Please wait a minute...
Chin. Phys. B, 2025, Vol. 34(7): 077101    DOI: 10.1088/1674-1056/add7ad
Special Issue: SPECIAL TOPIC — Recent progress on kagome metals and superconductors
SPECIAL TOPIC — Recent progress on kagome metals and superconductors Prev   Next  

Observation of a long-range unidirectional charge density wave in kagome superconductor KV3Sb5

Xingwei Shi(石兴伟)1,2,†, Xiao Liu(刘潇)1,2,†, Geng Li(李更)1,2,3,‡, Zhen Zhao(赵振)1,2, Haitao Yang(杨海涛)1,2,3, Xiao Lin(林晓)2,§, and Hong-Jun Gao(高鸿钧)1,2,3
1 School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100190, China;
2 Beijing National Center for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China;
3 Hefei National Laboratory, Hefei 230088, China
Abstract  The interplay between 2$a_{0}\times2a_{0}$ charge density wave (CDW), nematicity and superconductivity in $A$V$_{3}$Sb$_{5}$ ($A = {\rm K}$, Rb, Cs) compounds gives rise to a rich landscape of intriguing physical phenomena. In addition to the 2$a_{0}\times2a_{0}$ CDW, a unidirectional 4$a_{0}$ stripe CDW is also observed on the Sb surface of RbV$_{3}$Sb$_{5}$ and CsV$_{3}$Sb$_{5}$. However, reports of stripe-like CDWs in KV$_{3}$Sb$_{5}$ have been limited. Here, we report the first observation of a long-range unidirectional stripe order with a $6a_{0}$ modulation period on the Sb surface of KV$_{3}$Sb$_{5}$, coexisting with the $2a_{0} \times 2a_{0}$ CDW. Notably, the intensity of the $6a_{0}$ stripes in STM topographies exhibits pronounced contrast reversal between opposite bias voltages. Additionally, the wave vector of the $6a_{0}$ modulation shows no energy-dependent dispersion, confirming its CDW origin. Furthermore, the $6a_{0}$ CDW is robust under a 7 T out-of-plane magnetic field and persists over a temperature range from 215 mK to 720 mK. These results provide compelling evidence for the emergence of a long-range unidirectional CDW in KV$_{3}$Sb$_{5}$.
Keywords:  kagome superconductor      KV$_3$Sb$_5$      charge density wave      unidirectional strain  
Received:  14 April 2025      Revised:  08 May 2025      Accepted manuscript online:  13 May 2025
PACS:  71.45.Lr (Charge-density-wave systems)  
  74.55.+v (Tunneling phenomena: single particle tunneling and STM)  
  74.70.-b (Superconducting materials other than cuprates)  
Fund: Project supported by the National Key Research and Development Project of China (Grant Nos. 2024YFA1207700 and 2022YFA1204100), the National Natural Science Foundation of China (Grant No. 62488201), the CAS Project for Young Scientists in Basic Research (Grant No. YSBR-003), the Youth Innovation Promotion Association (Grant No. 2023005), and the Innovation Program of Quantum Science and Technology (Grant No. 2021ZD0302700).
