|
|
|
Geometric structure of N2Oq+ (q = 5, 6) studied by Ne8+ ion-induced Coulomb explosion imaging |
| Xi Zhao(赵曦)1, Xu Shan(单旭)1,†, Xiaolong Zhu(朱小龙)2, Lei Chen(陈磊)1, Zhenjie Shen(沈镇捷)1, Wentian Feng(冯文天)2, Dalong Guo(郭大龙)2, Dongmei Zhao(赵冬梅)2, Ruitian Zhang(张瑞田)2, Yong Gao(高永)2, Zhongkui Huang(黄忠魁)2, Shaofeng Zhang(张少锋)2, Xinwen Ma(马新文)2,‡, and Xiangjun Chen(陈向军)1 |
1 Hefei National Laboratory for Physical Sciences at the Microscale and Department of Modern Physics, University of Science and Technology of China, Hefei 230026, China;
2 Institute of Modern Physics, Chinese Academy of Sciences, Lanzhou 730000, China |
|
|
|
|
Abstract We report the study on the complete three-body Coulomb explosion (CE) of N2Oq+ (q = 5, 6) induced by 56-keV/u Ne8+ ion collision with N2O gaseous molecule. Six CE channels for N2O5+ and seven for N2O6+ are identified by measuring three ionic fragments and the charge-changed projectile in quadruple coincidence. Correspondingly the kinetic energy release (KER) and momentum correlation angle (MCA) distributions of three ionic fragments for each of the CE channels are also deduced. Numerical computation is presented to reconstruct the geometric structure of N2Oq+ prior to dissociation based on the measured KER and MCA. The N-N and N-O bond lengths and the N-N-O bond angles of N2Oq+ for each of the channels are determined.
|
Received: 31 March 2021
Revised: 30 April 2021
Accepted manuscript online: 10 May 2021
|
|
PACS:
|
34.50.Gb
|
(Electronic excitation and ionization of molecules)
|
| |
34.80.Ht
|
(Dissociation and dissociative attachment)
|
|
| Fund: Project supported by the National Key Research and Development Program of China (Grant Nos. 2017YFA0402300 and 2017YFA0303501) and the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB34000000). The authors thank the staff of the 320-kV platform for multidisciplinary research with highly charged ions at the Institute of Modern Physics, Chinese Academy of Sciences, for their technical support. |
Corresponding Authors:
Xu Shan, Xinwen Ma
E-mail: xshan@ustc.edu.cn;x.ma@impcas.ac.cn
|
Cite this article:
Xi Zhao(赵曦), Xu Shan(单旭), Xiaolong Zhu(朱小龙), Lei Chen(陈磊), Zhenjie Shen(沈镇捷), Wentian Feng(冯文天), Dalong Guo(郭大龙), Dongmei Zhao(赵冬梅), Ruitian Zhang(张瑞田), Yong Gao(高永), Zhongkui Huang(黄忠魁), Shaofeng Zhang(张少锋), Xinwen Ma(马新文), and Xiangjun Chen(陈向军) Geometric structure of N2Oq+ (q = 5, 6) studied by Ne8+ ion-induced Coulomb explosion imaging 2021 Chin. Phys. B 30 113302
|
[1] Vager Z, Kanter E P, Both G, Cooney P J, Faibis A, Koenig W, Zabransky B J and Zajfman D 1986 Phys. Rev. Lett. 57 2793
[2] Vager Z, Naaman R and Kanter E P 1989 Science 244 426
[3] Dörner R, Mergel V, Jagutzki O, Spielberger L, Ullrich J, Moshammer R and Schmidt-Böcking H 2000 Phys. Rep. 330 95
