| ELECTROMAGNETISM, OPTICS, ACOUSTICS, HEAT TRANSFER, CLASSICAL MECHANICS, AND FLUID DYNAMICS |
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Molecular fluorescence significantly enhanced by gold nanoparticles@zeolitic imidazolate framework-8 |
| Yuyi Zhang(张钰伊)1, Yajie Bian(卞亚杰)1, Wei Zhang(张炜)1, Yiting Liu(刘易婷)1, Xiaolei Zhang(张晓磊)1,2,†, Mengdi Chen(陈梦迪)1,‡, Bingwen Hu(胡炳文)1, and Qingyuan Jin(金庆原)1,3,§ |
1 State Key Laboratory of Precision Spectroscopy, Shanghai Key Laboratory of Magnetic Resonance, School of Physics and Electronic Science, East China Normal University, Shanghai 200241, China;
2 Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan 030006, China;
3 Department of Optical Science and Engineering, Fudan University, Shanghai 200433, China |
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Abstract Noble metal nanoparticles exhibit unique surface plasmon resonance dependent optical properties. On this basis, gold nanoparticles (AuNPs) encapsulated in metal-organic frameworks (MOFs) can form AuNPs@MOFs composites to modulate the optical properties of fluorescent molecules, which is less reported. In this paper, based on the fluorescence enhancement effect of AuNPs on 2-(2-hydroxyphenyl)-1H-benzimidazole (HPBI) molecules, zeolitic imidazolate framework-8 (ZIF-8) crystals with structural stability were introduced. AuNPs@ZIF-8 exhibited a significantly pronounced fluorescence enhancement of the HPBI molecules. In addition, by comparing the fluorescence characteristics of the HPBI molecules adsorbed on AuNPs@ZIF-8 and those captured in AuNPs@ZIF-8, we found that the ZIF-8 can act as a spacer layer with highly effective near-field enhancement. All our preliminary results shed light on future research on the composite structures of noble metal particles and MOFs for fluorescent probes and sensing applications.
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Received: 28 May 2022
Revised: 14 July 2022
Accepted manuscript online: 18 July 2022
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PACS:
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42.70.-a
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(Optical materials)
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Corresponding Authors:
Xiaolei Zhang, Mengdi Chen, Qingyuan Jin
E-mail: xlzhang@admin.ecnu.edu.cn;mdchen@lps.ecnu.edu.cn;qyjin@fudan.edu.cn
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Cite this article:
Yuyi Zhang(张钰伊), Yajie Bian(卞亚杰), Wei Zhang(张炜), Yiting Liu(刘易婷), Xiaolei Zhang(张晓磊),Mengdi Chen(陈梦迪), Bingwen Hu(胡炳文), and Qingyuan Jin(金庆原) Molecular fluorescence significantly enhanced by gold nanoparticles@zeolitic imidazolate framework-8 2023 Chin. Phys. B 32 054208
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