Corresponding Authors:  Geng Li, Xiao Lin     E-mail:  gengli.iop@iphy.ac.cn;xlin@ucas.ac.cn

Cite this article: 

Xingwei Shi(石兴伟), Xiao Liu(刘潇), Geng Li(李更), Zhen Zhao(赵振), Haitao Yang(杨海涛), Xiao Lin(林晓), and Hong-Jun Gao(高鸿钧) Observation of a long-range unidirectional charge density wave in kagome superconductor KV3Sb5 2025 Chin. Phys. B 34 077101

[1] Kiesel M L and Thomale R 2012 Phys. Rev. B 86 121105
[2] Wang W S, Li Z Z, Xiang Y Y and Wang Q H 2013 Phys. Rev. B 87 115135
[3] Kang M, Fang S, Ye L, Po H C, Denlinger J, Jozwiak C, Bostwick A, Rotenberg E, Kaxiras E, Checkelsky J G and Comin R 2020 Nat. Commun. 11 4004
[4] Riberolles S X M, Slade T J, Han T, Li B, Abernathy D L, Canfield P C, Ueland B G, Orth P P, Ke L and McQueeney R J 2024 Nat. Commun. 15 1592
[5] Liu Z, Li M, Wang Q, Wang G, Wen C, Jiang K, Lu X, Yan S, Huang Y, Shen D, Yin J X, Wang Z, Yin Z, Lei H and Wang S 2020 Nat. Commun. 11 4002
[6] Zhang T, Yilmaz T, Vescovo E, Li H X, Moore R G, Lee H N, Miao H, Murakami S and McGuire M A 2022 npj Comput. Mater. 8 1
[7] Shi M, Yu F, Yang Y, Meng F, Lei B, Luo Y, Sun Z, He J, Wang R, Jiang Z, Liu Z, Shen D, Wu T, Wang Z, Xiang Z, Ying J and Chen X 2022 Nat. Commun. 13 2773
[8] Kiesel M L, Platt C and Thomale R 2013 Phys. Rev. Lett. 110 126405
[9] Nakatsuji S, Kiyohara N and Higo T 2015 Nature 527 212
[10] Liu E, Sun Y, Kumar N, Muechler L, Sun A, Jiao L, Yang S Y, Liu D, Liang A, Xu Q, Kroder J, Süß V, Borrmann H, Shekhar C, Wang Z, Xi C, Wang W, Schnelle W, Wirth S, Chen Y, Goennenwein S T B and Felser C 2018 Nat. Phys. 14 1125
[11] Ye L, Kang M, Liu J, von Cube F, Wicker C R, Suzuki T, Jozwiak C, Bostwick A, Rotenberg E, Bell D C, Fu L, Comin R and Checkelsky J G 2018 Nature 555 638
[12] Wu L, Hu Y, Fan D, Wang D and Wan X 2023 Chin. Phys. Lett. 40 117103
[13] Teng X, Oh J S, Tan H, Chen L, Huang J, Gao B, Yin J X, Chu J H, Hashimoto M, Lu D, Jozwiak C, Bostwick A, Rotenberg E, Granroth G E, Yan B, Birgeneau R J, Dai P and Yi M 2023 Nat. Phys. 19 814
[14] Ortiz B R, Gomes L C, Morey J R,Winiarski M, Bordelon M, Mangum J S, Oswald I W H, Rodriguez-Rivera J A, Neilson J R, Wilson S D, Ertekin E, McQueen T M and Toberer E S 2019 Phys. Rev. Mater. 3 094407
[15] Ortiz B R, Teicher S M L, Hu Y, Zuo J L, Sarte P M, Schueller E C, Abeykoon A M M, Krogstad M J, Rosenkranz S, Osborn R, Seshadri R, Balents L, He J and Wilson S D 2020 Phys. Rev. Lett. 125 247002
[16] Jiang Y X, Yin J X, Denner M M, Shumiya N, Ortiz B R, Xu G, Guguchia Z, He J, Hossain M S, Liu X, Ruff J, Kautzsch L, Zhang S S, Chang G, Belopolski I, Zhang Q, Cochran T A, Multer D, Litskevich M, Cheng Z J, Yang X P, Wang Z, Thomale R, Neupert T, Wilson S D and Hasan M Z 2021 Nat. Mater. 20 1353
