Review of Raman spectroscopy of two-dimensional magnetic van der Waals materials

doi:10.1088/1674-1056/ac1e0f

Abstract Ultrathin van der Waals (vdW) magnets provide a possibility to access magnetic ordering in the two-dimensional (2D) limit, which are expected to be applied in the spintronic devices. Raman spectroscopy is a powerful characterization method to investigate the spin-related properties in 2D vdW magnets, including magnon and spin-lattice interaction, which are hardly accessible by other optical methods. In this paper, the recent progress of various magnetic properties in 2D vdW magnets studied by Raman spectroscopy is reviewed, including the magnetic transition, spin-wave, spin-lattice interaction, symmetry tuning induced by spin ordering, and nonreciprocal magneto-phonon Raman scattering.

Keywords: two-dimensional (2D) magnets Raman spectroscopy magnon spin-lattice interaction

Received: 28 April 2021
Revised: 23 July 2021
Accepted manuscript online: 17 August 2021

PACS:	71.70.Ej	(Spin-orbit coupling, Zeeman and Stark splitting, Jahn-Teller effect)
	33.20.Fb	(Raman and Rayleigh spectra (including optical scattering) ?)
	07.55.Db	(Generation of magnetic fields; magnets)
	72.10.Di	(Scattering by phonons, magnons, and other nonlocalized excitations)

Fund: Project supported by Beijing Natural Science Foundation, China (Grant No. JQ18014), the National Natural Science Foundation of China (Grant No. 12074371), Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB28000000), and CAS Interdisciplinary Innovation Team.

Corresponding Authors: Jun Zhang
E-mail: zhangjwill@semi.ac.cn

Cite this article:

Yu-Jia Sun(孙宇伽), Si-Min Pang(庞思敏), and Jun Zhang(张俊) Review of Raman spectroscopy of two-dimensional magnetic van der Waals materials 2021 Chin. Phys. B 30 117104

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