Please wait a minute...
Chin. Phys. B, 2010, Vol. 19(4): 043201    DOI: 10.1088/1674-1056/19/4/043201
ATOMIC AND MOLECULAR PHYSICS Prev   Next  

Selective excitation and suppression of coherent anti-Stokes Raman scattering by shaping femtosecond pulses

Zhang Shi-An(张诗按), Zhang Hui(张晖), Wang Zu-Geng(王祖赓), and Sun Zhen-Rong(孙真荣)
State Key Laboratory of Precision Spectroscopy (East China Normal University), and Department of Physics, East China Normal University, Shanghai 200062, China
Abstract  Femtosecond coherent anti-Stokes Raman scattering (CARS) suffers from poor selectivity between neighbouring Raman levels due to the large bandwidth of the femtosecond pulses. This paper provides a new method to realize the selective excitation and suppression of femtosecond CARS by manipulating both the probe and pump (or Stokes) spectra. These theoretical results indicate that the CARS signals between neighbouring Raman levels are differentiated from their indistinguishable femtosecond CARS spectra by tailoring the probe spectrum, and then their selective excitation and suppression can be realized by supplementally manipulating the pump (or Stokes) spectrum with the $\pi $ spectral phase step.
Keywords:  coherent anti-Stokes Raman scattering (CARS)      selective excitation      selective suppression      pulse shaping  
Received:  29 June 2009      Revised:  03 August 2009      Accepted manuscript online: 
PACS:  42.65.Dr (Stimulated Raman scattering; CARS)  
  42.65.Re (Ultrafast processes; optical pulse generation and pulse compression)  
Fund: Project supported by Programme for Changjiang Scholars and Innovative Research Team in University (PCSIRT), Shanghai Leading Academic Discipline Project (Grant No.~B408), National Key Project for Basic Research of China (Grant Nos.~2006CB806006 and 2006CB

Cite this article: 

Zhang Shi-An(张诗按), Zhang Hui(张晖), Wang Zu-Geng(王祖赓), and Sun Zhen-Rong(孙真荣) Selective excitation and suppression of coherent anti-Stokes Raman scattering by shaping femtosecond pulses 2010 Chin. Phys. B 19 043201

