| SPECIAL TOPIC — Structures and properties of materials under high pressure |
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Pressure-induced superconductivity and phase transition in PbSe and PbTe |
| Yuyang Jiang(江宇阳)1,†, Cuiying Pei(裴翠颖)1,†, Qi Wang(王琦)1,2, Juefei Wu(吴珏霏)1, Lili Zhang(张丽丽)3, Chao Xiong(熊超)1, and Yanpeng Qi(齐彦鹏)1,2,4,‡ |
1 School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China;
2 ShanghaiTech Laboratory for Topological Physics, ShanghaiTech University, Shanghai 201210, China;
3 Shanghai Synchrotron Radiation Facility, Shanghai Advanced Research Institute, Chinese Academy of Sciences, Shanghai 201203, China;
4 Shanghai Key Laboratory of High-resolution Electron Microscopy, ShanghaiTech University, Shanghai 201210, China |
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Abstract The IV-VI semiconducting chalcogenides are a large material family with distinct physical behavior. Here, we systematically investigate the effect of pressure on the electronic and crystal structures of PbSe and PbTe by combining high-pressure electrical transport and synchrotron x-ray diffraction (XRD) measurements. The resistivity of PbSe and PbTe changes dramatically under high pressure and a non-monotonic evolution of $\rho (T)$ is observed. Both PbSe and PbTe are found to undergo semiconductor-metal transition upon compression and show superconductivity under higher pressure. The structural evolutions from the Fm$\bar{3}m$ to Pnma phase and then to the Pm$\bar{3}m$ phase in PbSe are verified by the x-ray diffraction. The present findings reveal the internal correlation between the structural evolution and the physical properties in lead chalcogenides.
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Received: 29 September 2024
Revised: 01 November 2024
Accepted manuscript online: 05 November 2024
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PACS:
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61.50.Ks
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(Crystallographic aspects of phase transformations; pressure effects)
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74.70.-b
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(Superconducting materials other than cuprates)
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74.62.Fj
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(Effects of pressure)
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| Fund: Project supported by the National Natural Science Foundation of China (Grant No. 52272265) and the National Key R&D Program of China (Grant No. 2023YFA1607400). The authors thank the support from Analytical Instrumentation Center (# SPSTAIC10112914), SPST, ShanghaiTech University. |
Corresponding Authors:
Yanpeng Qi
E-mail: qiyp@shanghaitech.edu.cn
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Cite this article:
Yuyang Jiang(江宇阳), Cuiying Pei(裴翠颖), Qi Wang(王琦), Juefei Wu(吴珏霏), Lili Zhang(张丽丽), Chao Xiong(熊超), and Yanpeng Qi(齐彦鹏) Pressure-induced superconductivity and phase transition in PbSe and PbTe 2024 Chin. Phys. B 33 126105
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