Attosecond spectroscopy for filming the ultrafast movies of atoms, molecules and solids

doi:10.1088/1674-1056/aca6d2

Abstract Three decades ago, a highly nonlinear nonpertubative phenomenon, now well-known as the high harmonic generation (HHG), was discovered when intense laser irradiates gaseous atoms. As the HHG produces broadband coherent radiation, it becomes the most promising source to obtain attosecond pulses. The door to the attosecond science was opened ever since. In this review, we will revisit the incredible adventure to the attoworld. Firstly, the progress of attosecond pulse generation is outlined. Then, we introduce the efforts on imaging the structures or filming the ultrafast dynamics of nuclei and electrons with unprecedented attosecond temporal and Angstrom spatial resolutions, utilizing the obtained attosecond pulses as well as the high harmonic spectrum itself.

Keywords: strong-field physics attosecond science high harmonic generation ultrafast spectroscopy

Received: 24 July 2022
Revised: 22 November 2022
Accepted manuscript online: 29 November 2022

PACS:	33.20.Xx	(Spectra induced by strong-field or attosecond laser irradiation)
	31.15.at	(Molecule transport characteristics; molecular dynamics; electronic structure of polymers)
	42.65.Ky	(Frequency conversion; harmonic generation, including higher-order harmonic generation)

Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 12021004 and 91950202).

Corresponding Authors: Wei Cao, Pengfei Lan, Peixiang Lu
E-mail: weicao@hust.edu.cn;pengfeilan@hust.edu.cn;lupeixiang@hust.edu.cn

Cite this article:

Lixin He(何立新), Xiaosong Zhu(祝晓松), Wei Cao(曹伟), Pengfei Lan(兰鹏飞), and Peixiang Lu(陆培祥) Attosecond spectroscopy for filming the ultrafast movies of atoms, molecules and solids 2022 Chin. Phys. B 31 123301

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