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Chin. Phys. B, 2023, Vol. 32(3): 030301    DOI: 10.1088/1674-1056/aca392
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Formalism of rotating-wave approximation in high-spin system with quadrupole interaction

Wen-Kui Ding(丁文魁)1,2,† and Xiao-Guang Wang(王晓光)1,3,‡
1 Key Laboratory of Optical Field Manipulation of Zhejiang Province and Department of Physics, Zhejiang Sci-Tech University, Hangzhou 310018, China;
2 Zhejiang Institute of Modern Physics and Department of Physics, Zhejiang University, Hangzhou 310027, China;
3 Graduate School of China Academy of Engineering Physics, Beijing 100193, China
Abstract  We investigate the rotating wave approximation applied in the high-spin quantum system driven by a linearly polarized alternating magnetic field in the presence of quadrupole interactions. The conventional way to apply the rotating wave approximation in a driven high-spin system is to assume the dynamics being restricted in the reduced Hilbert space. However, when the driving strength is relatively strong or the driving is off resonant, the leakage from the target resonance subspace cannot be neglected for a multi-level quantum system. We propose the correct formalism to apply the rotating wave approximation in the full Hilbert space by taking this leakage into account. By estimating the operator fidelity of the time propagator, our formalism applied in the full Hilbert space unambiguously manifests great advantages over the conventional method applied in the reduced Hilbert space.
Keywords:  rotating wave approximation      quadrupole interaction      high-spin system  
Received:  02 June 2022      Revised:  09 September 2022      Accepted manuscript online:  17 November 2022
PACS:  03.65.-w (Quantum mechanics)  
  76.60.Gv (Quadrupole resonance)  
Fund: Project supported by the National Key Research and Development Program of China (Grant Nos. 2017YFA0304202 and 2017YFA0205700), the National Natural Science Foundation of China (Grant Nos. 11875231 and 11935012), and the Fundamental Research Funds for the Central Universities (Grant No. 2018FZA3005).
Corresponding Authors:  Wen-Kui Ding     E-mail:  wenkuiding@zju.edu.cn;xgwang@zstu.edu.cn

Cite this article: 

Wen-Kui Ding(丁文魁) and Xiao-Guang Wang(王晓光) Formalism of rotating-wave approximation in high-spin system with quadrupole interaction 2023 Chin. Phys. B 32 030301

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