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Controlling the contributions to high-order harmonic generation from different nuclei of N2 with an orthogonally polarizedtwo-color laser field |
Hui Du(杜慧), Xue-Fei Pan(潘雪飞), Hai-Feng Liu(刘海凤), Hong-Dan Zhang(张宏丹), Jun Zhang(张军), Jing Guo(郭静), Xue-Shen Liu(刘学深) |
Institute of Atomic and Molecular Physics, Jilin University, Changchun 130012, China |
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Abstract The generation of high-order harmonic and the attosecond pulse of the N2 molecule with an orthogonally polarized two-color laser field are investigated by the strong-field Lewenstein model. We show that the control of contributions to high-order harmonic generation (HHG) from different nuclei is realized by properly selecting the relative phase. When the relative phase is chosen to be φ=0.4π, the contribution to HHG from one nucleus is much more than that from another. Interference between two nuclei can be suppressed greatly; a supercontinuum spectrum of HHG appears from 40 eV to 125 eV. The underlying physical mechanism is well explained by the time-frequency analysis and the semi-classical three-step model with a finite initial transverse velocity. By superposing several orders of harmonics, an isolated attosecond pulse with a duration of 80 as can be generated.
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Received: 07 April 2016
Revised: 25 April 2016
Accepted manuscript online:
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PACS:
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32.80.Rm
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(Multiphoton ionization and excitation to highly excited states)
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42.65.Ky
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(Frequency conversion; harmonic generation, including higher-order harmonic generation)
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42.65.Re
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(Ultrafast processes; optical pulse generation and pulse compression)
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Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 11271158, 61575077, and 11574117). |
Corresponding Authors:
Xue-Shen Liu
E-mail: liuxs@jlu.edu.cn
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Cite this article:
Hui Du(杜慧), Xue-Fei Pan(潘雪飞), Hai-Feng Liu(刘海凤), Hong-Dan Zhang(张宏丹), Jun Zhang(张军), Jing Guo(郭静), Xue-Shen Liu(刘学深) Controlling the contributions to high-order harmonic generation from different nuclei of N2 with an orthogonally polarizedtwo-color laser field 2016 Chin. Phys. B 25 093202
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