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Chin. Phys. B, 2023, Vol. 32(1): 018507    DOI: 10.1088/1674-1056/aca7e8
Special Issue: SPECIAL TOPIC — Physics in micro-LED and quantum dots devices
TOPICAL REVIEW—Physics in micro-LED and quantum dots devices Prev   Next  

Ion migration in metal halide perovskite QLEDs and its inhibition

Yuhui Dong(董宇辉)1,2, Danni Yan(严丹妮)1,2, Shuai Yang(杨帅)1,2, Naiwei Wei(魏乃炜)1,2, Yousheng Zou(邹友生)1,2,†, and Haibo Zeng(曾海波)1,2‡
1 Institute of Optoelectronics&Nanomaterials, College of Materials Science and Engineering, Nanjing University of Science and Technology, Nanjing 210094, China;
2 Key Laboratory of Advanced Display Materials and Devices, Ministry of Industry and Information Technology, Nanjing 210094, China
Abstract  Benefiting from the excellent properties such as high photoluminescence quantum yield (PLQY), wide gamut range, and narrow emission linewidth, as well as low-temperature processability, metal halide perovskite quantum dots (QDs) have attracted wide attention from researchers. Despite tremendous progress has been made during the past several years, the commercialization of perovskite QDs-based LEDs (PeQLEDs) is still plagued by the instability. The ion migration in halide perovskites is recognized as the key factor causing the performance degradation of PeQLEDs. In this review, the elements species of ion migration, the effects of ion migration on device performance and stability, and effective strategies to hinder/mitigate ion migration in PeQLEDs are successively discussed. Finally, the forward insights on the future research are highlighted.
Keywords:  perovskite quantum dots      light-emitting diodes      ion migration      stability  
Received:  31 August 2022      Revised:  16 November 2022      Accepted manuscript online:  02 December 2022
PACS:  85.60.Jb (Light-emitting devices)  
  61.82.Rx (Nanocrystalline materials)  
  31.30.J- (Relativistic and quantum electrodynamic (QED) effects in atoms, molecules, and ions)  
  42.60.Lh (Efficiency, stability, gain, and other operational parameters)  
Fund: This work was supported by the Natural Natural Science Foundation of China (Grant Nos. 61904081 and 51672132), the Natural Science Foundation of Jiangsu Province, China (Grant No. BK20190449), and the Postdoctoral Research Funding Program of Jiangsu Province, China (Grant No. 2020Z144).
Corresponding Authors:  Yousheng Zou, Haibo Zeng     E-mail:  yshzou75@njust.edu.cn;zeng.haibo@njust.edu.cn

Cite this article: 

Yuhui Dong(董宇辉), Danni Yan(严丹妮), Shuai Yang(杨帅), Naiwei Wei(魏乃炜),Yousheng Zou(邹友生), and Haibo Zeng(曾海波) Ion migration in metal halide perovskite QLEDs and its inhibition 2023 Chin. Phys. B 32 018507

[1] Ren X, Zhang X, Xie H, Cai J, Wang C, Chen E, Xu S, Ye Y, Sun J, Yan Q and Guo T 2022 Nanomaterials 12 2243
[2] Li J, Xu L, Wang T, Song J, Chen J, Xue J, Dong Y, Cai B, Shan Q, Han B and Zeng H 2017 Adv. Mater. 29 1603885
[3] Pan J, Shang Y, Yin J, De Bastiani M, Peng W, Dursun I, Sinatra L, El-Zohry A M, Hedhili M N, Emwas A H, Mohammed O F, Ning Z and Bakr O M 2018 J. Am. Chem. Soc. 140 562
