Content of ATOMIC AND MOLECULAR PHYSICS in our journal

        Published in last 1 year |  In last 2 years |  In last 3 years |  All
    Please wait a minute...
    For selected: Toggle thumbnails
    Low-energy inelastic electron scattering from carbon monoxide: Excitation and de-excitation of the X1Σ+, a3Π, a'3Σ+, A1Π, d3Δ, e3Σ-, I1Σ- and D1Δ electronic states
    Pengyu Wei(卫鹏宇), Chaowen Huang(黄朝文), Xinlu Cheng(程新路), and Hong Zhang(张红)
    Chin. Phys. B, 2024, 33 (4): 043101.   DOI: 10.1088/1674-1056/ad123e
    Abstract12)      PDF (703KB)(3)      
    Cross-sections for electronic excitation and de-excitation among the ground state and lowest-lying seven electronic excited states of carbon monoxide (CO) by low-energy electron impact are computed using the $R$-matrix method. The excitation cross-sections from the ground state to the electronic states ${\rm a}^{3}\Pi $, ${\rm a}^{\prime 3}\Sigma^{+}$ and ${\rm A}^{1}\Pi $ agree with previous experimental and theoretical results. In addition, the cross-sections for the ${\rm I}^{1}\Sigma^{-}$ and ${\rm D}^{1}\Delta $ states of CO, which will cascade to CO ${\rm a}^{\prime 3}\Sigma^{+}$ and ${\rm A}^{1}\Pi $ states, are calculated. Furthermore, in contrast to the typical increase in electronic excitation cross-sections with collision energy, the de-excitation cross-sections show a negative trend with increasing energy.
    A proposal for detecting weak electromagnetic waves around 2.6 μm wavelength with Sr optical clock
    Ruo-Shui Han(韩弱水), Wei Wang(王伟), and Tao Wang(汪涛)
    Chin. Phys. B, 2024, 33 (4): 043201.   DOI: 10.1088/1674-1056/ad1b45
    Abstract18)      PDF (955KB)(6)      
    Infrared signal detection is widely used in many fields. Due to the detection principle, however, the accuracy and range of detection are limited. Thanks to the ultra stability of the 87Sr optical lattice clock, external infrared electromagnetic wave disturbances can be responded to. Utilizing the ac Stark shift of the clock transition, we propose a new method to detect infrared signals. According to our calculations, the theoretical detection accuracy in the vicinity of its resonance band of 2.6 μm can reach the order of 10-14 W, while the minimum detectable signal of common detectors is on the order of 10-10 W.
    Absolute partial and total ionization cross sections of carbon monoxide with electron collision from 350 eV to 8000 eV
    Taj Wali Khan, Weizhe Huang(黄伟哲), Enliang Wang(王恩亮), Xu Shan(单旭), and Xiangjun Chen(陈向军)
    Chin. Phys. B, 2024, 33 (4): 043401.   DOI: 10.1088/1674-1056/ad20dd
    Abstract25)      PDF (800KB)(17)      
    The absolute partial and total cross sections for electron impact ionization of carbon monoxide are reported for electron energies from 350 eV to 8000 eV. The product ions (CO+, C+, O+, CO2+, C2+, and O2+) are measured by employing an ion imaging mass spectrometer and two ion-pair dissociation channels (C+ + O+ and C2+ + O+) are identified. The absolute cross sections for producing individual ions and their total, as well as for the ion-pair dissociation channels are obtained by normalizing the data of CO+ to that of Ar+ from CO—Ar mixture target with a fixed 1:1 ratio. The overall errors are evaluated by considering various kinds of uncertainties. A comprehensive comparison is made with the available data, which shows a good agreement with each other over the energy ranges that are overlapped. This work presents new cross-section data with electron energies above 1000 eV.
