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Special Issue:
SPECIAL TOPIC — The third carbon: Carbyne with one-dimensional sp-carbon
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| TOPICAL REVIEW—The third carbon: Carbyne with one-dimensional sp-carbon |
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Pulsed laser ablation in liquid of sp-carbon chains: Status and recent advances |
| Pietro Marabotti, Sonia Peggiani, Alessandro Vidale, and Carlo Spartaco Casari† |
| Department of Energy, Politecnico di Milano, Via Ponzio 34/3, 20133, Milano, Italy |
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Abstract This review provides a discussion of the current state of research on sp-carbon chains synthesized by pulsed laser ablation in liquid. In recent years, pulsed laser ablation in liquid (PLAL) has been widely employed for polyynes synthesis thanks to its flexibility with varying laser parameters, solvents, and targets. This allows the control of sp-carbon chains properties as yield, length, termination and stability. Although many reviews related to PLAL have been published, a comprehensive work reporting the current status and advances related to the synthesis of sp-carbon chains by PLAL is still missing. Here we first review the principle of PLAL and the mechanisms of formation of sp-carbon chains. Then we discuss the role of laser fluence (i.e. energy density), solvent, and target for sp-carbon chains synthesis. Lastly, we report the progress related to the prolonged stability of sp-carbon chains by PLAL encapsulated in polymeric matrices. This review will be a helpful guide for researchers interested in synthesizing sp-carbon chains by PLAL.
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Received: 31 May 2022
Revised: 12 July 2022
Accepted manuscript online: 18 July 2022
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PACS:
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52.38.Mf
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(Laser ablation)
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81.05.U-
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(Carbon/carbon-based materials)
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81.05.uj
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(Diamond/nanocarbon composites)
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81.07.-b
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(Nanoscale materials and structures: fabrication and characterization)
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| Fund: The authors acknowledge funding from the European Research Council (ERC) under the European Union's Horizon 2020 research and innovation program ERC Consolidator Grant (ERC CoG2016 EspLORE grant agreement No. 724610, website:www.esplore.polimi.it). We thank A. Sacchi and M. Benoliel for their assitance during the measurements and the data analyses. |
Corresponding Authors:
Carlo Spartaco Casari
E-mail: carlo.casari@polimi.it
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Cite this article:
Pietro Marabotti, Sonia Peggiani, Alessandro Vidale, and Carlo Spartaco Casari Pulsed laser ablation in liquid of sp-carbon chains: Status and recent advances 2022 Chin. Phys. B 31 125202
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