Lithium-ion transport in inorganic solid state electrolyte

doi:10.1088/1674-1056/25/1/018211

Abstract

An overview of ion transport in lithium-ion inorganic solid state electrolytes is presented, aimed at exploring and designing better electrolyte materials. Ionic conductivity is one of the most important indices of the performance of inorganic solid state electrolytes. The general definition of solid state electrolytes is presented in terms of their role in a working cell (to convey ions while isolate electrons), and the history of solid electrolyte development is briefly summarized. Ways of using the available theoretical models and experimental methods to characterize lithium-ion transport in solid state electrolytes are systematically introduced. Then the various factors that affect ionic conductivity are itemized, including mainly structural disorder, composite materials and interface effects between a solid electrolyte and an electrode. Finally, strategies for future material systems, for synthesis and characterization methods, and for theory and calculation are proposed, aiming to help accelerate the design and development of new solid electrolytes.

Keywords: lithium-ion batteries solid state electrolyte ionic conductivity ion transport mechanism

Received: 18 May 2015
Revised: 22 July 2015
Accepted manuscript online:

PACS:	82.47.Aa	(Lithium-ion batteries)
	65.40.gk	(Electrochemical properties)

Fund:

Project supported by the National Natural Science Foundation of China (Grant No. 51372228), the Shanghai Pujiang Program, China (Grant No. 14PJ1403900), and the Shanghai Institute of Materials Genome from the Shanghai Municipal Science and Technology Commission, China (Grant No. 14DZ2261200).

Corresponding Authors: Si-Qi Shi, Hong Li
E-mail: sqshi@shu.edu.cn;hli@aphy.iphy.ac.cn

Cite this article:

Jian Gao(高健), Yu-Sheng Zhao(赵予生), Si-Qi Shi(施思齐), Hong Li(李泓) Lithium-ion transport in inorganic solid state electrolyte 2016 Chin. Phys. B 25 018211

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