|
|
|
Electrodynamics of a prototypical altermagnetic compound MnTe |
| Bixia Gao(高碧霞)1,2, Yixuan Luo(罗伊轩)3, Liye Cao(曹立叶)1,2, Tao Sun(孙涛)4, Zehao Yu(于泽浩)1,2, Lei Wang(王蕾)1,2, Xinyu Zhang(张新雨)1,2, Hongbo Hu(胡宏波)1,2, Yanfeng Guo(郭艳峰)3,5, and Rongyan Chen(陈荣艳)1,2,† |
1 Center for Advanced Quantum Studies, School of Physics and Astronomy, Beijing Normal University, Beijing 100875, China; 2 Key Laboratory of Multiscale Spin Physics, Ministry of Education, Beijing Normal University, Beijing 100875, China; 3 State Key Laboratory of Quantum Functional Materials, School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China; 4 Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China; 5 ShanghaiTech Laboratory for Topological Physics, ShanghaiTech University, Shanghai 201210, China |
|
|
|
|
Abstract Altermagnetism, characterized by compensated antiparallel spins and momentum-dependent spin splitting, has offered a promising platform for novel spintronic phenomena. Among this class of materials, hexagonal MnTe stands out due to its high Néel temperature and giant spin splitting. However, a comprehensive understanding of its charge dynamics remains incomplete. Here, we employ infrared spectroscopy to investigate the charge dynamics of single crystalline MnTe. The low energy optical conductivity reveals a suppressed Drude response across all temperatures, consistent with the reported p-type doping as indicated by previous angle-resolved photoemission spectroscopy (ARPES) measurement. An indirect band gap of about 0.48 eV attributed to impurity-assisted transitions, and a direct gap of 1.60 eV are identified via the Tauc relation at 10 K. Moreover, we observe a subtle difference at around 1.44 eV in the optical conductivity between the antiferromagnetic and paramagnetic states, which might be linked to altermagnetism-related band splitting. Additionally, Fano line shape analysis of a phonon mode at around 135 cm$^{-1}$ reveals appreciable coupling between the phonon and spin fluctuations near the Néel temperature. Our results provide key insights into the charge dynamics of MnTe, underscoring its rich physics beyond a conventional semiconductor.
|
Received: 01 September 2025
Revised: 05 December 2025
Accepted manuscript online: 10 December 2025
|
|
PACS:
|
78.30.-j
|
(Infrared and Raman spectra)
|
| |
78.40.Fy
|
(Semiconductors)
|
| |
63.20.-e
|
(Phonons in crystal lattices)
|
| |
75.50.Ee
|
(Antiferromagnetics)
|
|
| Fund: R.Y.C. acknowledges the support by the National Key Research and Development Program of China (Grant Nos. 2021YFA1400400 and 2023YFA1406100), the National Natural Science Foundation of China (Grant No. 12074042), the Young Scientists Fund of the National Natural Science Foundation of China (Grant No. 11704033), and the Fundamental Research Funds for the Central Universities (Grant No. 2243300003). Y.F.G. acknowledges the open research fund of Beijing National Laboratory for Condensed Matter Physics (Grant No. 2023BNLCMPKF002). This work was supported by the Synergetic Extreme Condition User Facility (SECUF). |
Corresponding Authors:
Rongyan Chen
E-mail: rychen@bnu.edu.cn
|
Cite this article:
Bixia Gao(高碧霞), Yixuan Luo(罗伊轩), Liye Cao(曹立叶), Tao Sun(孙涛), Zehao Yu(于泽浩), Lei Wang(王蕾), Xinyu Zhang(张新雨), Hongbo Hu(胡宏波), Yanfeng Guo(郭艳峰), and Rongyan Chen(陈荣艳) Electrodynamics of a prototypical altermagnetic compound MnTe 2026 Chin. Phys. B 35 037801
|
[1] Šmejkal L, Sinova J and Jungwirth T 2022 Phys. Rev. X 12 040501 [2] Šmejkal L, Sinova J and Jungwirth T 2022 Phys. Rev. X 12 031042 [3] Mazin I 2022 Phys. Rev. X 12 040002 [4] Mazin I 2023 Phys. Rev. B 107 L100418 [5] Radaelli P G 2024 Phys. Rev. B 110 214428 [6] McClarty P A and Rau J G 2024 Phys. Rev. Lett. 132 176702 [7] Smolyanyuk A, Šmejkal L and Mazin I I 2025 Phys. Rev. B 111 064406 [8] Parfenov O E, Averyanov D V, Sokolov I S, Mihalyuk A N, Kondratev O A, Taldenkov A N, Tokmachev A M and Storchak V G 2025 J. Am. Chem. Soc. 147 5911 [9] Squire C F 1939 Phys. Rev. 56 922 [10] Grazhdankina N and Gurfel D 1959 Sov. Phys. J. 35 907 [11] Komatsubara T, Murakami M and Hirahara E 1963 J. Phys. Soc. Jpn. 18 356 [12] Szuszkiewicz W, Hennion B, Witkowska B, Łusakowska E and Mycielski A 2005 Phys. Status Solidi 2 1141 [13] Krause M and Bechstedt F 2013 J. Supercond. Novel Magn. 26 1963 [14] Wang P, Zhu S C, Zou Y T, Chen H Y, Liu Y, Li W W, Chen J, Zhu J L, Wu L S, Wang S M, Yang W G, Xiao Y M, Chow P, Wang L P and Zhao Y S 2022 Chem. Mater. 