Abstract The negatively charged nitrogen vacancy (NV) center ensemble in as-grown chemical vapor deposition (CVD) diamond is a promising candidate for quantum sensing due to its long coherence time and excellent optical properties. However, achieving a high concentration of NV centers in as-grown CVD diamond remains a critical challenge, which constrains the performance of NV based sensors. In this study, we observe that NV center formation efficiency is significantly enhanced during the initial growth phase, with a coherence time of 1.1 μs. These findings demonstrate that high-concentration NV centers can be achieved in as-grown diamonds, greatly enhancing their utility in high-performance magnetometers and quantum sensing.
Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 11374280 and 50772110).
Corresponding Authors:
Wei Zhu, Guanzhong Wang
E-mail: zhuw@ustc.edu.cn;gzwang@ustc.edu.cn
Cite this article:
Yuanjie Yang(杨元杰), Shengran Lin(林盛然), Jiaxin Zhao(赵嘉昕), Changfeng Weng(翁长风), Liren Lou(楼立人), Wei Zhu(祝巍), and Guanzhong Wang(王冠中) Ultrahigh concentration of NV- centers embedded in the CVD epi-diamond layer near the interface with an HPHT diamond substrate 2025 Chin. Phys. B 34 056102
[1] Takeuchi M, Yasuoka M, Ishii M, Ohtani N and Shikata S 2023 Diam. Relat. Mater. 140 110510 [2] Zou D, Shen S, Li L, Wang Q, Liang K, Chen L, Wu G and Shen W 2024 Phys. B 676 415614 [3] Bai R, Zhu X, Yang F, Gao T, Wang Z, Yu L, Wang J, Zhou L and Du G 2022 Chin. Phys. B 31 074203 [4] Wang J, Feng F, Zhang J, Chen J, Zheng Z, Guo L, Zhang W, Song X, Guo G, Fan L, Zou C, Lou L, Zhu W and Wang G 2015 Phys. Rev. B 91 155404 [5] Xu K, Xie T, Li Z, Xu X, Wang M, Ye X, Kong F, Geng J, Duan C, Shi F and Du J 2017 Phys. Rev. Lett. 118 130504 [6] Masuyama Y, Suzuki K, Hekizono A, Iwanami M, Hatano M, Iwasaki T and Ohshima T 2021 Sensors 21 977 [7] Budakian R, Finkler A, Eichler A, Poggio M, Degen C L, Tabatabaei S, Lee I, Hammel P C, Eugene S P, Taminiau T H, Walsworth R L, London P, Bleszynski Jayich A, Ajoy A, Pillai A, Wrachtrup J, Jelezko F, Bae Y, Heinrich A J, Ast C R, Bertet P, Cappellaro P, Bonato C, Altmann Y and Gauger E 2024 Nanotechnology 35 412001 [8] Atatüre M, Englund D, Vamivakas N, Lee S Y and Wrachtrup J 2018 Nat. Rev. Mater. 3 38 [9] Delle Donne C, Iuliano M, Van Der Vecht B, Ferreira G M, Jirovská H, Van Der Steenhoven T J W, Dahlberg A, Skrzypczyk M, Fioretto D, Teller M, Filippov P, Montblanch A R P, Fischer J, Van Ommen H B, Demetriou N, Leichtle D, Music L, Ollivier H, Te Raa I, Kozlowski W, Taminiau T H, Pawełczak P, Northup T E, Hanson R and Wehner S 2025 Nature 639 321 [10] Shandilya P K, Flagan S, Carvalho N C, Zohari E, Kavatamane V K, Losby J E and Barclay P E 2022 J. Light. Technol. 