| CONDENSED MATTER: STRUCTURAL, MECHANICAL, AND THERMAL PROPERTIES |
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Negative thermal expansion and photoluminescence in solid solution (HfSc)0.83W2.25P0.83O12δ |
| Yuan Liang(梁源)1,2, Yong-Guang Cheng(程永光)2, Xiang-Hong Ge(葛向红)2, Bao-He Yuan(袁保合)2, Juan Guo(郭娟)2, Qian Sun(孙强)2, Er-Jun Liang(梁二军)2 |
1. Department of Applied Physics, Donghua University, Shanghai 201620, China;
2. School of Physical Science & Engineering and Key Laboratory of Materials Physics of Ministry of Education of China, Zhengzhou University, Zhengzhou 450052, China |
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Abstract A solid solution of (HfSc)0.83W2.25P0.83O12-δ is synthesized by the high-temperature, solid-state reaction and fast-quenching method. It is shown that it possesses an orthorhombic structure with space group Pmmm (47) and exhibits negative thermal expansion (NTE) property with low anisotropy in thermal expansion. The coefficients of thermal expansion (CTEs) for a, b, and c axes are -1.41×10-6 K-1, -2.23×10-6 K-1, and -1.87×10-6 K-1, respectively. This gives rise to volume and linear CTEs of -3.10×10-6 K-1 and -1.03×10-6 K-1, respectively. Besides, it exhibits also intense photoluminescence from 360 nm to about 600 nm. The mechanism of NTE and the correlation of the PL with axial thermal expansion property are discussed.
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Received: 18 May 2017
Revised: 29 June 2017
Accepted manuscript online:
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PACS:
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65.40.De
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(Thermal expansion; thermomechanical effects)
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81.05.Je
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(Ceramics and refractories (including borides, carbides, hydrides, nitrides, oxides, and silicides))
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61.50.-f
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(Structure of bulk crystals)
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78.55.-m
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(Photoluminescence, properties and materials)
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| Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 11574276, 51302249, and 11405028) and the Fundamental Research Fund for the Central Universities, China. |
Corresponding Authors:
Yuan Liang
E-mail: yliang@dhu.edu.cn
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Cite this article:
Yuan Liang(梁源), Yong-Guang Cheng(程永光), Xiang-Hong Ge(葛向红), Bao-He Yuan(袁保合), Juan Guo(郭娟), Qian Sun(孙强), Er-Jun Liang(梁二军) Negative thermal expansion and photoluminescence in solid solution (HfSc)0.83W2.25P0.83O12δ 2017 Chin. Phys. B 26 106501
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