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Special Issue:
SPECIAL TOPIC — States and new effects in nonequilibrium
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| TOPICAL REVIEW—States and new effects in nonequilibrium |
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Photophysics of metal-organic frameworks: A brief overview |
| Qingshuo Liu(刘晴硕)1, Junhong Yu(余俊宏)2,†, and Jianbo Hu(胡建波)1,2,‡ |
1 State Key Laboratory for Environment-Friendly Energy Materials, Southwest University of Science and Technology, Mianyang 621010, China;
2 Laboratory for Shock Wave and Detonation Physics, Institute of Fluid Physics, China Academy of Engineering Physics, Mianyang 621900, China |
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Abstract Metal-organic frameworks (MOFs), which are self-assembled porous coordination materials, have garnered considerable attention in the fields of optoelectronics, photovoltaic, photochemistry, and photocatalysis due to their diverse structures and excellent tunability. However, the performance of MOF-based optoelectronic applications currently falls short of the industry benchmark. To enhance the performance of MOF materials, it is imperative to undertake comprehensive investigations aimed at gaining a deeper understanding of photophysics and sequentially optimizing properties related to photocarrier transport, recombination, interaction, and transfer. By utilizing femtosecond laser pulses to excite MOFs, time-resolved optical spectroscopy offers a means to observe and characterize these ultrafast microscopic processes. This approach adds the time coordinate as a novel dimension for comprehending the interaction between light and MOFs. Accordingly, this review provides a comprehensive overview of the recent advancements in the photophysics of MOFs and additionally outlines potential avenues for exploring the time domain in the investigation of MOFs.
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Received: 16 August 2023
Revised: 26 September 2023
Accepted manuscript online: 28 September 2023
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PACS:
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72.20.Jv
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(Charge carriers: generation, recombination, lifetime, and trapping)
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71.35.-y
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(Excitons and related phenomena)
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71.20.Nr
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(Semiconductor compounds)
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| Fund: Project supported by the Science Challenge Project (Grant No. TZ2018001), the National Natural Science Foundation of China (Grant Nos. 11872058 and 21802036), the Project of State Key Laboratory of Environment-friendly Energy Materials, and Southwest University of Science and Technology (Grant No. 21fksy07). |
Corresponding Authors:
Junhong Yu, Jianbo Hu
E-mail: yujunhong@caep.cn;jianbo.hu@caep.cn
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Cite this article:
Qingshuo Liu(刘晴硕), Junhong Yu(余俊宏), and Jianbo Hu(胡建波) Photophysics of metal-organic frameworks: A brief overview 2024 Chin. Phys. B 33 017204
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