Please wait a minute...
Chin. Phys. B, 2017, Vol. 26(5): 058201    DOI: 10.1088/1674-1056/26/5/058201
INTERDISCIPLINARY PHYSICS AND RELATED AREAS OF SCIENCE AND TECHNOLOGY Prev   Next  

Wavelength dependence of electron localization of H2+ and its isotopomers in the UV-pump-probe scheme

Shan Xue(薛山)1,2, Hong-Chuan Du(杜洪川)1,2, Sheng-Jun Yue(岳生俊)1,2, Hong-Mei Wu(吴红梅)1,2, Bi-Tao Hu(胡碧涛)1,2
1 School of Nuclear Science and Technology, Lanzhou University, Lanzhou 730000, China;
2 Key Laboratory of Special Function Materials and Structure Design (Ministry of Education), Lanzhou University, Lanzhou 730000, China
Abstract  

The wavelength dependence of electron localization of H2+ and its isotopomers in the ultraviolet pump-probe scheme is investigated by numerically solving the time-dependent Schrödinger equation. By combining with a semiclassical method, an effective analytical formula expressed in the adiabatic representation is established to describe the localization probability with several zero crossings. A stable zone with respect to the laser intensity and carrier envelope phase is found at a relatively long probe wavelength. Finally, the critical probe wavelengths to reach at the stable zone are derived by using the three-dimensional model. Slower nuclear motion of heavier isotopomers leads to a longer critical wavelength.

Keywords:  strong field physics      electron localization      molecular dissociation      pump-probe  
Received:  02 October 2016      Revised:  06 December 2016      Accepted manuscript online: 
PACS:  82.53.Eb (Pump probe studies of photodissociation)  
  42.50.Hz (Strong-field excitation of optical transitions in quantum systems; multiphoton processes; dynamic Stark shift)  
  33.80.Rv (Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states))  
Fund: 

Project supported by the National Natural Science Foundation of China (Grant Nos. 11404153, 11135002, 11475076, and 11405077) and the Fundamental Research Funds for the Central Universities of China (Grants Nos. lzujbky-2016-29, lzujbky-2016-31, and lzujbky-2016-209).

Corresponding Authors:  Hong-Chuan Du, Bi-Tao Hu     E-mail:  duhch@lzu.edu.cn;hubt@lzu.edu.cn

Cite this article: 

Shan Xue(薛山), Hong-Chuan Du(杜洪川), Sheng-Jun Yue(岳生俊), Hong-Mei Wu(吴红梅), Bi-Tao Hu(胡碧涛) Wavelength dependence of electron localization of H2+ and its isotopomers in the UV-pump-probe scheme 2017 Chin. Phys. B 26 058201

