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Special Issue:
TOPICAL REVIEW — The third carbon: Carbyne with one-dimensional sp-carbon
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| TOPICAL REVIEW—The third carbon: Carbyne with one-dimensional sp-carbon |
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Raman spectroscopy of isolated carbyne chains confined in carbon nanotubes: Progress and prospects |
| Johannes M. A. Lechner, Pablo Hernández López, and Sebastian Heeg† |
| Institut für Physik and IRIS Adlershof, Humboldt Universität zu Berlin, 12489 Berlin, Germany |
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Abstract Carbyne is an infinitely long linear chain of carbon atoms with sp1 hybridization and the truly one-dimensional allotrope of carbon. While obtaining freestanding carbyne is still an open challenge, the study of confined carbyne, linear chains of carbon encapsulated in carbon nanotubes, provides a pathway to explore carbyne and its remarkable properties in a well-defined environment. In this review, we discuss the basics and recent advances in studying single confined carbyne chains by Raman spectroscopy, which is their primary spectroscopic characterization method. We highlight where single carbyne chain studies are needed to advance our understanding of confined carbyne as a material system and provide an overview of the open questions that need to be addressed and of those aspects currently under debate.
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Received: 01 July 2022
Revised: 22 September 2022
Accepted manuscript online: 29 September 2022
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PACS:
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78.67.Ch
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(Nanotubes)
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78.67.Uh
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(Nanowires)
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| Fund: Johannes M. A. Lechner, Pablo Hernandez López, and Sebastian Heeg acknowledge funding from the Deutsche Forschungsgemeinschaft (DFG) under the Emmy Noether Initiative (HE 8642/1-1). |
Corresponding Authors:
Sebastian Heeg
E-mail: sebastian.heeg@physik.hu-berlin.de
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Cite this article:
Johannes M. A. Lechner, Pablo Hernández López, and Sebastian Heeg Raman spectroscopy of isolated carbyne chains confined in carbon nanotubes: Progress and prospects 2022 Chin. Phys. B 31 127801
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