[17] Shumiya N, Hossain Md S, Yin J X, Jiang Y X, Ortiz B R, Liu H, Shi Y, Yin Q, Lei H, Zhang S S, Chang G, Zhang Q, Cochran T A, Multer D, Litskevich M, Cheng Z J, Yang X P, Guguchia Z, Wilson S D and Hasan M Z 2021 Phys. Rev. B 104 35131
[18] Luo J, Zhao Z, Zhou Y Z, Yang J, Fang A F, Yang H T, Gao H J, Zhou R and Zheng G Q 2022 npj Quantum Mater. 7 1
[19] Li H, Zhang T T, Yilmaz T, Pai Y Y, Marvinney C E, Said A, Yin Q W, Gong C S, Tu Z J, Vescovo E, Nelson C S, Moore R G, Murakami S, Lei H C, Lee H N, Lawrie B J and Miao H 2021 Phys. Rev. X 11 031050
[20] Li H, Zhao H, Ortiz B R, Park T, Ye M, Balents L, Wang Z, Wilson S D and Zeljkovic I 2022 Nat. Phys. 18 265
[21] Li H, Fabbris G, Said A H, Sun J P, Jiang Y X, Yin J X, Pai Y Y, Yoon S, Lupini A R, Nelson C S, Yin Q W, Gong C S, Tu Z J, Lei H C, Cheng J G, Hasan M Z, Wang Z, Yan B, Thomale R, Lee H N and Miao H 2022 Nat. Commun. 13 6348
[22] Zhao H, Li H, Ortiz B R, Teicher SML, Park T, Ye M,Wang Z, Balents L, Wilson S D and Zeljkovic I 2021 Nature 599 216
[23] Hu B, Ye Y, Huang Z, Han X, Zhao Z, Yang H, Chen H and Gao H J 2022 Chin. Phys. B 31 058102
[24] Wang Z, Jiang Y X, Yin J X, Li Y, Wang G Y, Huang H L, Shao S, Liu J, Zhu P, Shumiya N, Hossain M S, Liu H, Shi Y, Duan J, Li X, Chang G, Dai P, Ye Z, Xu G, Wang Y, Zheng H, Jia J, Hasan M Z and Yao Y 2021 Phys. Rev. B 104 75148
[25] Wu P, Tu Y,Wang Z, Yu S, Li H, MaW, Liang Z, Zhang Y, Zhang X, Li Z, Yang Y, Qiao Z, Ying J, Wu T, Shan L, Xiang Z, Wang Z and Chen X 2023 Nat. Phys. 19 1143
[26] Nie L, Sun K, Ma W, Song D, Zheng L, Liang Z, Wu P, Yu F, Li J, Shan M, Zhao D, Li S, Kang B, Wu Z, Zhou Y, Liu K, Xiang Z, Ying J, Wang Z, Wu T and Chen X 2022 Nature 604 59
[27] Xu Y, Ni Z, Liu Y, Ortiz B R, Deng Q, Wilson S D, Yan B, Balents L and Wu L 2022 Nat. Phys. 18 1470
[28] Fukushima K, Obata K, Yamane S, Hu Y, Li Y, Yao Y,Wang Z, Maeno Y and Yonezawa S 2024 Nat. Commun. 15 2888
[29] Chen H, Yang H, Hu B, Zhao Z, Yuan J, Xing Y, Qian G, Huang Z, Li G, Ye Y, Ma S, Ni S, Zhang H, Yin Q, Gong C, Tu Z, Lei H, Tan H, Zhou S, Shen C, Dong X, Yan B, Wang Z and Gao H J 2021 Nature 599 222
[30] Deng H, Qin H, Liu G, Yang T, Fu R, Zhang Z, Wu X, Wang Z, Shi Y, Liu J, Liu H, Yan X Y, Song W, Xu X, Zhao Y, Yi M, Xu G, Hohmann H, Holbæk S C, Dürrnagel M, Zhou S, Chang G, Yao Y, Wang Q, Guguchia Z, Neupert T, Thomale R, Fischer M H and Yin J X 2024 Nature 632 775
[31] Yan X Y, Deng H, Yang T, Liu G, SongW, Miao H, Tu Z, Lei H,Wang S, Lin B C, Qin H and Yin J X 2024 Chin. Phys. Lett. 41 97401
[32] Li H, Oh D, Kang M, Zhao H, Ortiz B R, Oey Y, Fang S, Ren Z, Jozwiak C, Bostwick A, Rotenberg E, Checkelsky J G,Wang Z,Wilson S D, Comin R and Zeljkovic I 2023 Phys. Rev. X 13 031030
[33] Li H, Zhao H, Ortiz B R, Oey Y, Wang Z, Wilson S D and Zeljkovic I 2023 Nat. Phys. 19 637