[1] Zewail A H 2000 J. Phys. Chem. A 104 5660
[2] Brixner T and Gerber G 2003 Chem. Phys. Chem. 4 418
[3] González-Castrillo A, Palacios A, Bachau H and Martín F 2012 Phys. Rev. Lett. 108 063009
[4] Niikura H, Villeneuve D M and Corkum P B 2004 Phys. Rev. Lett. 92 133002
[5] Kremer M, Fischer B, Feuerstein B, de Jesus V L B, Sharma V, Hofrichter C, Rudenko A, Thumm U, Schröter C D, Moshammer R and Ullrich J 2009 Phys. Rev. Lett. 103 213003
[6] Singh K P, He F, Ranitovic P, Cao W, De S, Ray D, Chen S, Thumm U, Becker A, Murnane M M, Kapteyn H C, Litvinyuk I V and Cocke C L 2010 Phys. Rev. Lett. 104 023001
[7] Sansone G, Kelkensberg F, Perez-Torres J F, Morales F, Kling M F, Siu W, Ghafur O, Johnsson P, Swoboda M, Benedetti E, Ferrari F, Lepine F, Sanz-Vicario J L, Zherebtsov S, Znakovskaya I, L'Huillier A, Ivanov M Y, Nisoli M, Martin F and Vrakking M J J 2010 Nature 465 763
[8] Roudnev V, Esry B D and Ben-Itzhak I 2004 Phys. Rev. Lett. 93 163601
[9] Kling M F, Siedschlag Ch, Verhoef A J, Khan J I, Schultze M, Uphues Th, Ni Y F, Uiberacker M, Drescher M, Krausz F and Vrakking M J J 2006 Science 312 246
[10] Liu K, Hong W, Zhang Q and Lu P 2011 Opt. Express 19 26359
[11] Ray D, He F, De S, Cao W, Mashiko H, Ranitovic P, Singh K P, Znakovskaya I, Thumm U, Paulus G G, Kling M F, Litvinyuk I V and Cocke C L 2009 Phys. Rev. Lett. 103 223201
[12] Lan P, Takahashi E J and Midorikawa K 2012 Phys. Rev. A 86 013418
[13] Liu K, Zhang Q and Lu P 2012 Phys. Rev. A 86 033410
[14] He F, Becker A and Thumm U 2008 Phys. Rev. Lett. 101 213002
[15] He F, Ruiz C and Becker A 2007 Phys. Rev. Lett. 99 083002
[16] Fischer B, Kremer M, Pfeifer T, Feuerstein B, Sharma V, Thumm U, Schröter C D, Moshammer R and Ullrich J 2010 Phys. Rev. Lett. 105 223001
[17] Anis F and Esry B D 2012 Phys. Rev. Lett. 109 133001
[18] Niikura H, Corkum P B and Villeneuve D M 2003 Phys. Rev. Lett. 90 203601
[19] Jia Z, Zeng Z, Li R, Xu Z and Deng Y 2014 Phys. Rev. A 89 023419
[20] Lu R F, Zhang P Y and Han K L 2008 Phys. Rev. E 77 066701
[21] Xue S, Du H C, Xia Y and Hu B T 2015 Phys. Rev. A 92 013420
[22] Charron E, GiustiSuzor A and Meis F H 1995 J. Chem. Phys. 103 7359
[23] Mulliken R S 1939 J. Chem. Phys. 7 20
[24] He F 2012 Phys. Rev. A 86 063415
[25] Du H C, Wen Y Z, Wang X S and Hu B T 2014 Chin. Phys. B 23 033202
[26] Xue S, Du H C, Xia Y and Hu B T 2015 Chin. Phys. B 24 054210
[27] Feit M D, Fleck J A and Steiger A 1982 J. Comput. Phys. 47 412
[28] Thachuk M, Ivanov M Y and Wardlaw D M 1996 J. Chem. Phys. 105 4094
[29] Thachuk M, Ivanov M Y and Wardlaw D M 1998 J. Chem. Phys. 109 5747
[30] Herzberg G, Longuet-Higgins H C 1963 Discuss. Faraday Soc. 35 77
[31] Longuet-Higgins H C 1975 Proc. Roy. Soc. Ser. A 344 147
[32] Dietrich P, Ivanov M Y, Ilkov F A and Corkum P B 1996 Phys. Rev. Lett. 77 4150
[33] Yu C, He H, Wang Y, Shi Q, Zhang Y and Lu R 2014 J. Phys. B: At. Mol. Opt. Phys. 47 055601
[34] Frasinski L J, Posthumus J H, Plumridge J and Codling K 1999 Phys. Rev. Lett. 83 3625
[1] Polarization-dependent ultrafast carrier dynamics in GaAs with anisotropic response