    Microscopic mechanism of plasmon-mediated photocatalytic H2 splitting on Ag-Au alloy chain
    Yuhui Song(宋玉慧), Yirui Lu(芦一瑞), Axin Guo(郭阿鑫), Yifei Cao(曹逸飞), Jinping Li(李金萍), Zhengkun Fu(付正坤), Lei Yan(严蕾), and Zhenglong Zhang(张正龙)
    Chin. Phys. B, 2024, 33 (3): 033101.   DOI: 10.1088/1674-1056/ad123d
    Abstract44)   HTML0)    PDF (3141KB)(34)      
    Alloy nanostructures supporting localized surface plasmon resonances has been widely used as efficient photocatalysts, but the microscopic mechanism of alloy compositions enhancing the catalytic efficiency is still unclear. By using time-dependent density functional theory (TDDFT), we analyze the real-time reaction processes of plasmon-mediated H2 splitting on linear Ag-Au alloy chains when exposed to femtosecond laser pulses. It is found that H2 splitting rate depends on the position and proportion of Au atoms in alloy chains, which indicates that specially designed Ag-Au alloy is more likely to induce the reaction than pure Ag chain. Especially, more electrons directly transfer from the alloy chain to the anti-bonding state of H2, thereby accelerating the H2 splitting reaction. These results establish a theoretical foundation for comprehending the microscopic mechanism of plasmon-induced chemical reaction on the alloy nanostructures.
    Core level excitation spectra of La and Mn ions in LaMnO3
    Fujian Li(李福建), Xinlu Cheng(程新路), and Hong Zhang(张红)
    Chin. Phys. B, 2024, 33 (3): 033201.   DOI: 10.1088/1674-1056/acfaf5
    Abstract35)   HTML0)    PDF (1028KB)(44)      
    Manganese-based perovskite is popular for research on ferromagnetic materials, and its spectroscopic studies are essential for understanding its electronic structure, dielectric, electrical, and magnetic properties. In this paper, the M-edge spectra of La ions and the M-edge, L-edge, and K-edge spectra of Mn ions in LaMnO3 are calculated by considering both the free-ion multiplet calculation and the crystal field effects. We analyze spectral shapes, identify peak origins, and estimate the oxidation states of La and Mn ions in LaMnO3 theoretically. It is concluded that La ions in LaMnO3 predominantly exist in the trivalent state, while Mn ions exist primarily in the trivalent state with a minor presence of tetravalent ions. Furthermore, the calculated spectra are in better conformity with the experimental spectra when the proportion of Mn3+ is 90% and Mn4+ is 10%. This article enhances our comprehension of the oxidation states of La and Mn within the crystal and also provides a valuable guidance for spectroscopic investigations of other manganates.
    Theoretical investigations of population trapping phenomena in atomic four-color, three-step photoionization scheme
    Xiao-Yong Lu(卢肖勇) and Ya-Peng Sun(孙亚鹏)
    Chin. Phys. B, 2024, 33 (3): 033202.   DOI: 10.1088/1674-1056/ad10fc
    Abstract40)   HTML0)    PDF (2660KB)(32)      
    The four-color three-step selective photoionization process of atom is very important in laser isotope separation technology. The population trapping phenomena and their influences are studied theoretically in monochromatic and non-monochromatic laser fields based on the density matrix theory in this work. Time evolutions of the photoionization properties of the four-color, three-step process are given. The population trapping effects occur intensely in monochromatic excitation, while it gradually turns weak as the laser bandwidth increases. The effects of bandwidth, Rabi frequency, time delay, and frequency detuning on the population trapping effect are investigated in monochromatic and non-monochromatic laser fields. The effects of laser process parameters and atomic parameters on the effective selective photoionization are also discussed. The ionization probability and selectivity factors, as evaluation indexes, are difficult to improve synchronously by adjusting systematic parameters. Besides, the existence of metastable state may play a negative role when its population is low enough.
