Incommensurate-commensurate magnetic phase transition in double tungstate Li2Co(WO4)2
Xiyu Chen(陈西煜)1, Ning Ding(丁宁)2, Meifeng Liu(刘美风)1,†, Tao Zou(邹涛)3,‡, V. Ovidiu Garlea4, Jingwen Gong(龚婧雯)1, Fei Liu(刘飞)1, Yunlong Xie(谢云龙)1, Lun Yang(杨伦)1, Shuhan Zheng(郑书翰)1, Xiuzhang Wang(王秀章)1, Shuai Dong(董帅)2,§, T. Charlton4, and Jun-Ming Liu(刘俊明)1,5
1 Institute for Advanced Materials, Hubei Normal University, Huangshi 435002, China; 2 School of Physics, Southeast University, Nanjing 211189, China; 3 Collaborative Innovation Center of Light Manipulations and Applications, Shangdong Normal University, Jinan 250358, China; 4 Neutron Scattering División, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, USA; 5 Laboratory of Solid State Microstructures and Innovative Center of Advanced Microstructures, Nanjing University, Nanjing 210093, China
Abstract Magnetic susceptibility, specific heat, and neutron powder diffraction measurements have been performed on polycrystalline LiCo(WO) samples. Under zero magnetic field, two successive magnetic transitions at K and K are observed. The magnetic ordering temperatures gradually decrease as the magnetic field increases. Neutron diffraction reveals that LiCo(WO) enters an incommensurate magnetic state with a temperature dependent between and . The magnetic propagation vector locks-in to a commensurate value below . The antiferromagnetic structure is refined at 1.7 K with Co magnetic moment 2.8(1) , consistent with our first-principles calculations.
Fund: Project supported by the National Natural Science Foundation of China (Grant Nos. 11834002, 12074111, and 11704109) and the National Key R&D Project of China (Grant No. 2016YFA0300101).
Corresponding Authors:
Meifeng Liu, Tao Zou, Shuai Dong
E-mail: lmfeng1107@hbnu.edu.cn;taozoucn@gmail.com;sdong@seu.edu.cn
Cite this article:
Xiyu Chen(陈西煜), Ning Ding(丁宁), Meifeng Liu(刘美风), Tao Zou(邹涛), V. Ovidiu Garlea, Jingwen Gong(龚婧雯), Fei Liu(刘飞), Yunlong Xie(谢云龙), Lun Yang(杨伦), Shuhan Zheng(郑书翰), Xiuzhang Wang(王秀章), Shuai Dong(董帅), T. Charlton, and Jun-Ming Liu(刘俊明) Incommensurate-commensurate magnetic phase transition in double tungstate Li2Co(WO4)2 2022 Chin. Phys. B 31 047501
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