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Acta Physica Sinica (Overseas Edition), 1996, Vol. 5(5): 377-383    DOI: 10.1088/1004-423X/5/5/008
CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES Prev   Next  

THIRD-ORDER NONLINEAR OPTICAL PROPERTIES OF SnO2 NANOPARTICLES

YU BAO-LONG (余保龙)a, ZHANG GUI-LAN (张桂兰)a, TANG GUO-QING (汤国庆)a, WU XIAO-CHUN (吴晓春)a, CHEN WEN-JU (陈文驹)a, YANG BIN-ZHOU (杨斌洲)b, ZHAO PING (赵平)b
a Institute of Modern Optics, Nankai University, Tianjin 300071, China; b Xi'an Institute of Optics and fine Mechanics, Academia Sinica, Xi'an 710068, China
Abstract  We have measured the third-order nonlinear susceptibilities χ(3) of SnO2 nanoparticles both naked and coated with a layer of stearic acid by using Z-scan technique with 1.06μm pulse from a Q-switched Nd:YAG laser. The results show that the χ(3) of these nanoparticles is much larger than that of the bulk material. Moreover, we find that two-photon absorption is not present for the naked nanoparticles but it is preseut for the coated ones, and the χ(3) of the latter is larger than that of the former. It is demonstrated that the surface situations of the nanoparticles have great influence on their nonlinear optical properties.
Received:  09 December 1994      Revised:  25 September 1995      Accepted manuscript online: 
PACS:  42.65.An (Optical susceptibility, hyperpolarizability)  
  78.67.Bf (Nanocrystals, nanoparticles, and nanoclusters)  
  42.60.Gd (Q-switching)  
Fund: Project supported by the Climbing Programme-Chinese Nationed Key Project for Fundamental Research and State Key Laboratory of Transient Optical Technique. Xi'an Institute of Optics and Fine Mechanics, Academia Sinica, China.

Cite this article: 

YU BAO-LONG (余保龙), ZHANG GUI-LAN (张桂兰), TANG GUO-QING (汤国庆), WU XIAO-CHUN (吴晓春), CHEN WEN-JU (陈文驹), YANG BIN-ZHOU (杨斌洲), ZHAO PING (赵平) THIRD-ORDER NONLINEAR OPTICAL PROPERTIES OF SnO2 NANOPARTICLES 1996 Acta Physica Sinica (Overseas Edition) 5 377

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