Please wait a minute...
Chin. Phys. B, 2020, Vol. 29(8): 083304    DOI: 10.1088/1674-1056/aba9b9
ATOMIC AND MOLECULAR PHYSICS Prev   Next  

Responsive mechanism and coordination mode effect of a bipyridine-based two-photon fluorescent probe for zinc ion

Han Zhang(张瀚), Zhe Shao(邵哲), Ke Zhao(赵珂)
School of Physics and Electronics, Shandong Normal University, Jinan 250358, China
Abstract  The properties of one-photon absorption (OPA), emission and two-photon absorption (TPA) of a bipyridine-based zinc ion probe are investigated employing the density functional theory in combination with response functions. The responsive mechanism and coordination mode effect are explored. The structural fluctuation is illustrated by molecular dynamics simulation. The calculated OPA and emission wavelengths of the probe are consistent with the experimental data. It is found that the red-shift of OPA wavelength and the enhancement of TPA intensity are induced by the increased intra-molecular charge transfer mechanism upon metal binding. The structural fluctuation could result in the blue-shift of TPA wavelength and the decrease of the TPA cross section. The TPA properties are quite different among the zinc complexes with different coordination modes. The TPA wavelength of the complexes with two ligands is close to that of the probe, which is in agreement with the experimental observation.
Keywords:  two-photon absorption      fluorescent probe      zinc ion      coordination mode      bipyridine  
Received:  07 May 2020      Revised:  02 June 2020      Accepted manuscript online: 
PACS:  33.20.-t (Molecular spectra)  
  42.65.-k (Nonlinear optics)  
  47.11.Mn (Molecular dynamics methods)  
  82.30.Fi (Ion-molecule, ion-ion, and charge-transfer reactions)  
Fund: Project supported by the Natural Science Foundation of Shandong Province, China (Grant No. ZR2014AM026).
Corresponding Authors:  Ke Zhao     E-mail:  zhaoke@sdnu.edu.cn

Cite this article: 

Han Zhang(张瀚), Zhe Shao(邵哲), Ke Zhao(赵珂) Responsive mechanism and coordination mode effect of a bipyridine-based two-photon fluorescent probe for zinc ion 2020 Chin. Phys. B 29 083304

