| INTERDISCIPLINARY PHYSICS AND RELATED AREAS OF SCIENCE AND TECHNOLOGY |
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Structural behavior and metallization of AsSbS3 at high pressure |
| Tian Qin(覃天)1, Min Wu(武敏)2, Kai Wang(王凯)2, Ye Wu(吴也)1,†, and Haijun Huang(黄海军)1 |
1 School of Science, Wuhan University of Technology, Wuhan 430070, China;
2 Shandong Key Laboratory of Optical Communication Science and Technology, School of Physics Science and Information Technology, Liaocheng University, Liaocheng 252000, China |
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Abstract The group V-VI semiconductor material getchellite (crystalline AsSbS$_{3})$ has garnered extensive attention due to its wonderful electronic and optical properties. The pressure engineering is one of the most effective methods to modulate crystal structure and physical properties of semiconductor materials. In this study, the structural behavior, optical and electrical properties of AsSbS$_{3}$ under high pressure have been investigated systematically by in situ high-pressure experiments for the first time. The monoclinic structure of AsSbS$_{3}$ remains stable up to 47.0 GPa without phase transition. The gradual lattice contraction with increasing pressure results in a continuous narrowing of the bandgap then leads to pressure-induced metallization of AsSbS$_{3}$ at 31.5 GPa. Our research presents a high-pressure strategy for tuning the crystal structure and physical properties of AsSbS$_{3}$ to expand its potential applications in electronic and optoelectronic fields.
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Received: 08 July 2024
Revised: 06 September 2024
Accepted manuscript online: 10 September 2024
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PACS:
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81.40.Vw
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(Pressure treatment)
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61.50.Ks
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(Crystallographic aspects of phase transformations; pressure effects)
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71.20.Mq
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(Elemental semiconductors)
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72.80.Cw
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(Elemental semiconductors)
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| Fund: Project supported by the National Natural Science Foundation of China (Grant No. 42274123) and the Special Construction Project Fund for Shandong Provincial Taishan Scholars. |
Corresponding Authors:
Ye Wu
E-mail: yew@whut.edu.cn
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Cite this article:
Tian Qin(覃天), Min Wu(武敏), Kai Wang(王凯), Ye Wu(吴也), and Haijun Huang(黄海军) Structural behavior and metallization of AsSbS3 at high pressure 2024 Chin. Phys. B 33 118101
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