[1] Chen T, Vierheilig A, P Waltner, Heid M, Kiefer W and Materny A 2000 Chem. Phys. Lett. 326 375
[2] Rubner O, Schmitt M, Knopp G and Materny A 1998 J. Phys. Chem. A 102 9734
[3] Hashimoto M, Araki T and Kawata S 2000 Opt. Lett. 25 1768
[4] Yuan J H, Xiao F R, Wang G Y and Xu Z Z 2005 Chin. Phys. 14 935
[5] Zumbusch A, Holtom G R and Xie X S 1999 Phys. Rev. Lett. 82 4142
[6] Müller M, Squier J, Lange C A de and Brakenhoff G J 2000 J. Microsc. 197] 150
[7] Wang Y H, Peng Y J, He X, Song Y F and Yang Y Q 2009 Chin. Phys. B 18 1463
[8] Ujj L, Coates C G, Kelly J M, Kruger P E, McGarvey J J and Atkinson G H 2002 J. Phys. Chem. B 106 4854
[9] Cheng J, Volkmer A, Book L D and Xie X S 2001 J. Phys. Chem. B 105 1277
[10] Song J J, Eesley G L and Levenson M D 1976 Appl. Phys. Lett. 29 567
[11] Oron D, Dudovich N, Yelin D and Silberberg Y 2002 Phys. Rev. A 65 043408
[12] Oron D, Dudovich N, Yelin D and Silberberg Y 2002 Phys. Rev. Lett. 88 063004
[13] Pearson B J, White J L, Weinacht T C and Bucksbaum P H 2001 Phys. Rev. A 63] 063412
[14] Konradi J, Singh A K, Scaria A V and Materny A 2006 J. Raman Spectrosc. 37 697
[15] Konradi J, Singh A K and Materny A 2006 J. Photochem. Photobio. 180 289
[16] Zhang S, Zhang L, Zhang X, Ding L, Chen G, Sun Z and Wang Z 2007 Chem. Phys. Lett. 433 416
[17] Müller M and Schins J M 2002 J. Phys. Chem. B 106 3715
[18] Zhang S A, Wang Z G and Sun Z R 2008 Chin. Phys. Lett. 25 3260
[19] Malinovskaya S A, Bucksbaum P H and Berman P R 2004 Phys. Rev. A, 69 013801
[1] Simulating the resonance-mediated (1+2)-three-photon absorption enhancement in Pr3+ ions by a rectangle phase modulation
Wenjing Cheng(程文静), Yuan Li(李媛), Hongzhen Qiao(乔红贞), Meng Wang(王蒙), Shaoshuo Ma(马绍朔), Fangjie Shu(舒方杰), Chuanqi Xie(解传奇), and Guo Liang(梁果). Chin. Phys. B, 2022, 31(6): 063201.
[2] Up-conversion luminescence tuning in Er3+-doped ceramic glass by femtosecond laser pulse at different laser powers
Wen-Jing Cheng(程文静), Guo Liang(梁果), Ping Wu(吴萍), Shi-Hua Zhao(赵世华), Tian-Qing Jia(贾天卿), Zhen-Rong Sun(孙真荣), Shi-An Zhang(张诗按). Chin. Phys. B, 2018, 27(12): 123201.
[3] Scanning the energy dissipation process of energetic materials based on excited state relaxation and vibration-vibration coupling
Wen-Yan Wang(王文岩), Ning Sui(隋宁), Li-Quan Zhang(张里荃), Ying-Hui Wang(王英惠), Lin Wang(王琳), Quan Wang(王权), Jiao Wang(王娇), Zhi-Hui Kang(康智慧), Yan-Qiang Yang(杨延强), Qiang Zhou(周强), Han-Zhuang Zhang(张汉壮). Chin. Phys. B, 2018, 27(10): 104205.
[4] Simulating resonance-mediated two-photon absorption enhancement in rare-earth ions by a rectangle phase modulation
Da-Long Qi(齐大龙), Ye Zheng(郑烨), Wen-Jing Cheng(程文静), Yun-Hua Yao(姚云华), Lian-Zhong Deng(邓联忠), Dong-Hai Feng(冯东海), Tian-Qing Jia(贾天卿), Zhen-Rong Sun(孙真荣), Shi-An Zhang(张诗按). Chin. Phys. B, 2018, 27(1): 013202.
[5] On-chip optical pulse shaper for arbitrary waveform generation
Liao Sha-Sha (廖莎莎), Yang Ting (杨婷), Dong Jian-Ji (董建绩). Chin. Phys. B, 2014, 23(7): 073201.
[6] Diversity of photonic differentiators based on flexible demodulation of phase signals
Zheng Ao-Ling (郑傲凌), Dong Jian-Ji (董建绩), Lei Lei (雷蕾), Yang Ting (杨婷), Zhang Xin-Liang (张新亮). Chin. Phys. B, 2014, 23(3): 033201.
[7] Optical pulse shaper with integrated slab waveguide for arbitrary waveform generation using optical gradient force
Liao Sha-Sha (廖莎莎), Min Shu-Cun (闵书存), Dong Jian-Ji (董建绩). Chin. Phys. B, 2014, 23(12): 124211.
[8] Selective triggering of phase change in dielectric by femtosecond pulse trains based on electron dynamics control
Xu Chuan-Cai (徐传彩), Jiang Lan (姜澜), Leng Ni (冷妮), Liu Peng-Jun (刘鹏军). Chin. Phys. B, 2013, 22(4): 045203.
[9] Selective excitation of the molecular rotational wave packet by two time-delayed laser pulses
Xu Shu-Wu(徐淑武), Huang Yun-Xia(黄云霞), and Ji Xian-Ming(纪宪明) . Chin. Phys. B, 2011, 20(12): 123302.
[10] Coherent control of non-resonant two-photon transition in molecular system
Zhang Hui(张晖), Zhang Shi-An(张诗按), Wang Zu-Geng(王祖赓), and Sun Zhen-Rong(孙真荣). Chin. Phys. B, 2010, 19(11): 113208.
[11] Quantum coherent control of two-photon transitions by square phase-modulation
Zhang Shi-An(张诗按), Wang Zu-Geng(王祖赓), and Sun Zhen-Rong(孙真荣). Chin. Phys. B, 2008, 17(8): 2914-2918.
[12] The study of numerical character for femtosecond pulse shaping
Zou Hua(邹华), Zhu Wei-Hua(朱卫华), and Wang Guo-Dong(王国栋). Chin. Phys. B, 2007, 16(11): 3429-3433.
No Suggested Reading articles found!