[1] Denk W, Strickler J H and Webb W W 1990 Science 248 73
[2] Yao S and Belfield K D 2012 Eur. J. Org. Chem. 2012 3199
[3] Kim D, Ryu H G and Ahn K H 2014 Org. Biomol. Chem. 12 4550
[4] Kim H M and Cho B R 2015 Chem. Rev. 115 5014
[5] Kim H M and Cho B R 2011 Chem. Asian J. 6 58
[6] Sarkar A R, Kang D E, Kim H M and Cho B R 2014 Inorg. Chem. 53 1794
[7] Sumalekshmy S and Fahrni C J 2011 Chem. Mater. 23 483
[8] Kim D, Singha S, Wang T, Seo E, Lee J H, Lee S J, Kim K H and Ahn K H 2012 Chem. Commun. 48 10243
[9] Kim H M, An M J, Hong J H, Jeong B H, Kwon O, Hyon J Y, Hong S C, Lee K J and Cho B R 2008 Angew. Chem. Int. Ed. 47 2231
[10] Kim H J, Heo C H and Kim H M 2013 J. Am. Chem. Soc. 135 17969
[11] Das S K, Lim C S, Yang S Y, Han J H and Cho B R 2012 Chem. Commun. 48 8395
[12] Masanta G, Heo C H, Lim C S, Bae S K, Cho B R and Kim H M 2012 Chem. Commun. 48 3518
[13] Zhang Y, Wang J, Jia P, Yu X, Liu H, Liu X, Zhao N and Huang B 2010 Org. Biomol. Chem. 8 4582
[14] Bush A I, Pettingell W H, Multhaup G, Paradis M D, Vonsattel J P, Gusella J F, Beyreuther K, Masters C L and Tanzi R E 1994 Science 265 1464
[15] Cuajungco M P and Lees G J 1997 Neurobiol. Dis. 4 137
[16] Bush A I and Tanzi R E 2002 Proc. Natl. Acad. Sci. USA 99 7317
[17] Huang S, Zou L Y, Ren A M, Guo J F, Liu X T, Feng J K and Yang B Z 2013 Inorg. Chem. 52 5702
[18] Huang S, Yang B Z and Ren A M 2016 J. Mol. Struc. 1114 65
[19] Wang D, Ren A M, Zou L Y, Guo J F and Huang S 2017 J. Photoch. Photobio. A 341 20
[20] Wang D, Guo J F, Ren A M, Huang S, Zhang L and Feng J K 2014 J. Phys. Chem. B 118 10101
[21] Bednarska J, Zaleśny R, Murugan N A, Bartkowiak W, Ågren H and Odelius M 2016 J. Phys. Chem. B 120 9067
[22] Zhu M Y, Zhao K, Song J and Wang C K 2018 Chin. Phys. B 27 023302
[23] Zhang Y J, Zhang Q Y, Ding H J, Song X N and Wang C K 2015 Chin. Phys. B 24 023301
[24] Zhao K, Song J, Zhu M Y, Zhang H and Wang C K 2018 Chin. Phys. B 27 103301
[25] Li W, Fang B, Jin M and Tian Y 2017 Anal. Chem. 89 2553
[26] Zhao K, Song J and Zhang H 2019 Acta Phys. Sin. 68 183101(in Chinese)
[27] Luo Y, Norman P, Macak P and Ågren H 2000 J. Phys. Chem. A 104 4718
[28] Olsen J and Jorgensen P 1985 J. Chem. Phys. 82 3235
[29] Frisch M J, Trucks G W, Schlegel H B, et al. Gaussian 16, Revision C.01 Gaussian 2016 Inc. Wallingford CT
[30] Aidas K, Angeli C, Bak K L and et al. 2014 WIREs Comput. Mol. Sci. 4 269
[31] Wang J, Wolf R M, Caldwell J W, Kollman P A and Case D A 2004 J. Comput. Chem. 25 1157
[32] Wang J, Wolf R M, Caldwell J W, Kollman P A and Case D A 2005 J. Comput. Chem. 26 114
[33] Case D A, Babin V, Berryman J T, et al. 2014 AMBER 14 (San Francisco:University of California)
[34] Zhao K, Liu P W, Wang C K and Luo Y 2010 J. Phys. Chem. B 114 10814
[35] Zhao K and Luo Y 2010 J. Phys. Chem. B 114 13167
[36] van der Spoel D, Lindahl E and Hess B 2014 GROMACS User Manual version 4.6.7, www.gromacs.org
[37] Xue L, Fang Z, Li G and Wang H 2011 Sens. Actuator B-Chem. 156 410
[38] Mu X, Wang J and Sun M 2019 J. Phys. Chem. C 123 14132
[39] Mu X, Wang X, Quan J and Sun M 2020 J. Phys. Chem. C 124 4968
[40] Mu X, Zong H, Zhu L and Sun M 2020 J. Phys. Chem. C 124 2319
[1] Computational design of ratiometric two-photon fluorescent Zn2+ probes based on quinoline and di-2-picolylamine moieties
Zhe Shao(邵哲), Wen-Ying Zhang(张纹莹), and Ke Zhao(赵珂). Chin. Phys. B, 2022, 31(5): 053302.
[2] Zebrafish imaging and two-photon fluorescence imaging using ZnSe quantum dots