[4] Ullrich J, Moshammer R, Dorn A, Dörner R, Schmidt L P H and Schmidt-Böcking H 2003 Rep. Prog. Phys. 66 1463
[5] Baldit E, Saugout S and Cornaggia C 2005 Phys. Rev. A 71 021403
[6] Wu C, Yang Y, Wu Z, Chen B, Dong H, Liu X, Deng Y, Liu H, Liu Y and Gong Q 2011 Phys. Chem. Chem. Phys. 13 18398
[7] Legare F, Lee K F, Litvinyuk I V, Dooley P W, Bandrauk A D, Villeneuve D M and Corkum P B 2005 Phys. Rev. A 72 052717
[8] Hishikawa A, Iwamae A, Hoshina K, Kono M and Yamanouchi K 1998 Res. Chem. Intermed. 24 765
[9] Ueyama M, Hasegawa H, Hishikawa A and Yamanouchi K 2005 J. Chem. Phys. 123 154305
[10] Karimi R, Bisson É, Wales B, Beaulieu S, Giguére M, Long Z J, Liu W K, Kieffer J C, Légaré F and Sanderson J 2013 J. Chem. Phys. 138 204311
[11] Hishikawa A, Iwamae A and Yamanouchi K 1999 Phys. Rev. Lett. 83 1127
[12] Bocharova I, Karimi R, Penka E F, Brichta J P, Lassonde P, Fu X, Kieffer J C, Bandrauk A D, Litvinyuk I, Sanderson J and Leǵare F 2011 Phys. Rev. Lett. 107 063201
[13] Wu C, Wu C, Song D, Su H, Yang Y, Wu Z, Liu X, Liu H, Li M, Deng Y, Liu Y, Peng L Y, Jiang H and Gong Q 2013 Phys. Rev. Lett. 110 103601
[14] Wu C, Wu C, Fan Y, Xie X, Wang P, Deng Y, Liu Y and Gong Q 2015 J. Chem. Phys. 142 124303
[15] Wang E L, Shan X, Shen Z J, Li X Y, Gong M M, Tang Y G and Chen X J 2015 Phys. Rev. A 92 062713
[16] Wang E L, Shan X, Shen Z J, Gong M M, Tang Y G, Pan Y, Lau K C and Chen X J 2015 Phys. Rev. A 91 052711
[17] Siegmann B, Werner U, Lutz H O and Mann R 2002 J. Phys. B: At. Mol. Opt. Phys. 35 3755
[18] Rajgara F A, Krishnamurthy M and Mathur D 2001 Phys. Rev. A 64 032712
[19] Wang B, Han J, Zhu X L, Wei L, Ren B H, Zhang Y, Yu W D, Yan S C, Ma X W, Zou Y M, Chen L, and Wei B R 2021 Phys. Rev. A 103 042810
[20] Pitzer M, Kunitski M, Johnson A S, Jahnke T, Sann H, Sturm F, Schmidt L Ph H, Schmidt-Böcking H, Dörner R, Stohner J, Kiedrowski J, Reggelin M, Marquardt S, Schieöer A, Berger R and Schöffler M S 2013 Science 341 1096
[21] Herwig P, Zawatzky K, Grieser M, Heber O, Jordon-Thaden B, Krantz C, Novotny O, Repnow R, Schurig, Schwalm V D, Vager Z, Wolf A, Trapp O and Kreckel H 2013 Science 342 1084
[22] Ulrich B, Vredenborg A, Malakzadeh A, Schmidt L Ph H, Havermeier T, Meckel M, Cole K, Smolarski M, Chang Z, Jahnke T and Dörner R 2011 J. Phys. Chem. A 115 6936
[23] Wu J, Kuniski M, Schmidt L Ph H, Jahnke T and Dörner R 2012 J. Chem. Phys. 137 104308
[24] Wu C, Wu C, Song D, Su H, Xie X, Li M, Deng Y, Liu Y and Gong Q 2014 J. Chem. Phys. 140 141101
[25] Zhu X L, Yan S, Feng W T, Guo D L, Gao Y, Zhang R T, Zhang S F, Wang H B, Huang Z K, Zhang M, Hai B, Zhao D M, Wen W Q, Zhang P, Qian D B and Ma X 2017 Nucl. Instr. Meth. B 408 42
[26] Chen L, Shan X, Zhao X, Zhu X L, Hu X Q, Wu Y, Feng W T, Guo D L, Zhang R T, Gao Y, Huang Z K, Wang J G, Ma X and Chen X J 2019 Phys. Rev. A 99 012710
