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Special Issue:
TOPICAL REVIEW — Advanced calculation & characterization of energy storage materials & devices at multiple scale
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| TOPICAL REVIEW—Advanced calculation & characterization of energy storage materials & devices at multiple scale |
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Neutron-based characterization techniques for lithium-ion battery research |
| Enyue Zhao(赵恩岳)1,2, Zhi-Gang Zhang(张志刚)1,2, Xiyang Li(李西阳)2, Lunhua He(何伦华)1,2,4, Xiqian Yu(禹习谦)2, Hong Li(李泓)2, Fangwei Wang(王芳卫)1,2,3,4 |
1 Songshan Lake Materials Laboratory, Dongguan 523808, China;
2 Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China;
3 School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 101408, China;
4 China Spallation Neutron Source(CSNS), Dongguan 523808, China |
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Abstract During the past decades, Li-ion batteries have been one of the most important energy storage devices. Large-scale energy storage requires Li-ion batteries which possess high energy density, low cost, and high safety. Other than advanced battery materials, in-depth understanding of the intrinsic mechanism correlated with cell reaction is also essential for the development of high-performance Li-ion battery. Advanced characterization techniques, especially neutron-based techniques, have greatly promoted Li-ion battery researches. In this review, the characteristics or capabilities of various neutron-based characterization techniques, including elastic neutron scattering, quasi-elastic neutron scattering, neutron imaging, and inelastic neutron scattering, for the related Li-ion-battery researches are summarized. The design of in-situ/operando environment is also discussed. The comprehensive survey on neutron-based characterizations for mechanism understanding will provide guidance for the further study of high-performance Li-ion batteries.
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Received: 31 October 2019
Revised: 24 November 2019
Accepted manuscript online:
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PACS:
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82.47.Aa
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(Lithium-ion batteries)
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82.45.Fk
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(Electrodes)
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| Fund: Project supported by the National Key R&D Program of China (Grant No. 2016YFA0401503), the National Materials Genome Project of China (Grant No. 2016YFB0100106), and the National Natural Science Foundation of China (Grant No. 11675255). |
Corresponding Authors:
Fangwei Wang
E-mail: fwwang@iphy.ac.cn
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Cite this article:
Enyue Zhao(赵恩岳), Zhi-Gang Zhang(张志刚), Xiyang Li(李西阳), Lunhua He(何伦华), Xiqian Yu(禹习谦), Hong Li(李泓), Fangwei Wang(王芳卫) Neutron-based characterization techniques for lithium-ion battery research 2020 Chin. Phys. B 29 018201
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