 2008 Phys. Rev. Lett. 101 047401
[6] Yu R, Zhang W, Zhang H J, Zhang S C, Dai X and Fang Z 2010 Science 329 61
[7] Qiao Z, Yang S A, Feng W, Tse W K, Ding J, Yao Y, Wang J and Niu Q 2010 Phys. Rev. B 82 161414
[8] Ding J, Qiao Z, Feng W, Yao Y and Niu Q 2011 Phys. Rev. B 84 195444
[9] Ding J, Qiao Z, Feng W, et al. 2011 Phys. Rev. B 84 195444
[10] Qiao Z, Jiang H, Li X, et al. 2012 Phys. Rev. B 85 115439
[11] Ezawa M 2012 Phys. Rev. Lett. 109 055502
[12] Garrity K F and Vanderbilt D 2013 Phys. Rev. Lett. 110 116802
[13] Wang Z F, Liu Z and Liu F 2013 Phys. Rev. Lett. 110 196801
[14] Liu C C, Zhou J J and Yao Y 2015 Phys. Rev. B 91 165430
[15] Li P, Li X, Zhao W, Chen H, Chen M X, Guo Z X, Feng J, Gong X G and Macdonald A H 2017 Nano Lett. 17 6195
[16] Sun Q and Kioussis N 2018 Phys. Rev. B 97 1
[17] Li P 2019 Phys. Chem. Chem. Phys. 21 6712
[18] Wang K, Zhang Y, Zhao W, Li P, Ding J W, Xie G F and Guo Z X 2019 Phys. Chem. Chem. Phys. 21 9310
[19] Chang C Z, Zhang J, Feng X, Shen J, Zhang Z, Guo M, Li K, Ou Y, Wei P, Wang L L, Ji Z Q, Feng Y, Ji S, Chen X, Jia J, Dai X, Fang Z, Zhang S C, He K, Wang Y, Lu L, Ma X C and Xue Q K 2013 Science 340 167
[20] Kresse G and Furthmüller J 1996 Comput. Mater. Sci. 6 15
[21] Kresse G and Hafner J 1993 Phys. Rev. B 47 558
[22] Langreth D C and Mehl M J 1983 Phys. Rev. B 28 1809
[23] Perdew J P, Burke K and Ernzerhof M 1996 Phys. Rev. Lett. 77 3865
[24] Joubert D 1999 Phys. Rev. B 59 1758
[25] Becke A 1988 Phys. Rev. A 38 3098
[26] Heyd J, Scuseria G E and Ernzerhof M 2003 J. Chem. Phys. 118 8207
[27] Togo A, Oba F and Tanaka I 2008 Phys. Rev. B 78 134106
[28] Yao Y and Fang Z 2005 Phys. Rev. Lett. 95 156601
[1] Prediction of LiCrTe2 monolayer as a half-metallic ferromagnet with a high Curie temperature
Li-Man Xiao(肖丽蔓), Huan-Cheng Yang(杨焕成), and Zhong-Yi Lu(卢仲毅). Chin. Phys. B, 2023, 32(5): 057505.
[2] Evaluating thermal expansion in fluorides and oxides: Machine learning predictions with connectivity descriptors
Yilin Zhang(张轶霖), Huimin Mu(穆慧敏), Yuxin Cai(蔡雨欣), Xiaoyu Wang(王啸宇), Kun Zhou(周琨), Fuyu Tian(田伏钰), Yuhao Fu(付钰豪), and Lijun Zhang(张立军). Chin. Phys. B, 2023, 32(5): 056302.
[3] Rational design of Fe/Co-based diatomic catalysts for Li-S batteries by first-principles calculations
Xiaoya Zhang(张晓雅), Yingjie Cheng(程莹洁), Chunyu Zhao(赵春宇), Jingwan Gao(高敬莞), Dongxiao Kan(阚东晓), Yizhan Wang(王义展), Duo Qi(齐舵), and Yingjin Wei(魏英进). Chin. Phys. B, 2023, 32(3): 036803.
[4] Single-layer intrinsic 2H-phase LuX2 (X = Cl, Br, I) with large valley polarization and anomalous valley Hall effect
Chun-Sheng Hu(胡春生), Yun-Jing Wu(仵允京), Yuan-Shuo Liu(刘元硕), Shuai Fu(傅帅),Xiao-Ning Cui(崔晓宁), Yi-Hao Wang(王易昊), and Chang-Wen Zhang(张昌文). Chin. Phys. B, 2023, 32(3): 037306.
