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Incommensurate-commensurate magnetic phase transition in double tungstate Li2Co(WO4)2 |
| Xiyu Chen(陈西煜)1, Ning Ding(丁宁)2, Meifeng Liu(刘美风)1,†, Tao Zou(邹涛)3,‡, V. Ovidiu Garlea4, Jingwen Gong(龚婧雯)1, Fei Liu(刘飞)1, Yunlong Xie(谢云龙)1, Lun Yang(杨伦)1, Shuhan Zheng(郑书翰)1, Xiuzhang Wang(王秀章)1, Shuai Dong(董帅)2,§, T. Charlton4, and Jun-Ming Liu(刘俊明)1,5 |
1 Institute for Advanced Materials, Hubei Normal University, Huangshi 435002, China;
2 School of Physics, Southeast University, Nanjing 211189, China;
3 Collaborative Innovation Center of Light Manipulations and Applications, Shangdong Normal University, Jinan 250358, China;
4 Neutron Scattering División, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA;
5 Laboratory of Solid State Microstructures and Innovative Center of Advanced Microstructures, Nanjing University, Nanjing 210093, China |
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Abstract Magnetic susceptibility, specific heat, and neutron powder diffraction measurements have been performed on polycrystalline Li$_{2}$Co(WO$_{4}$)$_{2}$ samples. Under zero magnetic field, two successive magnetic transitions at $T_{\rm N1}\sim 9.4$ K and $T_{\rm N2}\sim 7.4$ K are observed. The magnetic ordering temperatures gradually decrease as the magnetic field increases. Neutron diffraction reveals that Li$_{2}$Co(WO$_{4}$)$_{2}$ enters an incommensurate magnetic state with a temperature dependent $\bm k$ between $T_{\rm N1}$ and $T_{\rm N2}$. The magnetic propagation vector locks-in to a commensurate value $\bm k = (1/2, 1/4, 1/4)$ below $T_{\rm N2}$. The antiferromagnetic structure is refined at 1.7 K with Co$^{2+}$ magnetic moment 2.8(1) $\mu_{\rm B}$, consistent with our first-principles calculations.
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Received: 01 November 2021
Revised: 08 November 2021
Accepted manuscript online: 10 November 2021
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PACS:
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75.25.-j
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(Spin arrangements in magnetically ordered materials (including neutron And spin-polarized electron studies, synchrotron-source x-ray scattering, etc.))
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75.50.Ee
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(Antiferromagnetics)
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75.47.Lx
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(Magnetic oxides)
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| Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 11834002, 12074111, and 11704109) and the National Key R&D Project of China (Grant No. 2016YFA0300101). |
Corresponding Authors:
Meifeng Liu, Tao Zou, Shuai Dong
E-mail: lmfeng1107@hbnu.edu.cn;taozoucn@gmail.com;sdong@seu.edu.cn
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Cite this article:
Xiyu Chen(陈西煜), Ning Ding(丁宁), Meifeng Liu(刘美风), Tao Zou(邹涛), V. Ovidiu Garlea, Jingwen Gong(龚婧雯), Fei Liu(刘飞), Yunlong Xie(谢云龙), Lun Yang(杨伦), Shuhan Zheng(郑书翰), Xiuzhang Wang(王秀章), Shuai Dong(董帅), T. Charlton, and Jun-Ming Liu(刘俊明) Incommensurate-commensurate magnetic phase transition in double tungstate Li2Co(WO4)2 2022 Chin. Phys. B 31 047501
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