High-sensitivity spectroscopic measurements under pulsed high magnetic field

doi:10.1088/1674-1056/adce95

Abstract Pulsed magnet technology is the only way to generate ultra-strong magnetic fields higher than 45 T so far. However, the inherently fast-changing field strength (typically on the order of 1000 T/s) poses significant challenges for spectroscopic measurements which rely on time integration of signals to improve spectral qualities. In this work, we report high-sensitivity spectroscopic measurements under pulsed high magnetic fields employing the long flat-top pulsed magnetic field technique. By means of a multiple-capacitor power supply, we were able to generate pulsed high magnetic fields with controllable flat-top pulse width and field stabilities. By synchronizing spectroscopic measurements with the waveform of the flat-top magnetic field, the integration time of each spectrum can be increased by up to 100 times compared with that of the conventional spectroscopic measurements under pulsed magnetic fields, thus enabling high-sensitivity spectroscopic measurements under ultra-strong pulsed magnetic fields. These findings promise an efficient way to significantly improve the performance and extend the application of optical measurements under pulsed high magnetic fields.

Keywords: pulsed magnet flat-top pulsed magnetic field optical spectroscopy photoluminescence

Received: 20 January 2025
Revised: 09 April 2025
Accepted manuscript online: 21 April 2025

PACS:	07.57.Pt	(Submillimeter wave, microwave and radiowave spectrometers; magnetic resonance spectrometers, auxiliary equipment, and techniques)
	07.55.-w	(Magnetic instruments and components)
	07.55.Db	(Generation of magnetic fields; magnets)

Fund: This work was financially supported by the National Key Research and Development Program of China (Grant No. 2022YFA1602700) and the National Natural Science Foundation of China (Grant No. 12274159).

Corresponding Authors: Weihang Zhou
E-mail: zhouweihang@hust.edu.cn

Cite this article:

Zheng Wang(王政), Yichun Pan(潘议淳), Guangran Yang(杨光冉), Wei Xie(谢微), and Weihang Zhou(周伟航) High-sensitivity spectroscopic measurements under pulsed high magnetic field 2025 Chin. Phys. B 34 070701

[1] Miyata A, Mitioglu A, Plochocka P, Portugall O, Wang J T W, Stranks S D, Snaith H J and Nicholas R J 2015 Nat. Phys. 11 582
[2] Goryca M, Li J, Stier A V, Taniguchi T,Watanabe K, Courtade E, Shree S, Robert C, Urbaszek B, Marie X and Crooker S A 2019 Nat. Commun. 10 4172
[3] Timothy Noe Ii G, Kim J H, Lee J, Wang Y, Wójcik A K, McGill S A, Reitze D H, Belyanin A A and Kono J 2012 Nat. Phys. 8 219
[4] Zhang X X, Cao T, Lu Z, Lin Y C, Zhang F, Wang Y, Li Z, Hone J C, Robinson J A, Smirnov D, Louie S G and Heinz T F 2017 Nat. Nanotechnol. 12 883
[5] Feierabend M, Brem S, Ekman A and Malic E 2020 2D Mater. 8 015013
[6] Boekhoven J 2018 Nat. Nanotechnol. 13 979
[7] Chen Z, Zhou W, Zhang B, Yu C H, Zhu J, Lu W and Shen S C 2009 Phys. Rev. Lett. 102 244103
[8] Zhou W, Chen Z, Zhang B, Yu C H, Lu W and Shen S C 2010 Phys. Rev. Lett. 105 024101
[9] Overstreet C, Asenbaum P, Curti J, Kim M and Kasevich M A 2022 Science 375 226
[10] Vaidman L 2012 Phys. Rev. A 86 040101
[11] Caprez A, Barwick B and Batelaan H 2007 Phys. Rev. Lett. 99 210401
[12] Portugall O, Puhlmann N, Müller H U, Barczewski M, Stolpe I and Ortenberg M v 1999 J. Phys. D: Appl. Phys. 32 2354
[13] Li L, Ding H, Peng T, Han X, Xia Z, Chen J, Duan X, Wang C, Pan Y, Vanacken J and Herlach F 2008 IEEE Trans. Appl. Supercond. 18 596
[14] Liu S, Peng T, Liu X, Shang H, Wang S, Pan Z, Jin G, Li J and Li L 2024 IEEE Trans. Appl. Supercond. 34 1
[15] Peng T, Liu S B, Pan Y, Lv Y L, Ding H F, Han X T, Xiao H X, Wang S, Jiang S and Li L 2022 IEEE Trans. Appl. Supercond. 32 1
[16] Li Z Y, Gu T Y, Wei W Q, Yuan Y, Wang Z, Luo K J, Pan Y P, Xie J F, Zhang S Z, Peng T, Liu L, Chen Q, Han X T, Luo Y K and Li L 2025 Chin. Phys. B 34 049901
[17] Xie J F, Zhang S Z, Shi J T, Wang J F, Li L and Han X T 2023 High Voltage. 8 898
[18] Tay F, Baydin A, Katsutani F and Kono J 2022 J. Phys. Soc. Jpn. 91 101006
[19] WeiW, Liu Q, Yuan L, Zhang J, Liu S, Zhou R, Luo Y and Han X 2023 IEEE Trans. Instrum. Meas. 72 1
[20] Xu Y, Gao Z, Yan Z, Chen J and Zhao C 2024 IEEE Trans. Appl. Supercond. 34 1
[21] Wang S, Peng T, Jiang F, Jiang S, Chen S, Deng L, Huang R and Li L 2020 IEEE Trans. Appl. Supercond. 30 1
[22] Xiao H, Ma Y, Lv Y, Ding T, Zhang S, Hu F, Li L and Pan Y 2014 IEEE Trans. Power Electron. 29 4532
[23] Kohama Y and Kindo K 2015 Rev. Sci. Instrum. 86 104701
[24] Geng J, Zhang D, Kim I, Kim H M, Higashitarumizu N, Rahman I K M R, Lam L, Ager J W, Davydov A V, Krylyuk S and Javey A 2024 Adv. Funct. Mater. 35 2413672
[25] Nelson J, Stanev T K, Lebedev D, Lamountain T, Gish J T, Zeng H, Shin H, Heinonen O,Watanabe K, Taniguchi T, Hersam M C and Stern N P 2023 Phys. Rev. B 107 115304
[26] Brotons-Gisbert M, Andres-Penares D, Suh J, Hidalgo F, Abargues R, Rodríguez-Cantó P J, Segura A, Cros A, Tobias G, Canadell E, Ordejón P,Wu J, Martínez-Pastor J P and Sánchez-Royo J F 2016 Nano Lett. 16 3221
[27] Li C, Zhao L, Shang Q, Wang R, Bai P, Zhang J, Gao Y, Cao Q, Wei Z and Zhang Q 2022 ACS Nano 16 1477
[28] Debbichi L, Eriksson O and Lebègue S 2015 J. Phys. Chem. Lett. 6 3098

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