[5] Li2NiSe2: A new-type intrinsic two-dimensional ferromagnetic semiconductor above 200 K
Li-Man Xiao(肖丽蔓), Huan-Cheng Yang(杨焕成), and Zhong-Yi Lu(卢仲毅). Chin. Phys. B, 2023, 32(3): 037501.
[6] Prediction of one-dimensional CrN nanostructure as a promising ferromagnetic half-metal
Wenyu Xiang(相文雨), Yaping Wang(王亚萍), Weixiao Ji(纪维霄), Wenjie Hou(侯文杰),Shengshi Li(李胜世), and Peiji Wang(王培吉). Chin. Phys. B, 2023, 32(3): 037103.
[7] First-principles prediction of quantum anomalous Hall effect in two-dimensional Co2Te lattice
Yuan-Shuo Liu(刘元硕), Hao Sun(孙浩), Chun-Sheng Hu(胡春生), Yun-Jing Wu(仵允京), and Chang-Wen Zhang(张昌文). Chin. Phys. B, 2023, 32(2): 027101.
[8] Bandgap evolution of Mg3N2 under pressure: Experimental and theoretical studies
Gang Wu(吴刚), Lu Wang(王璐), Kuo Bao(包括), Xianli Li(李贤丽), Sheng Wang(王升), and Chunhong Xu(徐春红). Chin. Phys. B, 2022, 31(6): 066205.
[9] Evaluation of performance of machine learning methods in mining structure—property data of halide perovskite materials
Ruoting Zhao(赵若廷), Bangyu Xing(邢邦昱), Huimin Mu(穆慧敏), Yuhao Fu(付钰豪), and Lijun Zhang(张立军). Chin. Phys. B, 2022, 31(5): 056302.
[10] Magnetic proximity effect induced spin splitting in two-dimensional antimonene/Fe3GeTe2 van der Waals heterostructures
Xiuya Su(苏秀崖), Helin Qin(秦河林), Zhongbo Yan(严忠波), Dingyong Zhong(钟定永), and Donghui Guo(郭东辉). Chin. Phys. B, 2022, 31(3): 037301.
[11] First-principles study of stability of point defects and their effects on electronic properties of GaAs/AlGaAs superlattice
Shan Feng(冯山), Ming Jiang(姜明), Qi-Hang Qiu(邱启航), Xiang-Hua Peng(彭祥花), Hai-Yan Xiao(肖海燕), Zi-Jiang Liu(刘子江), Xiao-Tao Zu(祖小涛), and Liang Qiao(乔梁). Chin. Phys. B, 2022, 31(3): 036104.
[12] First-principles study of two new boron nitride structures: C12-BN and O16-BN
Hao Wang(王皓), Yaru Yin(殷亚茹), Xiong Yang(杨雄), Yanrui Guo(郭艳蕊), Ying Zhang(张颖), Huiyu Yan(严慧羽), Ying Wang(王莹), and Ping Huai(怀平). Chin. Phys. B, 2022, 31(2): 026102.
[13] High-sensitive terahertz detection by parametric up-conversion using nanosecond pulsed laser
Yuye Wang(王与烨), Gang Nie(聂港), Changhao Hu(胡常灏), Kai Chen(陈锴), Chao Yan(闫超), Bin Wu(吴斌), Junfeng Zhu(朱军峰), Degang Xu(徐德刚), and Jianquan Yao(姚建铨). Chin. Phys. B, 2022, 31(2): 024204.
[14] Manipulation of intrinsic quantum anomalous Hall effect in two-dimensional MoYN2CSCl MXene
Yezhu Lv(吕叶竹), Peiji Wang(王培吉), and Changwen Zhang(张昌文). Chin. Phys. B, 2022, 31(12): 127303.
[15] Extraordinary mechanical performance in charged carbyne
Yong-Zhe Guo(郭雍哲), Yong-Heng Wang(汪永珩), Kai Huang(黄凯), Hao Yin(尹颢), and En-Lai Gao(高恩来). Chin. Phys. B, 2022, 31(12): 128102.
No Suggested Reading articles found!