    Theoretical investigation of electron-impact ionization of W8+ ion
    Shiping Zhang(张世平), Fangjun Zhang(张芳军), Denghong Zhang(张登红), Xiaobin Ding(丁晓彬), Jun Jiang(蒋军), Luyou Xie(颉录有), Yulong Ma(马玉龙), Maijuan Li(李麦娟), Marek Sikorski, and Chenzhong Dong(董晨钟)
    Chin. Phys. B, 2024, 33 (3): 033401.   DOI: 10.1088/1674-1056/ad1487
    Abstract46)   HTML0)    PDF (822KB)(44)      
    The electron-impact single ionization cross section for W8+ ion has been calculated using flexible atomic code, employing the level-to-level distorted-wave approximation. This calculations takes into account contributions form both direct ionization (DI) and excitation autoionization (EA). However, the theoretical predictions, based solely on the ground state, tends to underestimate the experimental values. This discrepancy can be mitigated by incorporation contributions from excited states. We extended the theoretical analysis, including the contributions from the long-lived metastable states with lifetimes exceeding 1.5×10-5 s. We employed two statistical models to predict the fraction of ground state ions in the parent ion beam. Assuming a 79% fraction of parent ions in ground configuration, the experiment measurements align with the predictions. Furthermore we derived the theoretical cross-section for the ground state as correlated plasma rate coefficients, and compared it with existing data. Despite the uncertainty in our calculations, our results are still acceptable.
    Generating attosecond pulses with controllable polarization from cyclic H32+ molecules by bichromatic circular fields
    Si-Qi Zhang(张思琪), Bing Zhang(张冰), Bo Yan(闫博), Xiang-Qian Jiang(姜向前), and Xiu-Dong Sun(孙秀冬)
    Chin. Phys. B, 2024, 33 (2): 023301.   DOI: 10.1088/1674-1056/ad062b
    Abstract61)   HTML0)    PDF (1070KB)(68)      
    We investigate the polarization properties of harmonics from the cyclic H32+ molecular ions in tailored bichromatic counter-rotating circularly polarized (BCCP) fields by solving the time-dependent Schrödinger equation. The allowed harmonics and their helicities are associated with the symmetry compatibility of the field-target systems, and large intensity difference between adjacent harmonics with opposite helicities appears in a wide spectral range when the BCCP field is at certain rotation angles. We try to explain the intensity difference by using a recombination model based on the quantum-orbit theory and by analyzing the ionization pathways. Moreover, to synthesize attosecond pulse trains with tunable polarization, the intensity difference is manipulated by introducing a seed XUV field, and by changing the relative amplitude ratio as well as the helicity of BCCP fields.
    Structure, electronic, and nonlinear optical properties of superalkaline M3O (M = Li, Na) doped cyclo[18]carbon
    Xiao-Dong Liu(刘晓东), Qi-Liang Lu(卢其亮), and Qi-Quan Luo(罗其全)
    Chin. Phys. B, 2024, 33 (2): 023601.   DOI: 10.1088/1674-1056/ace036
    Abstract68)   HTML0)    PDF (2801KB)(35)      
    Cyclo[18]carbon has received considerable attention thanks to its novel geometric configuration and special electronic structure. Superalkalis have low ionization energy. Doping a superalkali in cyclo[18]carbon is an effective method to improve the optical properties of the system because considerable electron transfer occurs. In this paper, the geometry, bonding properties, electronic structure, absorption spectrum, and nonlinear optical (NLO) properties of superalkaline $M_{3}$O ($M={\rm Li}$, Na)-doped cyclo[18]carbon were studied by using density functional theory. $M_{3}$O and the C$_{18}$ rings are not coplanar. The C$_{18}$ ring still exhibits alternating long and short bonds. The charge transfer between $M_{3}$O and C$_{18}$ forms stable [$M_{3}$O]$^{+}$[C$_{18}$]$^{-}$ ionic complexes. C$_{18}$$M_{3}$O ($M={\rm Li}$, Na) shows striking optical nonlinearity, i.e., their first- and second-order hyperpolarizability ($\beta_{\rm vec}$ and $\gamma_{\vert \vert }$) increase considerably at $\lambda = 1907$ nm and 1460 nm.