[34] Xiao Q, Lin Y, Li Q, Zheng X, Francoual S, Plueckthun C, Xia W, Qiu Q, Zhang S, Guo Y, Feng J and Peng Y 2023 Phys. Rev. Res. 5 L012032
[35] Arguello C J, Chockalingam S P, Rosenthal E P, Zhao L, Gutiérrez C, Kang J H, Chung W C, Fernandes R M, Jia S, Millis A J, Cava R J and Pasupathy A N 2014 Phys. Rev. B 89 235115
[36] Fang A, Ru N, Fisher I R and Kapitulnik A 2007 Phys. Rev. Lett. 99 46401
[37] Tan H, Liu Y, Wang Z and Yan B 2021 Phys. Rev. Lett. 127 46401
[38] Zheng L, Wu Z, Yang Y, Nie L, Shan M, Sun K, Song D, Yu F, Li J, Zhao D, Li S, Kang B, Zhou Y, Liu K, Xiang Z, Ying J, Wang Z, Wu T and Chen X 2022 Nature 611 682
[39] Soumyanarayanan A, Yee M M, He Y, van Wezel J, Rahn D J, Rossnagel K, Hudson EW, Norman M R and Hoffman J E 2013 Proc. Natl. Acad. Sci. USA 110 1623
[40] Gao S, Flicker F, Sankar R, Zhao H, Ren Z, Rachmilowitz B, Balachandar S, Chou F, Burch K S, Wang Z, van Wezel J and Zeljkovic I 2018 Proc. Natl. Acad. Sci. USA 115 6986
[1] Momentum-dependent anisotropy of the charge density wave gap in quasi-1D ZrTe3-xSex (x = 0.015)
Renjie Zhang(张任杰), Yudong Hu(胡裕栋), Yiwei Cheng(程以伟), Yigui Zhong(钟益桂), Xuezhi Chen(陈学智), Junqin Li(李俊琴), Kozo Okazaki, Yaobo Huang(黄耀波), Tian Shang(商恬), Shifeng Jin(金士锋), Baiqing Lv(吕佰晴), and Hong Ding(丁洪). Chin. Phys. B, 2025, 34(7): 077106.
[2] Nontrivial Fermi surface topology in kagome superconductor CsTi3Bi5 revealed by de Haas-van Alphen oscillation
Yuhang Zhang(张宇航), Xinwei Yi(易鑫伟), Zhen Zhao(赵振), Jiali Liu(刘家利), Aini Xu(胥艾妮), Dong Li(李栋), Zouyouwei Lu(鲁邹有为), Yue Liu(刘樾), Jihu Lu(卢佶虎), Hua Zhang(张华), Hui Chen(陈辉), Shiliang Li(李世亮), Ziyi Liu(刘子儀), Jinguang Cheng(程金光), Gang Su(苏刚), Haitao Yang(杨海涛), Xiaoli Dong(董晓莉), Hong-Jun Gao(高鸿钧), and Zhongxian Zhao(赵忠贤). Chin. Phys. B, 2025, 34(7): 077107.
[3] In-plane negative magnetoresistance and quantum oscillations in van der Waals antiferromagnet DyTe3
Qi Qi(齐琦), Senhao Lv(吕森浩), Ke Zhu(祝轲), Yaofeng Xie(谢耀锋), Guojing Hu(胡国静), Zhen Zhao(赵振), Guoyu Xian(冼国裕), Yechao Han(韩烨超), Yang Yang(杨洋), Lihong Bao(鲍丽宏), Xiao Lin(林晓), Hui Guo(郭辉), Haitao Yang(杨海涛), and Hong-Jun Gao(高鸿钧). Chin. Phys. B, 2025, 34(7): 077305.
[4] Scanning tunneling microscopy study on symmetry breaking of charge density wave in FeGe
Jiakang Zhang(张嘉康), Ziyuan Chen(陈子元), Xueliang Wu(吴学良), Mingzhe Li(李明哲), Yuanji Li(李元骥), Ruotong Yin(尹若彤), Jiashuo Gong(巩佳硕), Shiyuan Wang(王适源), Aifeng Wang(王爱峰), Dong-Lai Feng(封东来), and Ya-Jun Yan(闫亚军). Chin. Phys. B, 2025, 34(4): 047303.
[5] Two-fold symmetry of the in-plane resistance in kagome superconductor Cs(V1-xTax)3Sb5 with enhanced superconductivity
Zhen Zhao(赵振), Ruwen Wang(王汝文), Yuhang Zhang(张宇航), Ke Zhu(祝轲), Weiqi Yu(余维琪), Yechao Han(韩烨超), Jiali Liu(刘家利), Guojing Hu(胡国静), Hui Guo(郭辉), Xiao Lin(林晓), Xiaoli Dong(董晓莉), Hui Chen(陈辉), Haitao Yang(杨海涛), and Hong-Jun Gao(高鸿钧). Chin. Phys. B, 2024, 33(7): 077406.
