Please wait a minute...
Chin. Phys. B, 2010, Vol. 19(6): 067101    DOI: 10.1088/1674-1056/19/6/067101
CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES Prev   Next  

Electric dipolar interaction assisted growth of single crystalline organic thin films

Cai Jin-Ming(蔡金明)a)b), Zhang Yu-Yang(张余洋)a), Hu Hao(胡昊)a), Bao Li-Hong(鲍丽宏)a), Pan Li-Da(潘理达)a), Tang Wei(唐卫)a), Li Guo(李果)a), Du Shi-Xuan(杜世萱)a), Shen Jian(沈健)b), and Gao Hong-Jun(高鸿钧)a)
a Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China; b Materials Sciences and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA
Abstract  We report on a forest-like-to-desert-like pattern evolution in the growth of an organic thin film observed by using an atomic force microscope. We use a modified diffusion limited aggregation model to simulate the growth process and are able to reproduce the experimental patterns. The energy of electric dipole interaction is calculated and determined to be the driving force for the pattern formation and evolution. Based on these results, single crystalline films are obtained by enhancing the electric dipole interaction while limiting effects of other growth parameters.
Keywords:  electric dipolar interaction      organic thin films      diffusion limited aggregation model  
Received:  11 November 2009      Accepted manuscript online: 
PACS:  68.55.A- (Nucleation and growth)  
  68.37.Ps (Atomic force microscopy (AFM))  
  73.61.Ph (Polymers; organic compounds)  
  81.15.-z (Methods of deposition of films and coatings; film growth and epitaxy)  
Fund: Project supported by the National Natural Science Foundation of China (Grant No.~10774176), and the National Basic Research Program of China (Grant No.~2006CB806202).

Cite this article: 

Cai Jin-Ming(蔡金明), Zhang Yu-Yang(张余洋), Hu Hao(胡昊), Bao Li-Hong(鲍丽宏), Pan Li-Da(潘理达), Tang Wei(唐卫), Li Guo(李果), Du Shi-Xuan(杜世萱), Shen Jian(沈健), and Gao Hong-Jun(高鸿钧) Electric dipolar interaction assisted growth of single crystalline organic thin films 2010 Chin. Phys. B 19 067101

