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Abstract Rechargeable batteries, such as lithium-ion batteries, play an important role in the emerging sustainable energy landscape. Mechanical degradation and resulting capacity fade in high-capacity electrode materials critically hinder their use in high-performance lithium-ion batteries. This paper presents an overview of recent advances in understanding the electrochemically-induced mechanical behavior of the electrode materials in lithium-ion batteries. Particular emphasis is placed on stress generation and facture in high-capacity anode materials such as silicon. Finally, we identify several important unresolved issues for future research.
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Received: 15 August 2015
Revised: 14 November 2015
Accepted manuscript online:
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PACS:
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46.50.+a
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(Fracture mechanics, fatigue and cracks)
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62.20.-x
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(Mechanical properties of solids)
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82.45.Fk
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(Electrodes)
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| Fund: Project support by the NSF (Grant Nos. CMMI 1100205 and DMR 1410936). |
Corresponding Authors:
Ting Zhu
E-mail: ting.zhu@me.gatech.edu
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Cite this article:
Ting Zhu Mechanics of high-capacity electrodes in lithium-ion batteries 2016 Chin. Phys. B 25 014601
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