[4] Nenon D P, Pressler K, Kang J, Koscher B A, Olshansky J H, Osowiecki W T, Koc M A, Wang L W and Alivisatos A P 2018 J. Am. Chem. Soc. 140 17760
[5] Fang T, Wang T, Li X, Dong Y, Bai S and Song J 2021 Sci. Bull. 66 36
[6] De Roo J, Ibanez M, Geiregat P, Nedelcu G, Walravens W, Maes J, Martins J C, Van Driessche I, Kovalenko M V and Hens Z 2016 ACS Nano 10 2071
[7] Chen K, Jin W, Zhang Y, Yang T, Reiss P, Zhong Q, Bach U, Li Q, Wang Y, Zhang H, Bao Q and Liu Y 2020 J. Am. Chem. Soc. 142 3775
[8] Chen J, Jia D, Johansson E M J, Hagfeldt A and Zhang X 2021 Energy Environ. Sci. 14 224
[9] Wang Y, Li X, Zhao X, Xiao L, Zeng H and Sun H 2016 Nano Lett. 16 448
[10] Huang C Y, Zou C, Mao C, Corp K L, Yao Y C, Lee Y J, Schlenker C W, Jen A K Y and Lin L Y 2017 ACS Photonics 4 2281
[11] Song J, Li J, Li X, Xu L, Dong Y and Zeng H 2015 Adv. Mater. 27 7162
[12] Wang H C, Wang W, Tang A C, Tsai H Y, Bao Z, Ihara T, Yarita N, Tahara H, Kanemitsu Y, Chen S and Liu R S 2017 Angew. Chem. Int. Ed. 56 13650
[13] Zhang B B, Yuan S, Ma J P, Zhou Y, Hou J, Chen X, Zheng W, Shen H, Wang X C, Sun B, Bakr O M, Liao L S and Sun H T 2019 J. Am. Chem. Soc. 141 15423
[14] Dong Y, Tang X, Zhang Z, Song J, Niu T, Shan D and Zeng H 2020 Matter 3 273
[15] Yang Z, Dong Y, Zong S, Li L, Yang K, Wang Z, Zeng H and Cui Y 2022 Nanoscale 14 6392
[16] Mei X, Jia D, Chen J, Zheng S and Zhang X 2022 Nano Today 43 101449
[17] Dong Y, Wang Y K and Yuan F 2020 Nat. Nanotechnol. 15 668
[18] Kim Y H, Kim S and Kakekhani A 2021 Nat. Photon. 15 148
[19] Wang Y K, Yuan F and Dong Y 2021 Angew. Chem. Int. Ed. 60 16164
[20] Shen Y, Li Y Q, Zhang K, Zhang L J, Xie F M, Chen L, Cai X Y, Lu Y, Ren H, Gao X, Xie H, Mao H, Kera S and Tang J X 2022 Adv. Funct. Mater. 32 2206574
[21] Liu Z, Qiu W, Peng X, Sun G, Liu X, Liu D, Li Z, He F, Shen C, Gu Q, Ma F, Yip H L, Hou L, Qi Z and Su S J 2021 Adv. Mater. 33 e2103268
[22] Ye F, Shan Q, Zeng H and Choy W 2021 ACS Energy Lett. 6 3114
[23] Liu Y, Dong Y and Zhu T 2021 J. Am. Chem. Soc. 143 15606
[24] Guo B, Lai R, Jiang S, Zhou L, Ren Z, Lian Y, Li P, Cao X, Xing S, Wang Y, Li W, Zou C, Chen M, Hong Z, Li C, Zhao B and Di D 2022 Nat. Photon. 16 637
[25] Won Y H, Cho O, Kim T, Chung D Y, Kim T, Chung H, Jang H, Lee J, Kim D and Jang E 2019 Nature 575 634
[26] Li N, Jia Y, Guo Y and Zhao N 2022 Adv. Mater. 34 e2108102
[27] Dong Q, Mendes J, Lei L, Seyitliyev D, Zhu L, He S, Gundogdu K and So F 2020 ACS Appl. Mater. Interfaces 12 48845
[28] Xing G, Wu B, Wu X, Li M, Du B, Wei Q, Guo J, Yeow E K, Sum T C and Huang W 2017 Nat. Commun. 8 14558
[29] Yuan Y and Huang J 2016 Acc. Chem. Res. 49 286
[30] Dong Q, Lei L, Mendes J and So F 2020 J. Phys.: Mater. 3 012002
[31] Wang H C, Bao Z, Tsai H Y, Tang A C and Liu R S 2018 Small 14 1702433
[32] Xie M and Tian J 2022 J. Phys. Chem. Lett. 13 1962
[33] Eames C, Frost J M, Barnes P R, O'Regan B C, Walsh A and Islam M S 2015 Nat. Commun. 6 7497
[34] Conings B, Drijkoningen J, Gauquelin N, Babayigit A, D'Haen J, D'Olieslaeger L, Ethirajan A, Verbeeck J, Manca J, Mosconi E, Angelis F D and Boyen H G 2015 Adv. Energy Mater. 5 1500477