[1] Gao H J and Gao L 2009 Prog. Surf. Sci. doi:10.1016/j.progsurf.2009.10.001
[2] Gao H J, Sohlberg K, Xue Z Q, Chen H Y, Hou S M, Ma L P, Fang X W, Pang S J and Pennycook S J 2000 Phys. Rev. Lett. 84 1780
[3] Feng M, Lee J, Zhao J, Yates J T and Petek H 2007 J. Am. Chem. Soc. 129 12394
[4] Burrows P E and Forrest S R 1993 Appl. Phys. Lett. 62 3102
[5] Briseno A L, Mannsfeld S C B, Ling M M, Liu S H, Tseng R J, Reese C, Roberts M E, Yang Y, Wudl F and Bao Z N 2006 Nature 444 913
[6] Karl N 2001 Organic Electronic Materials (Berlin: Springer) p.~283
[7] Dimitrakopoulos C D and Malenfant P R L 2002 Adv. Mater. 14 99
[8] Fenter P, Schreiber F, Zhou L, Eisenberger P and Forrest S R 1997 Phys. Rev. B 56 3046
[9] Khenner M 2008 Phys. Rev. B 77 165414
[10] Ruiz R, Choudhary D, Nickel B, Toccoli T, Chang K C, Mayer A C, Clancy P, Blakely J M, Headrick R L, Iannotta S and Malliaras G G 2004 Chem. Mater. 16 4497
[11] Mulheran P A, Pellenc D, Bennett R A, Green R J and Sperrin M 2008 Phys. Rev. Lett. 100 068102
[12] Zhang Z Y and Lagally M G 1997 Science 276 377
[13] Weber U K, Burlakov V M, Perdigao L M A, Fawcett R H J, Beton P H, Champness N R, Jefferson J H, Briggs G A D and Pettifor D G 2008 Phys. Rev. Lett. 100 156101
[14] Shi D X, Ji W, Lin X, He X B, Lian J C, Gao L, Cai J M, Lin H, Du S X, Lin F, Seidel C, Chi L F, Hofer W A, Fuchs H and Gao H J 2006 Phys. Rev. Lett. 96 226106
[15] Gao H J, Canright G S, Pang S J, Sandler I M, Xue Z Q and Zhang Z Y 1998 Fractals 6 337
[16] Fernandez-Torrente I, Monturet S, Franke K J, Fraxedas J, Lorente N and Pascual J I 2007 Phys. Rev. Lett. 99 176103
[17] Schiek M, Balzer F, Al-Shamery K, Brewer J R, Lutzen A and Rubahn H G 2008 Small 4 176
[18] Carroll R L and Gorman C B 2002 Angew. Chem. Int. Ed. 41 4378
[19] Grabowski Z R, Rotkiewicz K and Rettig W 2003 Chem. Rev. 103 3899
[20] Bosch P, Fernandez-Arizpe A, Mateo J L, Catalina F and Peinado C 2002 J. Photochem. Photobiol. A : Chem. 153 135
[21] Bosch P, Fernandez-Arizpe A, Mateo J L, Lozano A E and Noheda P 2000 J. Photochem. Photobiol. A : Chem. 133 51
[22] Hakala K, Vatanparast R, Li S Y, Peinado C, Bosch P, Catalina F and Lemmetyinen H 2000 Macromolecules 33 5954
[23] Witten T A and Sander L M 1981 Phys. Rev. Lett. 47 1400
[1] Suppression of ice nucleation in supercooled water under temperature gradients
Li-Ping Wang(王利平), Wei-Liang Kong(孔维梁), Pei-Xiang Bian(边佩翔), Fu-Xin Wang(王福新), and Hong Liu(刘洪). Chin. Phys. B, 2021, 30(6): 068203.
[2] A low-dimensional crystal growth model on an isotropic and quasi-free sustained substrate
Chenxi Lu(卢晨曦), Senjiang Yu(余森江), Lingwei Li(李领伟), Bo Yang(杨波), Xiangming Tao(陶向明), Gaoxiang Ye(叶高翔). Chin. Phys. B, 2020, 29(3): 038101.
[3] Segregation behavior and embrittling effect of lanthanide La, Ce, Pr, and Nd at Σ3(111) tilt symmetric grain boundary in α-Fe
Jinli Cao(曹金利), Wen Yang(杨文), Xinfu He(贺新福). Chin. Phys. B, 2019, 28(12): 126802.
[4] Segregations and desorptions of Ge atoms in nanocomposite Si1-xGex films during high-temperature annealing
Yu Wang(汪煜), Meng Yang(杨濛), Gang Wang(王刚), Xiao-Xu Wei(魏晓旭), Jun-Zhuan Wang(王军转), Yun Li(李昀), Ze-Wen Zou(左则文), You-Dou Zheng(郑有炓), Yi Shi(施毅). Chin. Phys. B, 2017, 26(12): 126801.
[5] Structural, optical, and electrical properties of Cu-doped ZrO2 films prepared by magnetron co-sputtering
Nian-Qi Yao(姚念琦), Zhi-Chao Liu(刘智超), Guang-Rui Gu(顾广瑞), Bao-Jia Wu(吴宝嘉). Chin. Phys. B, 2017, 26(10): 106801.
[6] Effects of the Be22W phase formation on hydrogen retention and blistering in mixed Be/W systems
Jin-Li Cao(曹金利), Bing-Ling He(赫丙龄), Wei Xiao(肖伟), Li-Gen Wang(王立根). Chin. Phys. B, 2017, 26(7): 076801.
[7] First-principles study of He trapping in η-Fe2C
Bing-Ling He(赫丙玲), Jin-Long Wang(王金龙), Zhi-Xue Tian(田之雪), Li-Juan Jiang(蒋利娟), Wei Song(宋薇), Bin Wang(王斌). Chin. Phys. B, 2016, 25(11): 116801.
[8] Thick c-BN films deposited by radio frequency magnetron sputtering in argon/nitrogen gas mixture with additional hydrogen gas
Yan Zhao(赵艳), Wei Gao(高伟), Bo Xu(徐博), Ying-Ai Li(李英爱), Hong-Dong Li(李红东), Guang-Rui Gu(顾广瑞), Hong Yin(殷红). Chin. Phys. B, 2016, 25(10): 106801.
[9] Transient liquid assisted nucleation mechanism of YBa2Cu3O7-δ in coated conductor films derived by BaF2 process
Gu Zhao-Hui (谷朝辉), Yang Wen-Tao (杨文涛), Bai Chuan-Yi (白传易), Guo Yan-Qun (郭艳群), Lu Yu-Ming (鲁玉明), Liu Zhi-Yong (刘志勇), Lu Qi (路齐), Shu Gang-Qiang (舒刚强), Cai Chuan-Bing (蔡传兵). Chin. Phys. B, 2015, 24(9): 096805.
[10] Growth mechanism and modification of electronic and magnetic properties of silicene
Liu Hong-Sheng (柳洪盛), Han Nan-Nan (韩楠楠), Zhao Ji-Jun (赵纪军). Chin. Phys. B, 2015, 24(8): 087303.
[11] Effect of the thickness of InGaN interlayer on a-plane GaN epilayer
Wang Jian-Xia (王建霞), Wang Lian-Shan (汪连山), Zhang Qian (张谦), Meng Xiang-Yue (孟祥岳), Yang Shao-Yan (杨少延), Zhao Gui-Juan (赵桂娟), Li Hui-Jie (李辉杰), Wei Hong-Yuan (魏鸿源), Wang Zhan-Guo (王占国). Chin. Phys. B, 2015, 24(2): 026802.
[12] Effects of growing conditions on the electric and magnetic properties of strained La2/3Sr1/3MnO3 thin films
Lu Hai-Xia (卢海霞), Wang Jing (王晶), Shen Bao-Gen (沈保根), Sun Ji-Rong (孙继荣). Chin. Phys. B, 2015, 24(2): 027504.
[13] Preparation and characterization of thick cubic boron nitride films
Wang Ming-E (王明娥), Ma Guo-Jia (马国佳), Dong Chuang (董闯), Gong Shui-Li (巩水利). Chin. Phys. B, 2014, 23(6): 066805.
[14] Structural and electrical characterization of annealed Si1-xCx/SiC thin film prepared by magnetron sputtering
Huang Shi-Hua (黄仕华), Liu Jian (刘剑). Chin. Phys. B, 2014, 23(5): 058105.
[15] Effects of V/Ⅲ ratio on a-plane GaN epilayers with an InGaN interlayer
Wang Jian-Xia (王建霞), Wang Lian-Shan (汪连山), Yang Shao-Yan (杨少延), Li Hui-Jie (李辉杰), Zhao Gui-Juan (赵桂娟), Zhang Heng (张恒), Wei Hong-Yuan (魏鸿源), Jiao Chun-Mei (焦春美), Zhu Qin-Sheng (朱勤生), Wang Zhan-Guo (王占国). Chin. Phys. B, 2014, 23(2): 026801.
No Suggested Reading articles found!