|
|
Origin of itinerant ferromagnetism in two-dimensional Fe3GeTe2 |
Xi Chen(陈熙), Zheng-Zhe Lin(林正喆)†, and Li-Rong Cheng(程丽蓉) |
1 School of Physics and Optoelectronic Engineering, Xidian University, Xi'an 710071, China |
|
|
Abstract Magnetic order in two-dimensional systems was not supposed to exist at finite temperature. In recent years, the successful preparation of two-dimensional ferromagnetic materials such as CrI3, Cr2Ge2Te6, and Fe3GeTe2 opens up a new chapter in the remarkable field of two-dimensional materials. Here, we report on a theoretical analysis of the stability of ferromagnetism in Fe3GeTe2. We uncover the mechanism of holding long-range magnetic order and propose a model to estimate the Curie temperature of Fe3GeTe2. Our results reveal the essential role of magnetic anisotropy in maintaining the magnetic order of two-dimensional systems. The theoretical method used here can be generalized to future research of other magnetic two-dimensional systems.
|
Received: 21 September 2020
Revised: 30 November 2020
Accepted manuscript online: 08 December 2020
|
PACS:
|
75.70.Ak
|
(Magnetic properties of monolayers and thin films)
|
|
75.10.Jm
|
(Quantized spin models, including quantum spin frustration)
|
|
Fund: Project supported by the Fundamental Research Funds for the Central Universities, China (Grant No. XJS200503) and the Post-Doctoral Research Project of Shaanxi Province, China. |
Corresponding Authors:
†Corresponding author. E-mail: zzlin@xidian.edu.cn
|
Cite this article:
Xi Chen(陈熙), Zheng-Zhe Lin(林正喆), and Li-Rong Cheng(程丽蓉) Origin of itinerant ferromagnetism in two-dimensional Fe3GeTe2 2021 Chin. Phys. B 30 047502
|
1 Huang B, Clark G, Navarro-Moratalla E, Klein D R, Cheng R, Seyler K L, Zhong D, Schmidgall E, McGuire M A, Cobden D H, Yao W, Xiao D, Jarillo-Herrero P and Xu X D 2017 Nature 546 270 2 Pan L, Wen H, Huang L, Chen L, Deng H X, Xia J B and Wei Z 2019 Chin. Phys. B 28 107504 3 Zhao L S, Chen C P, Liu L L, Yu H X, Chen Y and Wang X C 2018 Chin. Phys. B 27 016301 4 Kang K, Lee K H, Han Y, Gao H, Xie S, Muller D A and Park J 2017 Nature 550 229 5 Li M Y, Shi Y, Cheng C C, Lu L S, Lin Y C, Tang H L, Tsai M L, Chu C W, Wei K H, He J H, Chang W H, Suenaga K and Li L J 2015 Science 349 524 6 Ribeiro-Palau R, Zhang C, Watanabe K, Taniguchi T, Hone J and Dean C R 2018 Science 361 690 7 Xu W, Liu W, Schmidt J F, Zhao W, Lu X, Raab T, Diederichs C, Gao W, Seletskiy D V and Xiong Q 2017 Nature 541 62 8 Yu Z, Ong Z Y, Li S, Xu J B, Zhang G, Zhang Y W, Shi Y and Wang X 2017 Adv. Func. Mat. 27 1604093 9 Yuan J H, Chen N, Mo H, Zhang Y and Zhang Z H 2016 Chin. Phys. Lett. 33 037302 10 Mermin N D and Wagner H 1966 Phys. Rev. Lett. 17 1133 11 Jiang P, Wang C, Chen D, Zhong Z, Yuan Z, Lu Z Y and Ji W 2019 Phys. Rev. B 99 144401 12 Kim H H, Yang B, Patel T, Sfigakis F, Li C, Tian S, Lei H and Tsen A W 2018 Nano Lett. 18 4885 13 Song T, Cai X, Tu M W Y, Zhang X, Huang B, Wilson N P, Seyler K L, Zhu L, Taniguchi T, Watanabe K, McGuire M A, Cobden D H, Xiao D, Yao W and Xu X 2018 Science 360 1214 14 Wang Z, Gutierrez-Lezama I, Ubrig N, Kroner M, Gibertini M, Taniguchi T, Watanabe K, Imamoglu A, Giannini E and Morpurgo A F 2018 Nat. Commun. 