Special Issue:
SPECIAL TOPIC — States and new effects in nonequilibrium
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SPECIAL TOPIC—States and new effects in nonequilibrium |
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Optical manipulation of the topological phase in ZrTe5 revealed by time- and angle-resolved photoemission |
Chaozhi Huang(黄超之)1,†, Chengyang Xu(徐骋洋)1,†, Fengfeng Zhu(朱锋锋)1, Shaofeng Duan(段绍峰)1, Jianzhe Liu(刘见喆)1, Lingxiao Gu(顾凌霄)1, Shichong Wang(王石崇)1, Haoran Liu(刘浩然)1, Dong Qian(钱冬)1,2,3,‡, Weidong Luo(罗卫东)1,2,§, and Wentao Zhang(张文涛)1,2,¶ |
1 Key Laboratory of Artificial Structures and Quantum Control(Ministry of Education), School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240, China; 2 Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210093, China; 3 Tsung-Dao Lee Institute, Shanghai Jiao Tong University, Shanghai 200240, China |
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Abstract High-resolution time- and angle-resolved photoemission measurements were conducted on the topological insulator ZrTe5. With strong femtosecond photoexcitation, a possible ultrafast phase transition from a weak to a strong topological insulating phase was experimentally realized by recovering the energy gap inversion in a time scale that was shorter than 0.15 ps. This photoinduced transient strong topological phase can last longer than 2 ps at the highest excitation fluence studied, and it cannot be attributed to the photoinduced heating of electrons or modification of the conduction band filling. Additionally, the measured unoccupied electronic states are consistent with the first-principles calculation based on experimental crystal lattice constants, which favor a strong topological insulating phase. These findings provide new insights into the longstanding controversy about the strong and weak topological properties in ZrTe5, and they suggest that many-body effects including electron—electron interactions must be taken into account to understand the equilibrium weak topological insulating phase in ZrTe5.
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Received: 15 October 2023
Revised: 16 November 2023
Accepted manuscript online: 17 November 2023
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PACS:
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79.60.-i
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(Photoemission and photoelectron spectra)
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74.25.Jb
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(Electronic structure (photoemission, etc.))
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73.20.At
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(Surface states, band structure, electron density of states)
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78.47.J-
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(Ultrafast spectroscopy (<1 psec))
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Fund: W. T. Z. acknowledges support from the National Key R&D Program of China (Grant Nos. 2021YFA1400202 and 2021YFA1401800), the National Natural Science Foundation of China (Grant Nos. 12141404 and 11974243), and the Natural Science Foundation of Shanghai (Grant Nos. 22ZR1479700 and 23XD1422200). S. F. D. acknowledges support from the China Postdoctoral Science Foundation (Grant No. 2022M722108). D.Q. acknowledges support from the National Key R&D Program of China (Grant Nos. 2022YFA1402400 and 2021YFA1400100) and the National Natural Science Foundation of China (Grant No. 12074248). |
Corresponding Authors:
Dong Qian, Weidong Luo, Wentao Zhang
E-mail: dqian@sjtu.edu.cn;wdluo@sjtu.edu.cn;wentaozhang@sjtu.edu.cn
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Cite this article:
Chaozhi Huang(黄超之), Chengyang Xu(徐骋洋), Fengfeng Zhu(朱锋锋), Shaofeng Duan(段绍峰), Jianzhe Liu(刘见喆), Lingxiao Gu(顾凌霄), Shichong Wang(王石崇), Haoran Liu(刘浩然), Dong Qian(钱冬), Weidong Luo(罗卫东), and Wentao Zhang(张文涛) Optical manipulation of the topological phase in ZrTe5 revealed by time- and angle-resolved photoemission 2024 Chin. Phys. B 33 017901
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