    In situ calibrated angle between the quantization axis and the propagating direction of the light field for trapping neutral atoms
    Rui-Jun Guo(郭瑞军), Xiao-Dong He(何晓东), Cheng Sheng(盛诚), Kun-Peng Wang(王坤鹏), Peng Xu(许鹏), Min Liu(刘敏), Jin Wang(王谨), Xiao-Hong Sun(孙晓红), Yong Zeng(曾勇), and Ming-Sheng Zhan(詹明生)
    Chin. Phys. B, 2024, 33 (2): 023701.   DOI: 10.1088/1674-1056/acf11d
    Abstract65)   HTML0)    PDF (792KB)(18)      
    The recently developed magic-intensity trapping technique of neutral atoms efficiently mitigates the detrimental effect of light shifts on atomic qubits and substantially enhances the coherence time. This technique relies on applying a bias magnetic field precisely parallel to the wave vector of a circularly polarized trapping laser field. However, due to the presence of the vector light shift experienced by the trapped atoms, it is challenging to precisely define a parallel magnetic field, especially at a low bias magnetic field strength, for the magic-intensity trapping of 85Rb qubits. In this work, we present a method to calibrate the angle between the bias magnetic field and the trapping laser field with the compensating magnetic fields in the other two directions orthogonal to the bias magnetic field direction. Experimentally, with a constant-depth trap and a fixed bias magnetic field, we measure the respective resonant frequencies of the atomic qubits in a linearly polarized trap and a circularly polarized one via the conventional microwave Rabi spectra with different compensating magnetic fields and obtain the corresponding total magnetic fields via the respective resonant frequencies using the Breit-Rabi formula. With known total magnetic fields, the angle is a function of the other two compensating magnetic fields. Finally, the projection value of the angle on either of the directions orthogonal to the bias magnetic field direction can be reduced to 0(4)° by applying specific compensating magnetic fields. The measurement error is mainly attributed to the fluctuation of atomic temperature. Moreover, it also demonstrates that, even for a small angle, the effect is strong enough to cause large decoherence of Rabi oscillation in a magic-intensity trap. Although the compensation method demonstrated here is explored for the magic-intensity trapping technique, it can be applied to a variety of similar precision measurements with trapped neutral atoms.
    Efficient loading of cesium atoms in a magnetic levitated dimple trap
    Guoqing Zhang(张国庆), Guosheng Feng(冯国胜), Yuqing Li(李玉清), Jizhou Wu(武寄洲), and Jie Ma(马杰)
    Chin. Phys. B, 2024, 33 (2): 023702.   DOI: 10.1088/1674-1056/ad0b03
    Abstract50)   HTML0)    PDF (945KB)(14)      
    We report a detailed study of magnetically levitated loading of ultracold 133Cs atoms in a dimple trap. The atomic sample was produced in a combined red-detuned optical dipole trap and dimple trap formed by two small waist beams crossing a horizontal plane. The magnetic levitation for the 133Cs atoms forms an effective potential for a large number of atoms in a high spatial density. Dependence of the number of atoms loaded and trapped in the dimple trap on the magnetic field gradient and bias field is in good agreement with the theoretical analysis. This method has been widely used to obtain the Bose-Einstein condensation atoms for many atomic species.
    Ab initio potential energy surface and anharmonic vibration spectrum of NF3+
    Yan-Nan Chen(陈艳南), Jian-Gang Xu(徐建刚), Jiang-Peng Fan(范江鹏), Shuang-Xiong Ma(马双雄), Tian Guo(郭甜), and Yun-Guang Zhang(张云光)
    Chin. Phys. B, 2024, 33 (1): 013101.   DOI: 10.1088/1674-1056/ad04c6
    Abstract65)   HTML0)    PDF (1174KB)(15)      
    Potential energy surfaces (PESs), vibrational frequencies, and infrared spectra are calculated for NF3+ using ab initio calculations, based on UCCSD(T)/cc-pVTZ combined with vibrational configuration interaction (VCI). Based on an iterative algorithm, the surfaces (SURF) program adds automatic points to the lattice representation of the potential function, the one-dimensional and two-dimensional PESs are calculated after reaching a convergence threshold, finally the smooth image of the potential energy surface is fitted. The PESs accurately account for the interaction between the different modes, with the mode q6 symmetrical stretching vibrations having the greatest effect on the potential energy change of the whole system throughout the potential energy surface shift. The anharmonic frequencies are obtained when the VCI matrix is diagonalized. Fundamental frequencies, overtones, and combination bands of NF3+ are calculated, which generate the degenerate phenomenon between their frequencies. Finally, the calculated anharmonic frequency is used to plot the infrared spectra. Modal antisymmetric stretching ν5 and symmetric stretching ν6 exhibit a phenomenon of large-intensity borrowing. This study can provide data to support the characterization in the laboratory.
