Abstract The double-doped La$_{2/3+4x/3}$Sr$_{1/3-4x/3}$Mn$_{1-x}$Mg$_{x}$O$_{3}$ samples with fixed Mn3+/Mn4+ ratio equal to 2/1 are investigated by means of magnetism and transport measurements. Phase separation is observed at temperature higher than Tconset for x=0.10 and 0.15. For x=0.10, rather strong phase separation induces drastic magnetic random potential and results in the localization of carriers. Thus, the variable-range hopping process dominates. For other samples, there is no or only weak phase separation above Tconset. Thus, thermal activation mechanism is responsible for the high temperature transport behaviour. For x=0.20 and 0.25, unexpected AFM behaviour is observed at low temperature. All these results are well understood by considering the special role of the ``double-doping".
Received: 28 March 2006
Revised: 13 June 2006
Accepted manuscript online:
PACS:
75.60.Ej
(Magnetization curves, hysteresis, Barkhausen and related effects)
Fund: Project
supported by the National Natural Science Foundation of China (Grant
Nos 10504029
and 10334090), and the State Key Project of Fundamental Research, China
(Grant No 001CB610604).
Cite this article:
Qu Zhe(屈哲), Pi Li(皮雳), Fan Ji-Yu(樊济宇), Tan Shun(谭舜), Zhang Bei (张贝), Zhang Meng(张锰), and Zhang Yu-Heng (张裕恒) Electric and magnetic behaviour in double doped La$_{2/3+4x/3}$Sr$_{1/3-4x/3}$Mn$_{1-x}$Mg$_{x}$O$_{3}$ 2007 Chinese Physics 16 258
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