Crystallization evolution and relaxation behavior of high entropy bulk metallic glasses using microalloying process

doi:10.1088/1674-1056/abd92c

Abstract The role of the microalloying process in relaxation behavior and crystallization evolution of Zr₂₀Cu₂₀Ni₂₀Ti₂₀Hf₂₀ high entropy bulk metallic glass (HEBMG) was investigated. We selected Al and Nb elements as minor elements, which led to the negative and positive effects on the heat of mixing in the master HEBMG composition, respectively. According to the results, both elements intensified β relaxation in the structure; however, α relaxation remained stable. By using different frequencies in dynamic mechanical analysis, it was revealed that the activation energy of β relaxation for the Nb-added sample was much higher, which was due to the creation of significant structural heterogeneity under the microalloying process. Moreover, it was found that Nb addition led to a diversity in crystallization stages at the supercooled liquid region. It was suggested that the severe structural heterogeneity in the Nb-added sample provided multiple energy-level sites in the structure for enhancing the crystallization stages.

Keywords: metallic glasses disordered structures amorphous materials relaxation

Received: 13 September 2020
Revised: 13 December 2020
Accepted manuscript online: 07 January 2021

PACS:

64.70.pe

(Metallic glasses)

Corresponding Authors: Danhong Li, Mahander Pandey
E-mail: lidh@czust.edu.cn;Pandey.mahander1@gmail.com

Cite this article:

Danhong Li(李丹虹), Changyong Jiang(江昌勇), Hui Li(栗慧), and Mahander Pandey Crystallization evolution and relaxation behavior of high entropy bulk metallic glasses using microalloying process 2021 Chin. Phys. B 30 066401

[1] Makarov A S, Goncharova E V, Afonin G V, Qiao J C, Kobelev N P and Khonik V A 2020 JETP Lett. 111 586
[2] Kim J, Oh H S, Kim J, Ryu C W, Lee G W, Chang H J and Park E S 2018 Acta Mater. 155 350
[3] Gong P, Wang S, Li F and Wang X 2018 Metall. Mater. Trans. A 49 2918
[4] Yang K, Fan X, Li B, Li Y, Wang X and Xu X 2018 J. Therm. Anal. Calorim. 132 979
[5] Xing Q W and Zhang Y 2017 Chin. Phys. B 26 18104
[6] Cao D, Wu Y, Li H X, Liu X J, Wang H, Wang X Z and Lu Z P 2018 Intermetallics 99 44
[7] Du Y, Zhou Q, Ren Y, Kuang W, Han W, Zhang S, Zhai H and Wang H 2018 J. Alloys Compd. 762 422
[8] Zhao S, Wang P, Cheng X, Zhang Y, Wen Z, Zhang Q, Yao K F, Chen N and Wang W H 2019 Sci. China Mater. 62 907
[9] Tong Y, Qiao J C, Zhang C, Pelletier J M and Yao Y 2016 J. Non. Cryst. Solids 452 57
[10] Cao J W, Han J G, Guo Z H, Zhao W B, Guo Y Q, Xia Z H and Qiao J W 2016 Mater. Sci. Eng. A 673 141
[11] Zhou Q, Du Y, Han W, Ren Y, Zhai H and Wang H 2019 Scr. Mater. 164 121
[12] Wang X, Gong P, Deng L, Jin J, Wang S and Zhou P 2017 J. Non. Cryst. Solids 470 27
[13] Fang Q, Yi M, Li J, Liu B and Huang Z 2018 Appl. Surf. Sci. 443 122
[14] Wu K, Liu C, Li Q, Huo J, Li M, Chang C and Sun Y 2019 J. Magn. Magn. Mater. 489 165404
[15] Li C, Li Q, Li M, Chang C, Li H, Dong Y and Sun Y 2019 J. Alloys Compd. 791 947
[16] Duan Y J, Qiao J C, Crespo D, Goncharova E V, Makarov A S, Afonin G V and Khonik V A 2020 J. Alloys Compd. 830 154564
[17] Gu J L, Luan H W, Zhao S F, Bu H T, Si J J, Shao Y and Yao K F 2020 Mater. Sci. Eng. A 786 139417
[18] Yin H, Huang Y, Daisenberg D, Xue P, Jiang S, Ru W, Jiang S, Bao Y, Bian X, Tong X, Shen H and Sun J 2019 Scr. Mater. 163 29
[19] Wada T, Jiang J, Yubuta K, Kato H and Takeuchi A 2019 Materialia 7 100372
[20] Tong Y, Qiao J C, Pelletier J M and Yao Y 2020 J. Alloys Compd. 820 153119
[21] Jin J, Li F, Yin G, Wang X and Gong P 2020 Thermochim. Acta 690 178650
[22] Bizhanova G, Li F, Ma Y, Gong P and Wang X 2019 J. Alloys Compd. 779 474
[23] Wang X, Dai W, Zhang M, Gong P and Li N 2018 J. Mater. Sci. Technol. 34 2006
[24] Chen C, Wong K, Krishnan R P, Zhifeng L, Yu D, Lu Z and Chathoth S M 2019 J. Mater. Sci. Technol. 35 44
[25] Tong Y, Qiao J C, Pelletier J M and Yao Y 2020 Intermetallics 119 106726
[26] Chen F C, Dai F P, Yang X Y, Ruan Y and Wei B B 2020 Chin. Phys. B 29 066401
[27] Zong H T, Ma M Z, Zhang X Y, Qi L, Li G, Jing Q and Liu R P 2011 Chin. Phys. Lett. 28 36103
[28] Samavatian M, Gholamipour R and Samavatian V 2021 Comput. Mater. Sci. 186 110025
[29] Wu S Y, Wei S H, Guo G Q, Wang J G and Yang L 2016 Sci. Rep. 6 38098
[30] Samavatian M, Gholamipour R, Samavatian V and Farahani F 2019 Mater. Res. Express 6 065202
[31] Li M, Guan H, Yang S, Ma X and Li Q 2020 Mater. Sci. Eng. A 140542
[32] Jiang W and Zhang B 2020 J. Appl. Phys. 127 115104
[33] Zhu F, Nguyen H K, Song S X, Aji D P B, Hirata A, Wang H, Nakajima K and Chen M W 2016 Nat. Commun. 7 11516
[34] Liu Y H, Fujita T, Aji D P B, Matsuura M and Chen M W 2014 Nat. Commun. 5 3238
[35] Qiao J C, Wang Q, Crespo D, Yang Y and Pelletier J M 2017 Chin. Phys. B 26 16402
[36] Hubek R, Seleznev M, Binkowski I, Peterlechner M, Divinski S V and Wilde G 2018 J. Appl. Phys. 124 225103
[37] Zhai H, Wang H and Liu F 2017 Trans. Nonferrous Met. Soc. China 27 363
[38] Zhu J, Yang M, Wang C, Yang S, Han J, Xie G and Liu X 2019 J. Alloys Compd. 781 8
[39] Qiao J C, Wang Q, Pelletier J M, Kato H, Casalini R, Crespo D, Pineda E, Yao Y and Yang Y 2019 Prog. Mater. Sci. 104 250
[40] Liu M, Qiao J, Hao Q, Chen Y, Yao Y, Crespo D and Pelletier J M 2019 Metals 9 1013
[41] Hao Q, Jia W Y and Qiao J C 2020 J. Non. Cryst. Solids 546 120266

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Crystallization evolution and relaxation behavior of high entropy bulk metallic glasses using microalloying process

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