    High-order harmonic generation of ZnO crystals in chirped and static electric fields
    Ling-Yu Zhang(张玲玉), Yong-Lin He(何永林), Zhuo-Xuan Xie(谢卓璇), Fang-Yan Gao(高芳艳), Qing-Yun Xu(徐清芸), Xin-Lei Ge(葛鑫磊), Xiang-Yi Luo(罗香怡), and Jing Guo(郭静)
    Chin. Phys. B, 2024, 33 (1): 013102.   DOI: 10.1088/1674-1056/acfa89
    Abstract100)   HTML2)    PDF (14461KB)(122)      
    High harmonic generation in ZnO crystals under chirped single-color field and static electric field are investigated by solving the semiconductor Bloch equation (SBE). It is found that when the chirp pulse is introduced, the interference structure becomes obvious while the harmonic cutoff is not extended. Furthermore, the harmonic efficiency is improved when the static electric field is included. These phenomena are demonstrated by the classical recollision model in real space affected by the waveform of laser field and inversion symmetry. Specifically, the electron motion in k-space shows that the change of waveform and the destruction of the symmetry of the laser field lead to the incomplete X-structure of the crystal-momentum-resolved (k-resolved) inter-band harmonic spectrum. Furthermore, a pre-acceleration process in the solid four-step model is confirmed.
    Collision off-axis position dependence of relativistic nonlinear Thomson inverse scattering of an excited electron in a tightly focused circular polarized laser pulse
    Yubo Wang(王禹博), Qingyu Yang(杨青屿), Yifan Chang(常一凡), Zongyi Lin(林宗熠), and Youwei Tian(田友伟)
    Chin. Phys. B, 2024, 33 (1): 013301.   DOI: 10.1088/1674-1056/acd921
    Abstract72)   HTML0)    PDF (5925KB)(16)      
    This paper presents a novel view of the impact of electron collision off-axis positions on the dynamic properties and relativistic nonlinear Thomson inverse scattering of excited electrons within tightly focused, circularly polarized laser pulses of varying intensities. We examine the effects of the transverse ponderomotive force, specifically how the deviation angle and speed of electron motion are affected by the initial off-axis position of the electron and the peak amplitude of the laser pulse. When the laser pulse intensity is low, an increase in the electron's initial off-axis distance results in reduced spatial radiation power, improved collimation, super-continuum phenomena generation, red-shifting of the spectrum's harmonic peak, and significant symmetry in the radiation radial direction. However, in contradiction to conventional understandings, when the laser pulse intensity is relatively high, the properties of the relativistic nonlinear Thomson inverse scattering of the electron deviate from the central axis, changing direction in opposition to the aforementioned effects. After reaching a peak, these properties then shift again, aligning with the previous direction. The complex interplay of these effects suggests a greater nuance and intricacy in the relationship between laser pulse intensity, electron position, and scattering properties than previously thought.