[27] Zhao X, Shan X, Zhu X L, Chen L, Shen Z J, Feng W T, Guo D L, Zhao D M, Zhang R T, Gao Y, Huang Z K, Zhang S F, Ma X and Chen X J 2021 Phys. Rev. A 103 012802
[28] Wang D, Guo G, Min G and Zhang X 2017 Phys. Rev. A 95 012705
[29] Werner U, Siegmann B and Mann R 2007 Scientific Report 2006 (GSI Report 2007-1) p. 253
[30] Khan A, Tribedi L C and Misra D 2017 Phys. Rev. A 96 012703
[31] Frasinski L J, Hatherly P A and Codling K 1991 Phys. Lett. A 156 227
[32] Khan A and Misra D 2016 J. Phys. B At. Mol. Opt. Phys. 49 055201
[33] Bhatt P, Singh R, Yadav N and Shanker R 2012 Phys. Rev. A 86 052708
[34] Love N A and Price S D 2004 Phys. Chem. Chem. Phys. 6 4558
[35] Eland J H D and Murphy V J 1991 Rapid Commun. Mass Spectrom. 5 221
[36] Alagia M, Candori P, Falcinelli S, Lavollée M, Pirani F, Richter R, Strangesand S and Vecchiocattivi F 2006 Chem. Phy. Lett. 432 398
[37] Price S D, Eland J H D, Fournier P G, Fournier J and Millie P 1988 J. Chem. Phys. 88 1511
[38] Taylor S, Eland J H D and Hochlaf M 2006 J. Chem. Phys. 124 204319
[39] Curtis D M and Eland J H D 1985 Int. J. Mass Spectrom. Ion Process. 63 241
[40] Zhou X, Ranitovic P, Hogle C W, Eland J H D, Kapteyn H C and Murnane M M 2012 Nat. Phys. 8 232
[41] Kübel M, Alnaser A S, Bergues B, Pischke T, Schmidt J, Deng Y, Jendrzejewski C, Ullrich J, Paulus G G, Azzeer A M, Kleineberg U, Moshammer R and Kling M F 2014 New J. Phys. 16 065017
[42] Levasseur N and Millié P 1990 J. Chem. Phys. 92 2974
[43] Zhang M, Najjari B, Hai B, Zhao D M, Lei J T, Dong D P, Zhang S F and Ma X W 2020 Chin. Phys. B 29 063302
[44] Ma X, Zhu X, Liu H, Li B, Zhang S, Cao S, Feng W and Xu S 2008 Sci. China Ser. G: Phys. Mech. Astron. 51 755
[45] Ma X, Zhang R T, Zhang S F, Zhu X L, Feng W T, Guo D L, Li B, Liu H P, Li C Y, Wang J G, Yan S C, Zhang P J and Wang Q 2011 Phys. Rev. A 83 052707
[46] Wiley W C and McLaren I H 1955 Rev. Sci. Instrum. 26 1150
[47] Harmony M D, Laurie V W, Kuczkowski R L, Schwendeman R H, Ramsay D A, Lovas F J, Lafferty W J and Maki A G 1979 J. Phys. Chem. Ref. Data 8 619 |
| No Suggested Reading articles found! |
|
|
Viewed |
|
|
|
Full text
|
|
|
|
|
Abstract
|
|
|
|
|
Cited |
|
|
|
|
Altmetric
|
|
blogs
Facebook pages
Wikipedia page
Google+ users
|
Online attention
Altmetric calculates a score based on the online attention an article receives. Each coloured thread in the circle represents a different type of online attention. The number in the centre is the Altmetric score. Social media and mainstream news media are the main sources that calculate the score. Reference managers such as Mendeley are also tracked but do not contribute to the score. Older articles often score higher because they have had more time to get noticed. To account for this, Altmetric has included the context data for other articles of a similar age.
View more on Altmetrics
|
|
|