Nan-Nan Zhang(张楠楠), Li-Ya Zhou(周立亚), Xiao Liu(刘潇), Zhong-Chao Wei(韦中超), Hai-Ying Liu(刘海英), Sheng Lan(兰胜), Zhao Meng(孟钊), and Hai-Hua Fan(范海华). Chin. Phys. B, 2021, 30(4): 044204.
[3] Ultrafast carrier dynamics of Cu2O thin film induced by two-photon excitation
Jian Liu(刘建), Jing Li(李敬), Kai-Jun Mu(牧凯军), Xin-Wei Shi(史新伟), Jun-Qiao Wang(王俊俏), Miao Mao(毛淼), Shu Chen(陈述), and Er-Jun Liang(梁二军). Chin. Phys. B, 2021, 30(11): 114205.
[4] Soliton evolution and control in a two-mode fiber with two-photon absorption
Qianying Li(李倩颖). Chin. Phys. B, 2020, 29(1): 014204.
[5] High-power ultraviolet 278-nm laser from fourth-harmonic generation of an Nd: YAG amplifier in CsB3O5 crystal
Miao He(何苗), Feng Yang(杨峰), Cheng Dong(董程), Zhi-Chao Wang(王志超), Lei Yuan(袁磊), Yi-Ting Xu(徐一汀), Guo-Chun Zhang(张国春), Zhi-Min Wang(王志敏), Yong Bo(薄勇), Qin-Jun Peng(彭钦军), Da-Fu Cui(崔大复), Yi-Cheng Wu(吴以成), Zu-Yan Xu(许祖彦). Chin. Phys. B, 2018, 27(5): 054211.
[6] Facile and controllable synthesis of molybdenum disulfide quantum dots for highly sensitive and selective sensing of copper ions
Xue Li(李雪), Da-Wei He(何大伟), Yong-Sheng Wang(王永生), Yin Hu(胡音), Xuan Zhao(赵宣), Chen Fu(付晨), Jing-Yan Wu(吴静燕). Chin. Phys. B, 2018, 27(5): 056104.
[7] Responsive mechanism and molecular design of di-2-picolylamine-based two-photon fluorescent probes for zinc ions
Mei-Yu Zhu(朱美玉), Ke Zhao(赵珂), Jun Song(宋军), Chuan-Kui Wang(王传奎). Chin. Phys. B, 2018, 27(2): 023302.
[8] Up-conversion luminescence tuning in Er3+-doped ceramic glass by femtosecond laser pulse at different laser powers
Wen-Jing Cheng(程文静), Guo Liang(梁果), Ping Wu(吴萍), Shi-Hua Zhao(赵世华), Tian-Qing Jia(贾天卿), Zhen-Rong Sun(孙真荣), Shi-An Zhang(张诗按). Chin. Phys. B, 2018, 27(12): 123201.
[9] Optical power limiting of ultrashort hyper-Gaussian pulses in cascade three-level system
Ji-Cai Liu(刘纪彩), Fen-Fen Guo(郭芬芬), Ya-Nan Zhao(赵亚男), Xing-Zhe Li(李兴哲). Chin. Phys. B, 2018, 27(10): 104209.
[10] Isomerism and coordination mode effects on two-photon absorption of tris(picolyl)amine-based fluorescent probes for zinc ions
Ke Zhao(赵珂), Jun Song(宋军), Mei-Yu Zhu(朱美玉), Han Zhang(张瀚), Chuan-Kui Wang(王传奎). Chin. Phys. B, 2018, 27(10): 103301.
[11] Simulating resonance-mediated two-photon absorption enhancement in rare-earth ions by a rectangle phase modulation
Da-Long Qi(齐大龙), Ye Zheng(郑烨), Wen-Jing Cheng(程文静), Yun-Hua Yao(姚云华), Lian-Zhong Deng(邓联忠), Dong-Hai Feng(冯东海), Tian-Qing Jia(贾天卿), Zhen-Rong Sun(孙真荣), Shi-An Zhang(张诗按). Chin. Phys. B, 2018, 27(1): 013202.
[12] Responsive mechanism of three novel hypochlorous acid fluorescent probes and solvent effect on their sensing performance
Yong Zhou(周勇), Yun-Kun Wang(王云坤), Xiao-Fei Wang(王晓菲), Yu-Jin Zhang(张玉瑾), Chuan-Kui Wang(王传奎). Chin. Phys. B, 2017, 26(8): 083102.
[13] Responsive mechanism of 2-(2'-hydroxyphenyl)benzoxazole-based two-photon fluorescent probes for zinc and hydroxide ions
Zhang Yu-Jin (张玉瑾), Zhang Qiu-Yue (张秋月), Ding Hong-Juan (丁红娟), Song Xiu-Neng (宋秀能), Wang Chuan-Kui (王传奎). Chin. Phys. B, 2015, 24(2): 023301.
[14] Polarization and phase control of two-photon absorption in an isotropic molecular system
Lu Chen-Hui (卢晨晖), Zhang Hui (张晖), Zhang Shi-An (张诗按), Sun Zhen-Rong (孙真荣). Chin. Phys. B, 2012, 21(12): 123202.
[15] Influence of rotational isomerism on two-photon absorption properties of FTC chromophores
Han Guang-Chao (韩广超), Zhao Ke (赵珂), Liu Peng-Wei (刘朋伟), Zhang Li-Li (张立立 ). Chin. Phys. B, 2012, 21(11): 118201.
No Suggested Reading articles found!