    Internal collision double ionization of molecules driven by co-rotating two-color circularly polarized laser pulses
    Xue-Feng Li(李雪峰), Yue Qiao(乔月), Dan Wu(吴丹), Rui-Xian Yu(蔚瑞贤), Ji-Gen Chen(陈基根), Jun Wang(王俊), Fu-Ming Guo(郭福明), and Yu-Jun Yang(杨玉军)
    Chin. Phys. B, 2024, 33 (1): 013302.   DOI: 10.1088/1674-1056/acf5d8
    Abstract90)   HTML0)    PDF (1316KB)(82)      
    The double ionization process of molecules driven by co-rotating two-color circularly polarized fields is investigated with a three-dimensional classical ensemble model. Numerical results indicate that a considerable part of the sequential double ionization (DI) events of molecules occur through internal collision double ionization (ICD), and the ICD recollision mechanism is significantly different from that in non-sequential double ionization (NSDI). By analyzing the results of internuclear distances R=5 a.u. and 2 a.u., these two recollision mechanisms are studied in depth. It is found that the dynamic behaviors of the recollision mechanisms of NSDI and ICD are similar. For NSDI, the motion range of electrons after the ionization is relatively large, and the electrons will return to the core after a period of time. In the ICD process, electrons will rotate around the parent ion before ionization, and the distance of the electron motion is relatively small. After a period of time, the electrons will come back to the core and collide with another electron. Furthermore, the molecular internuclear distance has a significant effect on the electron dynamic behavior of the two ionization mechanisms. This study will help to understand the multi-electron ionization process of complex systems.
    Electron vortices generation of photoelectron of H2+ by counter-rotating circularly polarized attosecond pulses
    Haojing Yang(杨浩婧), Xiaoyu Liu(刘晓煜), Fengzheng Zhu(朱风筝), Liguang Jiao(焦利光), and Aihua Liu(刘爱华)
    Chin. Phys. B, 2024, 33 (1): 013303.   DOI: 10.1088/1674-1056/ad011a
    Abstract103)   HTML0)    PDF (1733KB)(62)      
    Molecular-frame photoelectron momentum distributions (MF-PMDs) of an H2+ molecule ion in the presence of a pair of counter-rotating circularly polarized attosecond extreme ultraviolet laser pulses is studied by numerically solving the two-dimensional time-dependent Schrödinger equation within the frozen-nuclei approximation. At small time delay, our simulations show that the electron vortex structure is sensitive to the time delay and relative phase between the counter-rotating pulses when they are partially overlapped. By adjusting time delay and relative phase, we have the ability to manipulate the MF-PMDs and the appearance of spiral arms. We further show that the internuclear distance can affect the spiral vortices due to its different transition cross sections in the parallel and perpendicular geometries. The lowest-order perturbation theory is employed to interpret these phenomena qualitatively. It is concluded that the internuclear distance-dependent transition cross sections and the confinement effect in diatomic molecules are responsible for the variation of vortex structures in the MF-PMDs.
    Revising the H216O line-shape parameters around 1.1 μm based on the speed-dependent Nelkin-Ghatak profile and the Hartmann-Tran profile
    Hui Zhang(张惠), Jianjie Zheng(郑健捷), Qiang Liu(刘强), Wenyue Zhu(朱文越), Xianmei Qian(钱仙妹), Guisheng Jiang(江贵生), Shenlong Zha(查申龙), Qilei Zhang(张启磊), and Hongliang Ma(马宏亮)
    Chin. Phys. B, 2023, 32 (12): 123301.   DOI: 10.1088/1674-1056/acc7f5
    Abstract92)   HTML0)    PDF (1503KB)(17)      
    Accurate spectroscopic data for H216O in the 1.1 μ m region are particularly important for the study of Earth's atmosphere. The pure water vapor molecular spectra were measured based on direct laser absorption spectroscopy using a narrow line-width external cavity diode laser combined with a high-precision Fabry-Pérot etalon. A total of 31 H216O transitions were studied for the first time by using the speed-dependent Nelkin-Ghatak profile and the Hartmann-Tran profile. From an accurate line-shape analysis, we obtained the line intensities and the self-broadening coefficients, and they are compared with the available data reported in the HITRAN 2016 database and the HITRAN 2020 database. Finally, we obtained information on the influence of Dicke narrowing, as well as the correlations between Dicke narrowing and speed dependence, and of speed-dependent effects.
