Nonvolatile photorefractive properties in triply doped stoichiometric Mg:Fe:Mn:LiTaO3 crystals
Sun Ting (孙婷)a, Zhang Xiao-Dong (张晓东)b, Sun Liang (孙亮)c d, Wang Rui (王锐)a
a Department of Applied Chemistry, Harbin Institute of Technology, Harbin 150001, China; b School of Materials Science and Engineering, Harbin Institute of Technology, Harbin 150001, China; c School of Chemical Engineering & Technology, Harbin Institute of Technology, Harbin 150001, China; d School of Physics and Electronic Engineering, Yibin University, Yibin 644000, China
Abstract We have grown triply doped Mg:Fe:Mn:LiTaO3 crystals with near stoichiometry using the top seeded solution growth technique. The defect structure was investigated by infrared absorption spectra and Curie temperature. Using a blue laser as the source, excellent photorefractive properties were obtained. Nonvolatile holographic storage properties were investigated using the dual wavelength technique. We got a very high fixed diffraction efficiency and nonvolatile holographic storage sensitivity. The blue light has more than enough energy to excite holes of deep (Mn) and shallow (Fe) trap centers with the same phase, which enhance dramatically the blue photorefractive properties and the nonvolatile holographic storage. Mg2+ ion is no longer damage resistant at blue laser, but enhances photorefractive characteristics.
Fund: Project supported by the National Natural Science Foundation of China (Grant No. 51202045), the Postdoctoral Science Foundation of Heilongjiang Province, China, and the Fundamental Research Funds for the Central Universities of Ministry of Education of China (Grant No. HIT. NSRIF. 2013004).
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