[35] Zhang H, Fu X, Tang Y, Wang H, Zhang C, Yu W W, Wang X, Zhang Y and Xiao M 2019 Nat. Commun. 10 1088
[36] Cho H, Kim Y H, Wolf C, Lee H D and Lee T W 2018 Adv. Mater. 30 e1704587
[37] Barker A J, Sadhanala A, Deschler F, Gandini M, Senanayak S P, Pearce P M, Mosconi E, Pearson A J, Wu Y, Kandada A R S, Leijtens T, Angelis F D, Dutton S E, Petrozza A and Friend R H 2017 ACS Energy Lett. 2 1416
[38] ten Brinck S, Zaccaria F and Infante I 2019 ACS Energy Lett. 4 2739
[39] Meggiolaro D, Mosconi E and De Angelis F 2019 ACS Energy Lett. 4 779
[40] Kim Y H, Wolf C, Kim H and Lee T W 2018 Nano Energy 52 329
[41] Kamat P V and Kuno M 2021 Acc. Chem. Res. 54 520
[42] Vashishtha P and Halpert J E 2017 Chem. Mater. 29 5965
[43] Wen Z, Xie F and Choy W C H 2021 Nano Select 3 505
[44] Yuan Y, Wang Q, Shao Y, Lu H, Li T, Gruverman A and Huang J 2016 Adv. Energy Mater. 6 1501803
[45] Prakasam V, Tordera D, Bolink H J and Gelinck G 2019 Adv. Opt. Mater. 7 1900902
[46] Geng S, Wen Y, Zhou B, Wang Z, Wang Z, Wang P, Jing Y, Cao K, Wang K and Chen R 2021 ACS Appl. Electron. Mater. 3 2362
[47] Zhao L, Gao J, Lin Y L, Yeh Y W, Lee K M, Yao N, Loo Y L and Rand B P 2017 Adv. Mater. 29 1605317
[48] Cheng T, Tumen-Ulzii G, Klotz D, Watanabe S, Matsushima T and Adachi C 2020 ACS Appl. Mater. Interfaces 12 33004
[49] Kim H, Kim J S, Heo J M 2020 Nat. Commun. 11 3378
[50] Feng Y, Zhao Y, Zhou W K, Li Q, Saidi W A, Zhao Q and Li X Z 2018 J. Phys. Chem. Lett. 9 6536
[51] Cardenas-Daw C, Simon T, Stolarczyk J K and Feldmann J 2017 J. Am. Chem. Soc. 139 16462
[52] Shi Y, Wu W, Dong H, Li G, Xi K, Divitini G, Ran C, Yuan F, Zhang M, Jiao B, Hou X and Wu Z 2018 Adv. Mater. 30 e1800251
[56] Knight A J and Herz L M 2020 Energy Environ. Sci. 13 2024
[57] Shynkarenko Y, Bodnarchuk M I, Bernasconi C, Berezovska Y, Verteletskyi V, Ochsenbein S T and Kovalenko M V 2019 ACS Energy Lett. 4 2703
[53] Zhang S, Liu H, Li X and Wang S 2020 Nano Energy 77 105302
[54] Li H, Dong W, Shen X, Ge C, Song Y, Wang Z, Wang A, Yang Z, Hao M, Zhang Y, Zheng W, Zhang X and Dong Q 2022 J. Phys. Chem. C 126 1085
[55] Zhang X, Lu M, Zhang Y, Wu H, Shen X, Zhang W, Zheng W, Colvin V L and Yu W W 2018 ACS Cent. Sci. 4 1352
[58] Xu B, Wang W, Zhang X, Liu H, Zhang Y, Mei G, Chen S, Wang K, Wang L and Sun X W 2018 Sci. Rep. 8 15799
[59] Lee H, Ko D and Lee C 2019 ACS Appl Mater Interfaces 11 11667
[60] Bi E, Chen H, Xie F, Wu Y, Chen W, Su Y, Islam A, Gratzel M, Yang X and Han L 2017 Nat. Commun. 8 15330
[61] Kim Y H, Kim J S and Lee T W 2019 Adv. Mater. 31 e1804595
[62] Yuan Y, Chae J, Shao Y, Wang Q, Xiao Z, Centrone A and Huang J 2015 Adv. Energy Mater. 5 1500615
[63] Li J, Shan X, Bade S G R, Geske T, Jiang Q, Yang X and Yu Z 2016 J. Phys. Chem. Lett. 7 4059
[64] Futscher M H, Gangishetty M K, Congreve D N and Ehrler B 2020 ACS Appl. Electron. Mater. 2 1522
[65] Yao J S, Ge J, Han B N, Wang K H, Yao H B, Yu H L, Li J H, Zhu B S, Song J Z, Chen C, Zhang Q, Zeng H B, Luo Y and Yu S H 2018 J. Am. Chem. Soc. 140 3626
[66] Zhang J, Zhang L, Cai P, Xue X, Wang M, Zhang J and Tu G 2019 Nano Energy 62 434