    Mixed-field effect at the hyperfine level of 127I79Br in its rovibronic ground state: Toward field manipulation of cold molecules
    Zhengbin Bao(包正斌), Defu Wang(王得富), Xuping Shao(邵旭萍),Yunxia Huang(黄云霞), and Xiaohua Yang(杨晓华)
    Chin. Phys. B, 2023, 32 (12): 123302.   DOI: 10.1088/1674-1056/ace61c
    Abstract88)   HTML0)    PDF (901KB)(14)      
    The mixed-field effect at the hyperfine level of the rovibronic ground state of the 127I79Br (X1Σ, v = 0, J = 0) molecule is computed on the J-I uncoupled basis of |JMJI1M1I2M2>, where J is the molecular total angular momentum excluding nuclear spin, MJ is the projection number of J, I1 and I2 are the nuclear spins of the iodine and bromine atoms, and M1 and M2 are the projection numbers of I1 and I2, respectively. When the two applied electric and magnetic fields are parallel, the perturbations are rare and only one perturbation is observed in a relatively large field regime in our computation range. However, when the two fields are off-parallel, the perturbations increase significantly and some sublevels show the Feshbach-like resonance phenomenon. Therefore, such sublevels transit between weak-field seeking and strong-field seeking repeatedly, which can be utilized to enhance or suppress cold molecular collision and chemical reaction rates. Such behavior of the molecular hyperfine structure in the mixed off-parallel fields may also be utilized to construct an electric-field-assisted anti-Helmholtz magnetic trap for cold molecules and to realize evaporative cooling of cold molecules (sub-mK) into the ultracold regime (μK).
    Role of excited states in helium-like ions on high-order harmonic generation
    Jiang-Hua Luo(罗江华) and Jia-Jun Xiao(肖佳俊)
    Chin. Phys. B, 2023, 32 (11): 113201.   DOI: 10.1088/1674-1056/ace317
    Abstract95)   HTML1)    PDF (896KB)(37)      
    We theoretically investigate high-order harmonic generation (HHG) of helium (He), lithium cation (Li+), and beryllium dication (Be2+) using the time-dependent Hartree-Fock method to solve the three-dimensional time-dependent Schrödinger equation. It is found that the intensity of the HHG increases significantly from a certain harmonic order below the ionization threshold, and the initial position of the enhancement does not depend on the intensity or the wavelength of the driving laser field. Further analysis shows that excited states play an important role on this enhancement, consistent with the excited-state tunneling mechanism [Phys. Rev. Lett. 116 123901 (2016)]. Our results unambiguously show that excited-state tunneling is essential for understanding the enhancement of HHG. Accordingly, a four-step model is herein proposed to illustrate the multiphoton excitation effect in helium-like ions, which enriches the physics of HHG enhancement.
    Lifetime measurement of the 3d9 2D3/2 metastable level in Mo15+ at an electron beam ion trap
    Jialin Liu(刘佳林), Yintao Wang(王银涛), Bingsheng Tu(屠秉晟), Liangyu Huang(黄良玉), Ran Si(司然), Jiguang Li(李冀光), Mingwu Zhang(张明武), Yunqing Fu(傅云清), Yaming Zou(邹亚明), and Ke Yao(姚科)
    Chin. Phys. B, 2023, 32 (10): 103201.   DOI: 10.1088/1674-1056/acf121
    Abstract110)   HTML0)    PDF (1052KB)(42)      
    An experimental measurement of the lifetime of $3\rm d^9$ $^2{\rm D}_{3/2}$ metastable level in Mo$^{15+}$ is reported in this work. The Mo$^{15+}$ ions are produced and trapped in an electron beam ion trap with a magnetic field of 0.65 T. The decay photons emitted from $3\rm d^9$ $^2{\rm D}_{3/2}$ level are subsequently recorded via a cooled photomultiplier tube. Through meticulous scrutiny of potential systematic uncertainties affecting the measurement outcomes, we have determined the lifetime of Mo$^{15+}$ $3\rm d^9$ $^2{\rm D}_{3/2}$ metastable level to be 2.83(22) ms. The experimental result provides a clear distinguishment from existing calculations based on various theoretical approaches.
ISSN 1674-1056   CN 11-5639/O4

Current issue

, Vol. 33, No. 4

Previous issues

1992 - present