40 7538 [11] Basu T, Patra A, Murali M, Saini M, Banerjee A and Som 2025 ACS Omega 10 2372 [12] Liu X, Cui J, Sun F, Song X, Feng F, Wang J, Zhu W, Lou L and Wang G 2013 Appl. Phys. Lett. 103 143105 [13] Hei L F, Zhao Y, Wei J J, Liu J L, Li C M, Tang W Z and Lu F X 2016 Diam. Relat. Mater. 69 33 [14] Samlenski R, Haug C, Brenn R, Wild C, Locher R and Koidl P 1995 Appl. Phys. Lett. 67 2798 [15] Feng F, Wang J, Zhang W, Zhang J, Lou L, Zhu W and Wang G 2016 Appl. Phys. A 122 944 [16] Yokota Y, Kawarada H and Hiraki A 1990 Jpn. J. Appl. Phys. 29 L2232 [17] Romach Y, Müller C, Unden T, Rogers L J, Isoda T, Itoh K M, Markham M, Stacey A, Meijer J, Pezzagna S, Naydenov B, McGuinness L P, Bar-Gill N and Jelezko F 2015 Phys. Rev. Lett. 114 017601 [18] Hounsome L S, Jones R, Martineau P M, Fisher D, Shaw M J, Briddon P R and Ö berg S 2006 Phys. Rev. B 73 125203 [19] Ohno K, Joseph Heremans F, Bassett L C, Myers B A, Toyli D M, Bleszynski Jayich A C, Palmstrøm C J and Awschalom D D 2012 Appl. Phys. Lett. 101 082413 [20] Tallaire A, Achard J, Silva F, Sussmann R S, Gicquel A and Rzepka E 2004 Phys. Status Solidi A 201 2419 [21] Woods G S, Van Wyk J A and Collins A T 1990 Philos. Mag. B 62 589 [22] Liu J L, Zheng Y T, Lin L Z, Zhao Y, Chen L X, Wei J J, Wang J J, Guo J C, Feng Z H and Li C M 2018 J. Mater. Sci. 53 13030 [23] Tallaire A, Mayer L, Brinza O, Pinault-Thaury M A, Debuisschert T and Achard J 2017 Appl. Phys. Lett. 111 143101 [24] Anon [25] Martineau P M, Lawson S C, Taylor A J, Quinn S J, Evans D J F and Crowder M J 2004 Gems Gemol. 40 2 [26] Edmonds A M, D’Haenens-Johansson U F S, Cruddace R J, NewtonM E, Fu K M C, Santori C, Beausoleil R G, Twitchen D J and Markham M L 2012 Phys. Rev. B 86 035201 [27] Bou P, Vandenbulcke L, Herbin R and Hillion F 1992 J. Mater. Res. 7 2151 [28] Dréau A, Lesik M, Rondin L, Spinicelli P, Arcizet O, Roch J F and Jacques V 2011 Phys. Rev. B 84 195204 [29] Hu X, Liu G Q, Xu Z C and Pan X Y 2012 Chin. Phys. Lett. 29 024210 [30] Dutt M V G, Childress L, Jiang L, Togan E, Maze J, Jelezko F, Zibrov A S, Hemmer P R and Lukin M D 2007 Science 316 1312 [31] Ding S, Zhang J, Su K, Ren Z, Chen J, Yang Z, Zhang J and Hao Y 2024 Sci. China Mater. 67 2329 [32] Acosta V M, Bauch E, Ledbetter M P, Santori C, Fu K M C, Barclay P E, Beausoleil R G, Linget H, Roch J F, Treussart F, Chemerisov S, Gawlik W and Budker D 2009 Phys. Rev. B 80 115202 [33] Kleinsasser E E, Stanfield M M, Banks J K Q, Zhu Z, Li W D, Acosta V M, Watanabe H, Itoh K M and Fu K M C 2016 Appl. Phys. Lett. 108 202401 [34] Maertz B J, Wijnheijmer A P, Fuchs G D, Nowakowski M E and Awschalom D D 2010 Appl. Phys. Lett. 96 092504 [35] Le Sage D, Pham L M, Bar-Gill N, Belthangady C, LukinMD, Yacoby A and Walsworth R L 2012 Phys. Rev. B 85 121202
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