[67] Zou S, Liu Y, Li J, Liu C, Feng R, Jiang F, Li Y, Song J, Zeng H, Hong M and Chen X 2017 J. Am. Chem. Soc. 139 11443
[68] Tan S, Yavuz I, De Marco N, Huang T, Lee S J, Choi C S, Wang M, Nuryyeva S, Wang R, Zhao Y, Wang H C, Han T H, Dunn B, Huang Y, Lee J W and Yang Y 2020 Adv. Mater. 32 e1906995
[69] Song J, Fang T, Li J, Xu L, Zhang F, Han B, Shan Q and Zeng H 2018 Adv. Mater. 30 e1805409
[70] Ye F, Zhang H, Wang P, Cai J, Wang L, Liu D and Wang T 2020 Chem. Mater. 32 3211
[71] Zheng X, Yuan S and Liu J 2020 ACS Energy Lett. 5 793
[72] Yang J N, Song Y, Yao J S, Wang K H, Wang J J, Zhu B S, Yao M M, Rahman S U, Lan Y F, Fan F J and Yao H B 2020 J. Am. Chem. Soc. 142 2956
[73] Baek S, Kang S, Son C, Shin S J, Kim J H, Park J and Kim S W 2020 Adv. Opt. Mater. 8 1901897
[74] Kim Y C, An H J, Kim D H, Myoung J M, Heo Y J and Cho J H 2020 Adv. Funct. Mater. 31 2005553
[75] Hassan Y, Park J H, Crawford M L, Sadhanala A, Lee J, Sadighian J C, Mosconi E, Shivanna R, Radicchi E, Jeong M, Yang C, Choi H, Park S H, Song M H, De Angelis F, Wong C Y, Friend R H, Lee B R and Snaith H J 2021 Nature 591 72
[76] Bi C, Yao Z, Sun X, Wei X, Wang J and Tian J 2021 Adv. Mater. 33 e2006722
[77] Abdi-Jalebi M, Andaji-Garmaroudi Z, Cacovich S, Stavrakas C, Philippe B, Richter J M, Alsari M, Booker E P, Hutter E M, Pearson A J, Lilliu S, Savenije T J, Rensmo H, Divitini G, Ducati C, Friend R H and Stranks S D 2018 Nature 555 497
[78] Zhang L, Yuan F, Xi J, Jiao B, Dong H, Li J and Wu Z 2020 Adv. Funct. Mater. 30 2001834
[79] Tan Z K, Moghaddam R S, Lai M L, Docampo P, Higler R, Deschler F, Price M, Sadhanala A, Pazos L M, Credgington D, Hanusch F, Bein T, Snaith H J and Friend R H 2014 Nat. Nanotechnol. 9 687
[80] Zhao B, Bai S and Kim V 2018 Nat. Photon. 12 783
[81] Cho H, Wolf C, Kim J S, Yun H J, Bae J S, Kim H, Heo J M, Ahn S and Lee T W 2017 Adv. Mater. 29 1700579
[82] Ravi V K, Scheidt R A, Nag A, Kuno M and Kamat P V 2018 ACS Energy Lett. 3 1049
[83] Zhang X, Yin W, Zheng W and Rogach A L 2020 ACS Energy Lett. 5 2927
[84] Han B, Yuan S, Cai B, Song J, Liu W, Zhang F, Fang T, Wei C and Zeng H 2021 Adv. Funct. Mater. 31 2011003
[85] Li H, Lin H, Ouyang D, Yao C, Li C, Sun J, Song Y, Wang Y, Yan Y, Wang Y, Dong Q and Choy W C H 2021 Adv. Mater. 33 e2008820
[86] Tsai H, Shrestha S, Vilá R A, Huang W, Liu C, Hou C H, Huang H H, Wen X, Li M, Wiederrecht G, Cui Y, Cotlet M, Zhang X, Ma X and Nie W 2021 Nat. Photon. 15 843
[87] Xue X, Li M, Liu Z, Wang C, Xu J, Wang S, Zhang H, Zhong H and Ji W 2022 Fundamental Research
[88] Lee S, Park J H, Lee B R, Jung E D, Yu J C, Di Nuzzo D, Friend R H and Song M H 2017 J. Phys. Chem. Lett. 8 1784
[89] Ma D, Todorovic P and Meshkat S 2020 J. Am. Chem. Soc. 142 5126
[90] Han B, Yuan S, Fang T, Zhang F, Shi Z and Song J 2020 ACS Appl. Mater. Interfaces 12 14224
[91] Chu Z, Ye Q, Zhao Y, Ma F, Yin Z, Zhang X and You J 2021 Adv. Mater. 33 e2007169
[92] Guo Y, Apergi S, Li N, Chen M, Yin C, Yuan Z, Gao F, Xie F, Brocks G, Tao S and Zhao N 2021 Nat. Commun. 12 644
[93] Chen M, Shan X, Geske T, Li J and Yu Z 2017 ACS Nano 11 6312
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