Recrystallization of freezable bound water in aqueous solutions of medium concentrations

doi:10.1088/1674-1056/25/7/075101

Abstract

For aqueous solutions with freezable bound water, vitrification and recrystallization are mingled, which brings difficulty to application and misleads the interpretation of relevant experiments. Here, we report a quantification scheme for the freezable bound water based on the water-content dependence of glass transition temperature, by which also the concentration range for the solutions that may undergo recrystallization finds a clear definition. Furthermore, we find that depending on the amount of the freezable bound water, different temperature protocols should be devised to achieve a complete recrystallization. Our results may be helpful for understanding the dynamics of supercooled aqueous solutions and for improving their manipulation in various industries.

Keywords: recrystallization aqueous solution glass transition freezable bound water

Received: 21 February 2016
Revised: 28 March 2016
Accepted manuscript online:

PACS:	51.30.+i	(Thermodynamic properties, equations of state)
	64.70.D-	(Solid-liquid transitions)
	65.20.-w	(Thermal properties of liquids)

Fund:

Project supported by the Knowledge Innovation Project of Chinese Academy of Sciences on Water Science Research (Grant No. KJZD-EW-M03) and the National Natural Science Foundation of China (Grant Nos. 11474325 and 11290161).

Corresponding Authors: Qiang Wang
E-mail: qwang@iphy.ac.cn

Cite this article:

Lishan Zhao(赵立山), Liqing Pan(潘礼庆), Ailing Ji(纪爱玲), Zexian Cao(曹则贤), Qiang Wang(王强) Recrystallization of freezable bound water in aqueous solutions of medium concentrations 2016 Chin. Phys. B 25 075101

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Recrystallization of freezable bound water in aqueous solutions of medium concentrations

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