34 3931 [15] Chilcote M, Mazza A R, Lu Q, Gray I, Tian Q, Deng Q, Moseley D, Chen A H, Lapano J, Gardner J S, Eres G, Ward T Z, Feng E, Cao H, Lauter V, McGuire M A, Hermann R, Parker D, Han M G, Kayani A, Rimal G, Wu L, Charlton T R, Moore R G and Brahlek M 2024 Adv. Funct. Mater. 34 2405829 [16] Lee S, Lee S, Jung S, Jung J, Kim D, Lee Y, Seok B, Kim J, Park B G, Šmejkal L, Kang C J and Kim C 2024 Phys. Rev. Lett. 132 036702 [17] Kriegner D, Reichlova H, Grenzer J, Schmidt W, Ressouche E, Godinho J,Wagner T, Martin S Y, Shick A B, Volobuev V V, Springholz G, Holý V, Wunderlich J, Jungwirth T and Výborný K 2017 Phys. Rev. B 96 214418 [18] Gonzalez Betancourt R D, Zubáč J, Gonzalez-Hernandez R, Geishendorf K, Šobáň Z, Springholz G, Olejník K, Šmejkal L, Sinova J, Jungwirth T, Goennenwein S T B, Thomas A, Reichlová H, Železný J and Kriegner D 2023 Phys. Rev. Lett. 130 036702 [19] Zanmarchi G 1967 J. Phys. Chem. Solids 28 2123 [20] Allen J, Lucovsky G and Mikkelsen J 1977 Solid State Commun. 24 367 [21] Sandratskii L M, Egorov R F and Berdyshev A A 1981 Phys. Status Solidi B 104 103 [22] Podgòrny M and Oleszkiewicz J 1983 J. Phys. C: Solid State Phys. 16 2547 [23] Wei S H and Zunger A 1987 Phys. Rev. B 35 2340 [24] Oleszkiewicz J, Kisiel A and Ignatowicz S 1988 Thin Solid Films 157 1 [25] Angadi M and Thanigaimani V 1994 1994 Phys. Status Solidi A 143 K119 [26] Sato H, Mihara T, Furuta A, Tamura M, Mimura K, Happo N, Taniguchi M and Ueda Y 1997 Phys. Rev. B 56 7222 [27] Ferrer-Roca C, Segura A, Reig C and Muñoz V 2000 Phys. Rev. B 61 13679 [28] Reig C, Muñoz V, Gómez C, Ferrer C and Segura A 2001 J. Cryst. Growth 223 349 [29] Tanner D B 2015 Phys. Rev. B 91 035123 [30] Kluczyk K P, Gas K, Grzybowski M J, Skupiński P, Borysiewicz M A, Fas T, Suffczyński J, Domagala J Z, Grasza K, Mycielski A, Baj M, Ahn K H, Výborný K, Sawicki M and Gryglas-Borysiewicz M 2024 Phys. Rev. B 110 155201 [31] Huang H, Qu T, Cheng Y, Tai L, Eckberg C, Pan Q, Alrasheed A, Chong S K, Dai B, Li Y, Shu Q, Yang C Y, Yu J X, Yin G and Wang K L 2024 (Preprint 2405.04686) [32] Pereverzev Y V, Povstyanyi L V and Zvyagin A I 1976 Sov. J. Low Temp. Phys. 2 311 [33] Efrem D’Sa J, Bhobe P, Priolkar K, Das A, Paranjpe S, Prabhu R and Sarode P 2005 J. Magn. Magn. Mater. 285 267 [34] Chen Z G, Yuan R H, Dong T, Xu G, Shi Y G, Zheng P, Luo J L, Guo J G, Chen X L and Wang N L 2011 Phys. Rev. B 83 220507 [35] Homes C C, Wang Z C, Fruhling K and Tafti F 2023 Phys. Rev. B 107 045106 [36] Homes C, McConnell A, Clayman B, Bonn D, Liang R, Hardy W, Inoue M, Negishi H, Fournier P and Greene R 2000 Phys. Rev. Lett. 84 5391 [37] Osumi T, Souma S, Aoyama T, Yamauchi K, Honma A, Nakayama K, Takahashi T, Ohgushi K and Sato T 2024 Phys. Rev. B 109 115102 [38] Tauc J, Grigorovici R and Vancu A 1966 Phys. Status Solidi B 15 627 [39] Okamura H, Michizawa T, Nanba T, Kimura S, Iga F and Takabatake T 2005 J. Phys. Soc. Jpn. 74 1954 [40] Zhang J M, Lian R, Yang Y, Xu G, Zhong K and Huang Z 2017 Sci. Rep. 7 43626 [41] Fano U 1961 Phys. Rev. 124 1866 [42] Wenzel M, Ortiz B R, Wilson S D, Dressel M, Tsirlin A A and Uykur E 2022 Phys. Rev. B 105 245123 |
| No Suggested Reading articles found! |
|
|
Viewed |
|
|
|
Full text
|
|
|
|
|
Abstract
|
|
|
|
|
Cited |
|
|
|
|
Altmetric
|
|
blogs
Facebook pages
Wikipedia page
Google+ users
|
Online attention
Altmetric calculates a score based on the online attention an article receives. Each coloured thread in the circle represents a different type of online attention. The number in the centre is the Altmetric score. Social media and mainstream news media are the main sources that calculate the score. Reference managers such as Mendeley are also tracked but do not contribute to the score. Older articles often score higher because they have had more time to get noticed. To account for this, Altmetric has included the context data for other articles of a similar age.
View more on Altmetrics
|
|
|