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Concentration effect of the near-infrared quantum cutting of 1788-nm luminescence of Tm3+ ion in (Y1-xTmx)3Al5O12 powder phosphor |
Chen Xiao-Bo (陈晓波)a, Li Song (李崧)a, Ding Xian-Lin (丁贤林)b, Yang Xiao-Dong (杨小冬)a, Liu Quan-Lin (刘泉林)b, Gao Yan (高燕)c, Sun Ping (孙萍)a, Yang Guo-Jian (杨国建)a |
a Department of Physics and Applied Optics Beijing Area Major Laboratory, Beijing Normal University, Beijing 100875, China;
b School of Materials Science and Engineering & State Key Laboratory for Advanced Metals and Materials, University of Science and Technology of Beijing, Beijing 100083, China;
c Laboratory of Nanomaterials, National Center for Nanoscience and Technology of China, Beijing 100190, China |
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Abstract In the present paper, the concentration effect of near-infrared quantum cutting of Tm3+ ion in (Y1-xTmx)3Al5O12 powder phosphor is studied by means of experiments and calculations. In addition, the absorption spectra, visible-to-nearinfrared excitation and emission spectra, and fluorescence lifetimes are measured. It is found that (Y1-xTmx)3Al5O12 powder phosphor has a strong four-photon near-infrared quantum cutting luminescence of 1788.0-nm 3F4 →3H6 fluorescence of Tm3+ ion, when excited by 357.0-nm light. It is also found that the up-limit of the four-photon near-infrared quantum cutting luminescence efficiency of (Y0.700Tm0.300)3Al5O12 powder phosphor is approximately 302.19%. To the knowledge of the authors, this is the first time that a near-infrared quantum cutting efficiency up-limit exceeding 300% has been reported. The results of this manuscript are valuable in aiding the probing of the new generation Ge solar cell.
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Received: 28 February 2014
Revised: 27 April 2014
Accepted manuscript online:
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PACS:
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78.55.-m
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(Photoluminescence, properties and materials)
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78.56.-a
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(Photoconduction and photovoltaic effects)
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78.30.-j
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(Infrared and Raman spectra)
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Fund: Project supported by the National Natural Science Foundation of China (Grant No. 10674019) and the Significant Project of Fundamental Research Funds for the Central Universities of China (Grant No. 212-105560GK). |
Corresponding Authors:
Chen Xiao-Bo
E-mail: chen78xb@sina.com
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Cite this article:
Chen Xiao-Bo (陈晓波), Li Song (李崧), Ding Xian-Lin (丁贤林), Yang Xiao-Dong (杨小冬), Liu Quan-Lin (刘泉林), Gao Yan (高燕), Sun Ping (孙萍), Yang Guo-Jian (杨国建) Concentration effect of the near-infrared quantum cutting of 1788-nm luminescence of Tm3+ ion in (Y1-xTmx)3Al5O12 powder phosphor 2014 Chin. Phys. B 23 087809
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