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Chin. Phys. B, 2016, Vol. 25(1): 018211    DOI: 10.1088/1674-1056/25/1/018211
Special Issue: TOPICAL REVIEW — Fundamental physics research in lithium batteries
TOPICAL REVIEW—Fundamental physics research in lithium batteries Prev   Next  

Lithium-ion transport in inorganic solid state electrolyte

Jian Gao(高健)1,2, Yu-Sheng Zhao(赵予生)3, Si-Qi Shi(施思齐)4,2, Hong Li(李泓)1
1. Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China;
2. Materials Genome Institute, Shanghai University, Shanghai 200444, China;
3. Department of Physics and Astronomy and High Pressure Science and Engineering Center, University of Nevada, Las Vegas, Nevada 89154, USA;
4. School of Materials Science and Engineering, Shanghai University, Shanghai 200444, China
Abstract  

An overview of ion transport in lithium-ion inorganic solid state electrolytes is presented, aimed at exploring and designing better electrolyte materials. Ionic conductivity is one of the most important indices of the performance of inorganic solid state electrolytes. The general definition of solid state electrolytes is presented in terms of their role in a working cell (to convey ions while isolate electrons), and the history of solid electrolyte development is briefly summarized. Ways of using the available theoretical models and experimental methods to characterize lithium-ion transport in solid state electrolytes are systematically introduced. Then the various factors that affect ionic conductivity are itemized, including mainly structural disorder, composite materials and interface effects between a solid electrolyte and an electrode. Finally, strategies for future material systems, for synthesis and characterization methods, and for theory and calculation are proposed, aiming to help accelerate the design and development of new solid electrolytes.

Keywords:  lithium-ion batteries      solid state electrolyte      ionic conductivity      ion transport mechanism  
Received:  18 May 2015      Revised:  22 July 2015      Accepted manuscript online: 
PACS:  82.47.Aa (Lithium-ion batteries)  
  65.40.gk (Electrochemical properties)  
Fund: 

Project supported by the National Natural Science Foundation of China (Grant No. 51372228), the Shanghai Pujiang Program, China (Grant No. 14PJ1403900), and the Shanghai Institute of Materials Genome from the Shanghai Municipal Science and Technology Commission, China (Grant No. 14DZ2261200).

Corresponding Authors:  Si-Qi Shi, Hong Li     E-mail:  sqshi@shu.edu.cn;hli@aphy.iphy.ac.cn

Cite this article: 

Jian Gao(高健), Yu-Sheng Zhao(赵予生), Si-Qi Shi(施思齐), Hong Li(李泓) Lithium-ion transport in inorganic solid state electrolyte 2016 Chin. Phys. B 25 018211

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