[6] Magnetoresistance hysteresis in the superconducting state of kagome CsV3Sb5
Tian Le(乐天), Jinjin Liu(刘锦锦), Zhiwei Wang(王秩伟), and Xiao Lin(林效). Chin. Phys. B, 2024, 33(10): 107402.
[7] Surface-sensitive electronic structure of kagome superconductor CsV3Sb5
Zhisheng Zhao(赵志生), Jianghao Yao(姚江浩), Rui Xu(徐瑞), Yuzhe Wang(王禹喆), Sen Liao(廖森), Zhengtai Liu(刘正太), Dawei Shen (沈大伟), Shengtao Cui(崔胜涛), Zhe Sun(孙喆), Yilin Wang(王义林), Donglai Feng(封东来), and Juan Jiang(姜娟). Chin. Phys. B, 2024, 33(10): 107403.
[8] Manipulating charge density wave state in kagome compound RbV3Sb5
Yu-Xin Meng(孟雨欣), Cheng-Long Xue(薛成龙), Li-Guo Dou(窦立国), Wei-Min Zhao(赵伟民), Qi-Wei Wang(汪琪玮), Yong-Jie Xu(徐永杰), Xiangqi Liu(刘祥麒), Wei Xia(夏威), Yanfeng Guo(郭艳峰), and Shao-Chun Li(李绍春). Chin. Phys. B, 2023, 32(9): 096801.
[9] Electronic states of domain walls in commensurate charge density wave ground state and mosaic phase in 1T-TaS2
Yan Li(李彦), Yao Xiao(肖遥), Qi Zheng(郑琦), Xiao Lin(林晓), Li Huang(黄立), and Hong-Jun Gao(高鸿钧). Chin. Phys. B, 2023, 32(7): 077101.
[10] Flat band in hole-doped transition metal dichalcogenide observed by angle-resolved photoemission spectroscopy
Zilu Wang(王子禄), Haoyu Dong(董皓宇), Weichang Zhou(周伟昌), Zhihai Cheng(程志海), and Shancai Wang(王善才). Chin. Phys. B, 2023, 32(6): 067103.
[11] Anisotropy of 2H-NbSe2 in the superconducting and charge density wave states
Chi Zhang(张驰), Shan Qiao(乔山), Hong Xiao(肖宏), and Tao Hu(胡涛). Chin. Phys. B, 2023, 32(4): 047201.
[12] Superconductivity and unconventional density waves in vanadium-based kagome materials AV3Sb5
Hui Chen(陈辉), Bin Hu(胡彬), Yuhan Ye(耶郁晗), Haitao Yang(杨海涛), and Hong-Jun Gao(高鸿钧). Chin. Phys. B, 2022, 31(9): 097405.
[13] Charge density wave states in phase-engineered monolayer VTe2
Zhi-Li Zhu(朱知力), Zhong-Liu Liu(刘中流), Xu Wu(武旭), Xuan-Yi Li(李轩熠), Jin-An Shi(时金安), Chen Liu(刘晨), Guo-Jian Qian(钱国健), Qi Zheng(郑琦), Li Huang(黄立), Xiao Lin(林晓), Jia-Ou Wang(王嘉欧), Hui Chen(陈辉), Wu Zhou(周武), Jia-Tao Sun(孙家涛), Ye-Liang Wang(王业亮), and Hong-Jun Gao(高鸿钧). Chin. Phys. B, 2022, 31(7): 077101.
[14] Effect of strain on charge density wave order in α-U
Liuhua Xie(谢刘桦), Hongkuan Yuan(袁宏宽), and Ruizhi Qiu(邱睿智). Chin. Phys. B, 2022, 31(6): 067103.
[15] Surface-induced orbital-selective band reconstruction in kagome superconductor CsV3Sb5
Linwei Huai(淮琳崴), Yang Luo(罗洋), Samuel M. L. Teicher, Brenden R. Ortiz, Kaize Wang(王铠泽),Shuting Peng(彭舒婷), Zhiyuan Wei(魏志远), Jianchang Shen(沈建昌), Bingqian Wang(王冰倩), Yu Miao(缪宇),Xiupeng Sun(孙秀鹏), Zhipeng Ou(欧志鹏), Stephen D. Wilson, and Junfeng He(何俊峰). Chin. Phys. B, 2022, 31(5): 057403.
No Suggested Reading articles found!