9 2516 15 Sivadas N, Okamoto S, Xu X, Fennie C J and Xiao D 2018 Nano Lett. 18 7658 16 Gong C, Li L, Li Z, Ji H, Stern A, Xia Y, Cao T, Bao W, Wang C, Wang Y, Qiu Z Q, Cava R J, Louie S G, Xia J and Zhang X 2017 Nature 546 265 17 Zhang J, Cai X, Xia W, Liang A, Huang J, Wang C, Yang L, Yuan H, Chen Y, Zhang S, Guo Y, Liu Z and Li G 2019 Phys. Rev. Lett. 123 047203 18 Deng Y, Yu Y, Song Y, Zhang J, Wang N Z, Sun Z, Yi Y, Wu Y Z, Wu S, Zhu J, Wang J, Chen X H and Zhang Y 2018 Nature 563 94 19 Wang Z, Sapkota D, Taniguchi T, Watanabe K, Mandrus D and Morpurgo A F 2018 Nano Lett. 18 4303 20 Chen B, Yang J, Wang H, Imai M, Ohta H, Michioka C, Yoshimura K and Fang M 2013 J. Phys. Soc. Jpn. 82 124711 21 Deiseroth H J, Aleksandrov K, Reiner C, Kienle L and Kremer R K 2006 Eur. J. Inorg. Chem. 8 1561 22 May A F, Calder S, Cantoni C, Cao H and McGuire M A 2016 Phys. Rev. B 93 014411 23 Tian C K, Wang C, Ji W, Wang J C, Xia T L, Wang L, Liu J J, Zhang H X and Cheng P 2019 Phys. Rev. B 99 184428 24 Fei Z Y, Huang B, Malinowski P, Wang W B, Song T C, Sanchez J, Yao W, Xiao D, Zhu X Y, May A F, Wu W D, Cobden D H, Chu J H and Xu X D 2018 Nat. Mater. 17 778 25 Liu S, Yuan X, Zou Y, Sheng Y, Huang C, Zhang E, Ling J, Liu Y, Wang W, Zhang C, Zou J, Wang K and Xiu F 2017 npj 2D Mat. Appl. 1 30 26 Zheng G, Xie W Q, Albarakati S, Algarni M, Tan C, Wang Y, Peng J, Partridge J, Farrar L, Yi J, Xiong Y, Tian M, Zhao Y J and Wang L 2020 Phys. Rev. Lett. 125 047202 27 Onsager L 1944 Phys. Rev. 65 117 28 Fazekas P1999 Lecture Notes on Electron Correlation and Magnetism (Singapore: World Scientific) 29 Isaacs E B and Marianetti C A 2016 Phys. Rev. B 94 035120 30 Zhuang H L and Hennig R G 2016 Phys. Rev. B 93 054429 31 Holstein T and L P H 1940 Phys. Rev. 58 1098 32 Kresse G and Joubert D 1999 Phys. Rev. B 59 1758 33 Blöchl P E 1994 Phys. Rev. B 50 17953 34 Kresse G and Furthmüller J 1996 Phys. Rev. B 54 11169 35 Kresse G and Furthmüller J 1996 Comp. Mat. Sci. 6 15 36 Kresse G and Hafner J 1993 Phys. Rev. B 47 558 37 Kresse G and Hafner J 1994 Phys. Rev. B 49 14251 38 Perdew J P and Zunger A 1981 Phys. Rev. B 23 5048 39 Grimme S, Antony J, Ehrlich S and Krieg H 2010 J. Chem. Phys. 132 154104 40 Grimme S, Ehrlich S and Goerigk L 2011 J. Comp. Chem. 32 1456 41 Perdew J P, Burke K and Ernzerhof M 1996 Phys. Rev. Lett. 77 3865 42 Heyd J, Scuseria G E and Ernzerhof M 2003 J. Chem. Phys. 118 8207 43 Heyd J, Scuseria G E and Ernzerhof M 2006 J. Chem. Phys. 124 219906 44 Singh D J and Du M-H 2008 Phys. Rev. Lett. 100 237003 45 Xiang H, Lee C, Koo H J, Gong X and Whangbo M H 2013 Dalton Trans. 42 823 46 O'Handley R C1999 Modern Magnetic Materials: Principles and Applications (Wiley-Interscience, 1st ed.). 47 Blundell S2001 Magnetism in Condensed Matter (New York: Oxford University Press) |
No Suggested Reading articles found! |
|
|
Viewed |
|
|
|
Full text
|
|
|
|
|
Abstract
|
|
|
|
|
Cited |
|
|
|
|
Altmetric
|
blogs
Facebook pages
Wikipedia page
Google+ users
|
Online attention
Altmetric calculates a score based on the online attention an article receives. Each coloured thread in the circle represents a different type of online attention. The number in the centre is the Altmetric score. Social media and mainstream news media are the main sources that calculate the score. Reference managers such as Mendeley are also tracked but do not contribute to the score. Older articles often score higher because they have had more time to get noticed. To account for this, Altmetric has included the context data for other articles of a similar age.
View more on Altmetrics
|
|
|