Measurement of CO, HCN, and NO productions in atmospheric reaction induced by femtosecond laser filament

doi:10.1088/1674-1056/ac6b28

Abstract It is proved that the chemical reaction induced by femtosecond laser filament in the atmosphere produces CO, HCN, and NO, and the production CO and HCN are observed for the first time. The concentrations of the products are measured by mid-infrared tunable laser absorption spectroscopy. In the reduced pressure air, the decomposition of CO₂ is enhanced by vibration excitation induced by laser filament, resulting in the enhanced production of CO and HCN. At the same time, the CO and HCN generated from the atmosphere suffer rotation excitation induced by laser filament, enhancing their absorption spectra. It is found that NO, CO, and HCN accumulate to 134 ppm, 80 ppm, and 1.6 ppm in sealed air after sufficient reaction time. The atmospheric chemical reaction induced by laser filament opens the way to changing the air composition while maintaining environmental benefits.

Keywords: femtosecond laser filament atmospheric reaction CO HCN NO

Received: 07 March 2022
Revised: 21 April 2022
Accepted manuscript online: 28 April 2022

PACS:	78.47.-p	(Spectroscopy of solid state dynamics)
	82.53.-k	(Femtochemistry)
	78.30.-j	(Infrared and Raman spectra)
	82.33.Tb	(Atmospheric chemistry)

Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 1625501 and 62027822) and the Research Funds of Happiness Flower ECNU, China (Grant No. 2021ST2110).

Corresponding Authors: Lun-Hua Deng, Huai-Liang Xu
E-mail: lhdeng@phy.ecnu.edu.cn;huailiang@jlu.edu.cn

Cite this article:

Xiao-Dong Huang(黄晓东), Meng Zhang(张梦), Lun-Hua Deng(邓伦华), Shan-Biao Pang(庞山彪), Ke Liu(刘珂), and Huai-Liang Xu(徐淮良) Measurement of CO, HCN, and NO productions in atmospheric reaction induced by femtosecond laser filament 2022 Chin. Phys. B 31 097801

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Measurement of CO, HCN, and NO productions in atmospheric reaction induced by femtosecond laser filament

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