Low thermal expansion and broad band photoluminescence of Zr0.1Al1.9Mo2.9V0.1O12

doi:10.1088/1674-1056/abcf39

Abstract A new material of Zr_0.1Al_1.9Mo_2.9V_0.1O₁₂ is synthesized by the traditional solid state synthesis method. The phase transition, coefficient of thermal expansion, and luminescence properties of Zr_0.1Al_1.9Mo_2.9V_0.1O₁₂ are explored with Raman spectrometer, dilatometer, and x-ray diffraction (XRD) diffractometer. The results show that the Zr_0.1Al_1.9Mo_2.9V_0.1O₁₂ possesses the strong broad-band luminescence characteristics almost in the whole visible region. The sample is crystallized in a monoclinic structure group of P2₁/a (No. 14) crystallized at room temperature (RT). The crystal is changed from monoclinic to orthorhombic structure when the temperature increases to 463 K. The material has very low thermal expansion performance in a wide temperature range. Its excellent low thermal expansion and strong pale green light properties in a wide temperature range suggest its potential applications in light-emitting diode (LED) and other optoelectronic devices.

Keywords: low thermal expansion phase transition x-ray diffraction (XRD) Raman spectrum luminescence

Received: 31 July 2020
Revised: 23 November 2020
Accepted manuscript online: 01 December 2020

PACS:	65.40.De	(Thermal expansion; thermomechanical effects)
	81.05.Je	(Ceramics and refractories (including borides, carbides, hydrides, nitrides, oxides, and silicides))
	61.50.-f	(Structure of bulk crystals)
	78.30.-j	(Infrared and Raman spectra)

Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 11874328, U1731121, and 41401384) and the Shandong Province Higher Educational Science and Technology Program, China (Grant No. J17KB127).

Corresponding Authors: ^†Corresponding author. E-mail: Wangjunping-99@163.com

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Jun-Ping Wang(王俊平), Qing-Dong Chen(陈庆东), Li-Gang Chen(陈立刚), Yan-Jun Ji(纪延俊), You-Wen Liu(刘友文), and Er-Jun Liang(梁二军) Low thermal expansion and broad band photoluminescence of Zr_0.1Al_1.9Mo_2.9V_0.1O₁₂ 2021 Chin. Phys. B 30 036501

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Low thermal expansion and broad band photoluminescence of Zr0.1Al1.9Mo2.9V0.1O12

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Low thermal expansion and broad band photoluminescence of Zr_0.1Al_1.9Mo_2.9V_0.1O₁₂