High-pressure electrides: From design to synthesis

doi:10.1088/1674-1056/ab3f95

Abstract Electrides are unique ionic compounds that electrons serve as the anions. Many electrides with fascinating physical and chemical properties have been discovered at ambient condition. Under pressure, electrides are also revealed to be ubiquitous crystal morphology, enriching the geometrical topologies and electronic properties of electrides. In this Review, we overview the formation mechanism of high-pressure electrides (HPEs) and outline a scheme for exploring new HPEs from pre-design, CALYPSO assisted structural searches, indicators for electrides, to experimental synthesis. Moreover, the evolution of electronic dimensionality under compression is also discussed to better understand the dimensional distribution of anionic electrons in HPEs.

Keywords: electrides high pressure CALYPSO structural search

Received: 12 June 2019
Revised: 06 July 2019
Accepted manuscript online:

PACS:	62.50.-p	(High-pressure effects in solids and liquids)
	61.50.Ks	(Crystallographic aspects of phase transformations; pressure effects)

Corresponding Authors: Huiyang Gou
E-mail: huiyang.gou@hpstar.ac.cn

Cite this article:

Biao Wan(万彪), Jingwu Zhang(张静武), Lailei Wu(吴来磊), Huiyang Gou(缑慧阳) High-pressure electrides: From design to synthesis 2019 Chin. Phys. B 28 106201

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