Second harmonic generation of metal nanoparticles under tightly focused illumination

doi:10.1088/1674-1056/25/3/037803

Abstract The near-field and far-field second harmonic (SH) responses of a metal spherical nanoparticle placed in the focal region of a highly focused beam are investigated by using the calculation model based on three-dimensional finite-difference time-domain (FDTD) method. The results show that off-axis backward-propagating SH response can be reinforced by tightly focusing, due to the increase of the relative magnitude of the longitudinal field component and the phase shift along the propagation direction.

Keywords: second harmonic generation metal nanoparticles focused field

Received: 21 September 2015
Revised: 10 October 2015
Accepted manuscript online:

PACS:	78.67.Bf	(Nanocrystals, nanoparticles, and nanoclusters)
	42.65.Ky	(Frequency conversion; harmonic generation, including higher-order harmonic generation)
	42.25.Dd	(Wave propagation in random media)
	78.68.+m	(Optical properties of surfaces)

Fund: Project supported by the National Natural Science Foundation of China (Grant No. 61378005).

Corresponding Authors: Xiang-Hui Wang
E-mail: wangxianghui@nankai.edu.cn

Cite this article:

Jing-Wei Sun(孙经纬), Xiang-Hui Wang(王湘晖), Sheng-Jiang Chang(常胜江),Ming Zeng(曾明), Na Zhang(张娜) Second harmonic generation of metal nanoparticles under tightly focused illumination 2016 Chin. Phys. B 25 037803

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