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Thermally enhanced photoluminescence and temperature sensing properties of Sc2W3O12:Eu3+ phosphors |
| Yu-De Niu(牛毓德), Yu-Zhen Wang(汪玉珍), Kai-Ming Zhu(朱凯明), Wang-Gui Ye(叶王贵), Zhe Feng(冯喆), Hui Liu(柳挥), Xin Yi(易鑫), Yi-Huan Wang(王怡欢), and Xuan-Yi Yuan(袁轩一)† |
| Beijing Key Laboratory of Optoelectronic Functional Materials&Micro-nano Devices, Department of Physics, Renmin University of China, Beijing 100872, China |
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Abstract Recently, lanthanide-ion-doped luminescent materials have been extensively used as optical thermometry probes due to their fast responses, non-contact, and high sensitivity properties. Based on different responses of two emissions to temperature, the fluorescence intensity ratio (FIR) technique can be used to estimate the sensitivities for assessing the optical thermometry performances. In this study, we introduce different doping concentrations of Eu$^{3+}$ ions into negative thermal expansion material Sc$_{2}$W$_{3}$O$_{12}$ to increase the thermal-enhanced luminescence from 373 K to 548 K, and investigate the temperature sensing properties in detail. All samples can exhibit their good luminescence behaviors thermally enhanced. The emission intensity of Sc$_{2}$W$_{3}$O$_{12}$:6-mol% Eu$^{3+}$ phosphor reaches 147.8% of initial intensity at 473 K. As the Eu$^{3+}$ doping concentration increases, the resistance of the sample to thermal quenching decreases. The FIR technique based on each of the transitions $^{5}$D$\to {}^{7}$F$_{1}$ (592 nm) and $^{5}$D$\to ^{7}$F$_{2 }$ (613 nm) of Eu$^{3+}$ ions demonstrates a maximum relative temperature sensitivity of 3.063% K$^{-1}$ at 298 K for Sc$_{2}$W$_{3}$O$_{12}$:6-mol% Eu$^{3+}$ phosphor. The sensitivity of sample decreases with the increase of Eu$^{3+}$ concentration. Benefiting from the thermal-enhanced luminescence performance and good temperature sensing properties, the Sc$_{2}$W$_{3}$O$_{12}$:Eu$^{3+}$ phosphors can be used as optical thermometers.
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Received: 22 March 2022
Revised: 15 May 2022
Accepted manuscript online: 18 May 2022
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PACS:
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87.15.mq
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(Luminescence)
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32.50.+d
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(Fluorescence, phosphorescence (including quenching))
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78.55.-m
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(Photoluminescence, properties and materials)
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| Fund: Project supported by the National Natural Science Foundation of China (Grant No. 51872327). |
Corresponding Authors:
Xuan-Yi Yuan
E-mail: yuanxuanyi@ruc.edu.cn
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Cite this article:
Yu-De Niu(牛毓德), Yu-Zhen Wang(汪玉珍), Kai-Ming Zhu(朱凯明), Wang-Gui Ye(叶王贵), Zhe Feng(冯喆), Hui Liu(柳挥), Xin Yi(易鑫), Yi-Huan Wang(王怡欢), and Xuan-Yi Yuan(袁轩一) Thermally enhanced photoluminescence and temperature sensing properties of Sc2W3O12:Eu3+ phosphors 2023 Chin. Phys. B 32 028703
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