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Chinese Physics, 2007, Vol. 16(1): 258-265    DOI: 10.1088/1009-1963/16/1/044
CONDENSED MATTER: ELECTRONIC STRUCTURE, ELECTRICAL, MAGNETIC, AND OPTICAL PROPERTIES Prev   Next  

Electric and magnetic behaviour in double doped La$_{2/3+4x/3}$Sr$_{1/3-4x/3}$Mn$_{1-x}$Mg$_{x}$O$_{3}$

Qu Zhe(屈哲), Pi Li(皮雳), Fan Ji-Yu(樊济宇), Tan Shun(谭舜), Zhang Bei (张贝), Zhang Meng(张锰), and Zhang Yu-Heng (张裕恒)
Structure Research Laboratory, University of Science and Technology of China, Hefei 230026, China
Abstract  The double-doped La$_{2/3+4x/3}$Sr$_{1/3-4x/3}$Mn$_{1-x}$Mg$_{x}$O$_{3}$ samples with fixed Mn3+/Mn4+ ratio equal to 2/1 are investigated by means of magnetism and transport measurements. Phase separation is observed at temperature higher than Tconset for x=0.10 and 0.15. For x=0.10, rather strong phase separation induces drastic magnetic random potential and results in the localization of carriers. Thus, the variable-range hopping process dominates. For other samples, there is no or only weak phase separation above Tconset. Thus, thermal activation mechanism is responsible for the high temperature transport behaviour. For x=0.20 and 0.25, unexpected AFM behaviour is observed at low temperature. All these results are well understood by considering the special role of the ``double-doping".
Keywords:  perovskite manganites      double doping      phase separation      variable-range hopping mechanism  
Received:  28 March 2006      Revised:  13 June 2006      Accepted manuscript online: 
PACS:  75.60.Ej (Magnetization curves, hysteresis, Barkhausen and related effects)  
  61.66.Fn (Inorganic compounds)  
  64.75.-g (Phase equilibria)  
  72.20.Ee (Mobility edges; hopping transport)  
  72.80.Sk (Insulators)  
  76.30.-v (Electron paramagnetic resonance and relaxation)  
Fund: Project supported by the National Natural Science Foundation of China (Grant Nos 10504029 and 10334090), and the State Key Project of Fundamental Research, China (Grant No 001CB610604).

Cite this article: 

Qu Zhe(屈哲), Pi Li(皮雳), Fan Ji-Yu(樊济宇), Tan Shun(谭舜), Zhang Bei (张贝), Zhang Meng(张锰), and Zhang Yu-Heng (张裕恒) Electric and magnetic behaviour in double doped La$_{2/3+4x/3}$Sr$_{1/3-4x/3}$Mn$_{1-x}$Mg$_{x}$O$_{3}$ 2007 Chinese Physics 16 258

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