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Improvement in the calculation of anti-Stokes energy transfer and experimental justification based on Er0.01YbxY1-0.01-xVO4 crystal |
Chen Xiao-Bo(陈晓波)a) †, Lu Jian(卢建)b), Zhang Yun-Zhi(张蕴芝)b), Xu Xiao-Ling(徐小灵)a), Feng Bao-Hua(冯宝华)b), Wang Ce(王策)a), Gregory J. Salamoc), and Yang Guo-Jian(杨国建)a) |
a Nuclear Science & Technology School and Analytical Testing Center, Applied Optics Beijing Area Major Laboratory, Beijing Normal University, Beijing 100875, China; b Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China; c University Arkansas, Department of Physics, Fayetteville, AR 72701, USA |
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Abstract The improvement on the calculation of anti-Stokes energy transfer rate is studied in the present work. The additional proportion coefficient between Stokes and anti-Stokes light intensities of quantum Raman scattering theory as compared with the classical Raman theory is introduced to successfully describe the anti-Stokes energy transfer. The theoretical formula for the improvement on the calculation of anti-Stokes energy transfer rate is derived for the first time in this study. The correctness of introducing coefficient exp{ΔE / kT} from well-known Raman scatter theory is demonstrated also. Moreover, the experimental lifetime measurement in Er0.01YbxY1-0.01-xVO4 crystal is performed to justify the validity of our important improvement in the original phonon-assisted energy transfer theory for the first time.
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Received: 03 August 2009
Revised: 21 March 2010
Accepted manuscript online:
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Cite this article:
Chen Xiao-Bo(陈晓波), Lu Jian(卢建), Zhang Yun-Zhi(张蕴芝), Xu Xiao-Ling(徐小灵), Feng Bao-Hua(冯宝华), Wang Ce(王策), Gregory J. Salamo, and Yang Guo-Jian(杨国建) Improvement in the calculation of anti-Stokes energy transfer and experimental justification based on Er0.01YbxY1-0.01-xVO4 crystal 2010 Chin. Phys. B 19 097804
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