Effects of (LiCe) co-substitution on the structural and electrical properties of CaBi2Nb2O9 ceramics

doi:10.1088/1674-1056/21/3/037701

Abstract The piezoelectric, dielectric, and ferroelectric properties of the (LiCe) co-substituted calcium bismuth niobate (CaBi₂Nb₂O₉, CBNO) are investigated. The piezoelectric properties of CBNO ceramics are significantly enhanced and the dielectric loss tanδ decreased. This makes poling using (LiCe) co-substitution easier. The ceramics (where $\Box$ represents A-site Ca²⁺ vacancies, possess a pure layered structure phase and no other phases can be found. The Ca_0.88(LiCe)_0.04$\Box$_0.04Bi₂Nb₂O₉ ceramics possess optimal piezoelectric properties, with piezoelectric coefficient (d₃₃) and Curie temperature (T_C) found to be 13.3 pC/N and 960 ℃, respectively. The dielectric and piezoelectric properties of the (LiCe) co-substituted CBNO ceramics exhibit very stable temperature behaviours. This demonstrates that the CBNO ceramics are a promising candidate for ultrahigh temperature applications.

Keywords: co-substitution structural properties electrical properties CaBi₂Nb₂O₉

Received: 24 June 2011
Revised: 19 September 2011
Accepted manuscript online:

PACS:	77.65.Bn	(Piezoelectric and electrostrictive constants)
	77.80.B-	(Phase transitions and Curie point)
	77.84.-s	(Dielectric, piezoelectric, ferroelectric, and antiferroelectric materials)

Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 50632030 and 10804130) and the Shaanxi Provincial Natural Science Foundation, China (Grant No. 2011JM6012).

Corresponding Authors: Tian Xiao-Xia,xiaoxiatian@126.com
E-mail: xiaoxiatian@126.com

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Tian Xiao-Xia(田晓霞), Qu Shao-Bo(屈绍波), Du Hong-Liang(杜红亮), Li Ye(李晔), and Xu Zhuo(徐卓) Effects of (LiCe) co-substitution on the structural and electrical properties of CaBi₂Nb₂O₉ ceramics 2012 Chin. Phys. B 21 037701

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Effects of (LiCe) co-substitution on the structural and electrical properties of CaBi2Nb2O9 ceramics

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Effects of (LiCe) co-substitution on the structural and electrical properties of CaBi₂Nb₂O₉ ceramics