Ya-Chao Li(李亚超), Chao Ge(葛超), Peng Wang(汪鹏), Shuang Liu(刘爽), Xiao-Ran Ma(麻晓冉), Bing Wang(王冰), Hai-Ying Song(宋海英), and Shi-Bing Liu(刘世炳). Chin. Phys. B, 2022, 31(6): 067102.
[2] HeTDSE: A GPU based program to solve the full-dimensional time-dependent Schrödinger equation for two-electron helium subjected to strong laser fields
Xi Zhao(赵曦), Gangtai Zhang(张刚台), Tingting Bai(白婷婷), Jun Wang(王俊), and Wei-Wei Yu(于伟威). Chin. Phys. B, 2021, 30(7): 073201.
[3] Nonadiabatic molecular dynamics simulation of ${{\rm{C}}}_{2}{{\rm{H}}}_{2}^{2+}$ in a strong laser field
Ji-Gen Chen(陈基根), Gang-Tai Zhang(张刚台), Ting-Ting Bai(白婷婷), Jun Wang(王俊), Ping-Ping Chen(陈平平), Wei-Wei Yu(于伟威)§, and Xi Zhao(赵曦)¶. Chin. Phys. B, 2020, 29(11): 113202.
[4] The unique magnetic damping enhancement in epitaxial Co2Fe1-xMnxAl films
Shu-Fa Li(李树发), Chu-Yuan Cheng(程樗元), Kang-Kang Meng(孟康康), Chun-Lei Chen(陈春雷). Chin. Phys. B, 2019, 28(9): 097502.
[5] Phase-dependent double optomechanically induced transparency in a hybrid optomechanical cavity system with coherently mechanical driving
Shi-Chao Wu(吴士超), Li-Guo Qin(秦立国), Jian Lu(鹿建), Zhong-Yang Wang(王中阳). Chin. Phys. B, 2019, 28(7): 074204.
[6] Opto-electromechanically induced transparency in a hybrid opto-electromechanical system
Hui Liu(刘慧), Li-Guo Qin(秦立国), Li-Jun Tian(田立君), Hong-Yang Ma(马鸿洋). Chin. Phys. B, 2019, 28(10): 108502.
[7] Attosecond laser station
Hao Teng(滕浩), Xin-Kui He(贺新奎), Kun Zhao(赵昆), Zhi-Yi Wei(魏志义). Chin. Phys. B, 2018, 27(7): 074203.
[8] Ultra-fast x-ray-dynamic experimental subsystem
Liming Chen(陈黎明), Xin Lu(鲁欣), Dazhang Li(李大章), Yifei Li(李毅飞). Chin. Phys. B, 2018, 27(7): 074101.
[9] Theoretical study of the odd–even-order harmonic generation for asymmetric ions in non-Born–Oppenheimer approximation
Sheng-Jun Yue(岳生俊), Hong-Chuan Du(杜洪川), Hong-Mei Wu(吴红梅), Shan Xue(薛山), Jia-Chen Zhao(赵家琛), Bi-Tao Hu(胡碧涛). Chin. Phys. B, 2017, 26(7): 074215.
[10] Density function theoretical study on the complex involved in Th atom-activated C-C bond in C2H6
Qing-Qing Wang(王青青), Peng Li(李鹏), Tao Gao(高涛), Hong-Yan Wang(王红艳), Bing-Yun Ao(敖冰云). Chin. Phys. B, 2016, 25(6): 063102.
[11] Triple optomechanical induced transparency in a two-cavity system
Shi-Chao Wu(吴士超), Li-Guo Qin(秦立国), Jun Jing(景俊), Guo-Hong Yang(杨国宏), Zhong-Yang Wang(王中阳). Chin. Phys. B, 2016, 25(5): 054203.
[12] Investigation of electron localization in harmonic emission from asymmetric molecular ion
Zhang Cai-Ping (张彩萍), Miao Xiang-Yang (苗向阳). Chin. Phys. B, 2015, 24(4): 043302.
[13] Gigahertz longitudinal acoustic phonons originating from ultrafast ligand field transitions in hematite thin films
Xu Yue (徐悦), Jin Zuan-Ming (金钻明), Zhang Zheng-Bing (张郑兵), Zhang Ze-Yu (张泽宇), Lin Xian (林贤), Ma Guo-Hong (马国宏), Cheng Zhen-Xiang (程振祥). Chin. Phys. B, 2014, 23(4): 044206.
[14] Determination of temporal structure of femtosecond laser pulses by means of the laser-induced air plasma
Zhang Nan (张楠), Bao Wen-Xia (包文霞), Yang Jing-Hui (杨景辉), Zhu Xiao-Nong (朱晓农). Chin. Phys. B, 2013, 22(5): 054209.
[15] Study on wave packet dynamics of E1g+ state of Li2 with femtosecond-resolved photoelectron spectra
Liu Yu-Fang(刘玉芳), Liu Rui-Qiong(刘瑞琼), and Ding Jun-Xia(丁俊霞). Chin. Phys. B, 2010, 19(3): 033301.
No Suggested Reading articles found!