ELECTROMAGNETISM, OPTICS, ACOUSTICS, HEAT TRANSFER, CLASSICAL MECHANICS, AND FLUID DYNAMICS |
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Field-free orientation of diatomic molecule via the linearly polarized resonant pulses |
Li Su-Yu (李苏宇)a b, Guo Fu-Ming (郭福明)a b, Wang Jun (王俊)a b, Yang Yu-Jun (杨玉军)a b, Jin Ming-Xing (金明星)a b |
a Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China; b Jilin Provincial Key Laboratory of Applied Atomic and Molecular Spectroscopy, Jilin University, Changchun 130012, China |
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Abstract We propose a scheme to coherently control the field-free orientation of NO molecule whose rotational temperature is above 0 K. It is found that the maximum molecular orientation is affected by two factors: one is the sum of the population of M=0 rotational states and the other is their distribution, however, their distribution plays a much more significant role in molecular orientation than the sum of their population. By adopting a series of linearly polarized pulses resonant with the rotational states, the distribution of M= 0 rotational states is well rearranged. Though the number of pulses used is small, a relatively high orientation degree can be obtained. This scheme provides a promising approach to the achievement of a good orientation effect.
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Received: 27 January 2015
Revised: 04 April 2015
Accepted manuscript online:
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PACS:
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42.50.-p
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(Quantum optics)
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33.80.-b
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(Photon interactions with molecules)
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32.80.Qk
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(Coherent control of atomic interactions with photons)
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Fund: Project supported by the National Basic Research Program of China (Grant No. 2013CB922200), the National Natural Science Foundation of China (Grant Nos. 11034003, 11474129, 11274141, and 11304116), the Research Fund for the Doctoral Program of Higher Education of China (Grant No. 20130061110021), and the Graduate Innovation Fund of Jilin University (Grant No. 2015091). |
Corresponding Authors:
Jin Ming-Xing
E-mail: mxjin@jlu.edu.cn
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Cite this article:
Li Su-Yu (李苏宇), Guo Fu-Ming (郭福明), Wang Jun (王俊), Yang Yu-Jun (杨玉军), Jin Ming-Xing (金明星) Field-free orientation of diatomic molecule via the linearly polarized resonant pulses 2015 Chin. Phys. B 24 104205
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